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Abstracts - Dipartimento di Elettronica Applicata

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Meta 2010 & FEM 2010 – Rome, 13-15 December 2010<br />

Second Harmonic Generation in Gold<br />

Nanoantennas<br />

Alessio Benedetti, Marco Centini, Concita Sibilia, Mario Bertolotti<br />

<strong>Dipartimento</strong> <strong>di</strong> Scienze <strong>di</strong> Base e Applicate per l'Ingegneria- Sez Fisica.<br />

Sapienza Università <strong>di</strong> Roma. Via A. Scarpa 16 00161 Roma – Italy<br />

E-mail: concita.sibilia@uniroma1.it<br />

The second order nonlinear response from flat metal screens has been widely<br />

investigated, both theoretically and experimentally, from the late 1960s–1980s<br />

[1]. The last few years witnessed renewed interest in the study of nonlinear<br />

second order properties of metal/<strong>di</strong>electric composites thanks to the<br />

development of nanotechnologies and nanoscience. In this work we study the<br />

enhancement of SHG due to the interaction between two 3D metallic wires<br />

with sections of arbitrary shape, focusing on the effect of the surface<br />

morphology and defects. We also analyze the possibility of tailoring the<br />

emission pattern. Numerical calculations have been performed applying a<br />

Green's tensor method [2,3]. The SHG as a function of the wires cross section<br />

size is investigated in both the near and far field regimes. An accurate study of<br />

the effects related to the nonlinear surface contribution for the SHG process,<br />

and of the mo<strong>di</strong>fication of the nonlinear scattering cross section (NLSCS) due<br />

to surface roughness in realistic samples has been performed. Figure 1a shows<br />

the sample description: we note that the shape can be arbitrarily mo<strong>di</strong>fied to<br />

take into account for surface roughness and for <strong>di</strong>screpancies from perfect<br />

rectangular shape. In Figure 1b we plot the NLSCS for a gold nanoantenna<br />

calculated when a pump field consisting of a plane wave at 800 nm, polarized<br />

along the long axis <strong>di</strong>rection of the rods is considered.<br />

e) b)<br />

Figure 1: a)Sample which takes into account the imperfections and roughnesses of the metal<br />

surface. b) 3D Nonlinear SH-Scattering Cross Section for a gold nanoantenna (λ=400nm).<br />

References<br />

[1] J. E. Sipe and G. I. Stegeman, V. M. Agranovich and D. L. Mills, eds. (North-Holland,<br />

1982).<br />

[2] M. Paulus and O. J. F. Martin, J. Opt. Soc. Am. A 18, 854–861 (2001).<br />

[3] A. Benedetti et al., JOSA B 27, 3, 408-416 (2010)).<br />

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