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Curriculum Vitae - APC - Université Paris Diderot-Paris 7

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Figure 5. A- and B-Sketch of Quincke rollers in a Hele-Shaw microfluidic cell. Top views. A-Dilute system,<br />

uncorrelated velocities. B- Concentrated system: Collective directed motion? C-Tentative phase diagram.<br />

The first series of experiment will focus on homogenous channel geometries, namely wide<br />

isotropic shallow cells. The following question will be addressed first: can one observe a<br />

spontaneous collective and directed motion, viz. can Quincke rollers form swarms? An<br />

experimental fact, strongly suggests than a spontaneous symmetry breaking should occur in<br />

this system at sufficiently high concentration. As a matter of fact, it has been shown, that<br />

when an external macroscopic shear is applied to a suspension of Quincke colloids, they all<br />

rotate coherently, with the imposed fluid vorticity. This symmetry breaking enforced by the<br />

external drive results in an electrorheological shear thinning [19]. When rolling on a solid<br />

substrate, the colloids induce a net flow over distances comparable, at least, to their diameter.<br />

This induced flow is therefore expected to orient the rotation of the surrounding particle and<br />

yield correlated motion. At sufficiently high concentration, this local coupling is expected to<br />

propagate up to the system size. Practically, the height of the microfluidic channels containing<br />

the colloids will be chosen much larger that the colloid diameter to maximize the<br />

hydrodynamic couplings (height~100 microns, for micron size colloids). To check our<br />

prediction, we will measure the average particle velocity for increasing concentrations and<br />

electric field amplitudes. To distinguish between a crossover regime and a spontaneous<br />

symmetry-breaking scenario, we will measure the velocity-velocity correlation length and the<br />

lifetime of the coherent clusters as a function of the electric field amplitude for various<br />

concentrations. The magnitude of the E field is the parameter, which we control with the<br />

better accuracy. We shall notice that, this phenomenology is not opposed to the instability the<br />

polar phases predicted by the current models for active suspensions [14]. This theoretical<br />

prediction indeed applies only to anisotropic particles, having a velocity slave to the particle<br />

orientation. In our experiments, the translation speed of our colloids is not set by any<br />

permanent shape asymmetry; the direction of the roller velocity is set by its surface charge<br />

distribution, which is only weakly slaved to the geometrical orientation of the particle. In<br />

addition, the hydrodynamic coupling between two Quincke rollers is likely to differ from the<br />

conventional force-dipole picture. Therefore, our system will not process the two features<br />

responsible for the destabilization of the splay/bend modes of the active polar phase [14].<br />

To rationalize quantitatively our experimental findings, we will pursue our ongoing work on the<br />

modeling of active suspensions in collaboration with Eric Lauga UCSD. In line with the remark<br />

made above, we will need first to construct a realistic model for the roller-roller scattering<br />

process. These models will be built upon the experimental characterization of the roller-roller<br />

collision rules, which we will extract from direct image analysis in dilute systems.<br />

4.5.2.2. Traffic dynamics along colloidal roads.<br />

As a first step toward the traffic in more complex geometries, we will investigate, the<br />

collective dynamic of Quincke colloids along a 1D track, see Fig. 6. The colloidal tracks will<br />

be made by direct lithography on a conducting glass slides (ITO coating). The colloids will be

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