Euradwaste '08 - EU Bookshop - Europa

Euradwaste '08 - EU Bookshop - Europa Euradwaste '08 - EU Bookshop - Europa

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Phase-Out TRU Transmutation Scenarios studies based on Fast Neutron ADS Systems, E. Gonzalez and M. Embid-Segura. 7th NEA Information Exch. Meeting on Actinide and Fission Product P&T, Jeju (Republic of Korea), 14-16 October 2002. [19] Partitioning and Transmutation Potential for Waste Minimization in a Regional Context, Salvatores M. et al., 8th NEA Information Exch. Meeting on Actinide and Fission Product P&T, University of Nevada, Las Vegas 9-11 November, 2004. [20] Impact of Advanced Fuel Cycle Scenarios on Geological Disposal. J. Marivoet et al.. Proc. Euradwaste '08 Conference (2008). 140

Impact of Advanced Fuel Cycle Scenarios on Geological Disposal Summary Jan Marivoet 1 , Miguel Cuñado 2 , Simon Norris 3 , Eef Weetjens 1 1 SCK·CEN, Mol, Belgium 2 Enresa, Madrid, Spain 3 NDA RWMD, Harwell, United Kingdom The impact of advanced nuclear fuel cycles on radioactive waste management and geological disposal has been evaluated within the Red-Impact project. Five representative fuel cycles, which were considered in equilibrium, were identified and the resulting waste volumes and compositions were estimated. Repository designs for disposal in hard rock and clay formations, developed by national radioactive waste management agencies for today's waste types, were used as reference concepts. After a 50 years cooling time, the heat generated in the highlevel radioactive waste arising from advanced fuel cycles is significantly lower than that in spent fuel from the present "once through" fuel cycle. This would allow the dimensions of a geological repository to be comparatively reduced. The impact of advanced fuel cycles on the radiological consequences in the case of the expected evolution or reference scenario is rather limited. This is because the maximum dose in this scenario, which is calculated to occur a few tens of thousands of years after the disposal of the waste and is associated with radionuclide transport in groundwater, is essentially due to mobile fission and activation products; as geological disposal systems are very effective at retarding the migration of actinides, the contribution of the actinides to the effective dose is limited. The associated intermediate-level waste contains considerable amounts of mobile activation products; these species persist in giving relatively high post-closure doses. On the other hand, for the variant human intrusion scenario, calculated doses to a geotechnical worker resulting from inadvertent intrusion into a high-level waste repository are significantly reduced in the case of advanced fuel cycles, because of the much lower actinide content of the waste. However, it should be noted that the realism of human intrusion scenarios, and the weight that could be placed on the associated outcome, is strongly debatable. 1. Introduction During the last 15 years, various studies investigating the role and feasibility of partitioning and transmutation (P&T) within nuclear fuel cycles have been carried out. The European Commission (EC) has initiated several research projects within its various framework programmes on the possibilities of applying P&T techniques to reduce the inventories of long-lived isotopes in radioactive waste [1,2]. The final objective of these EC-funded research projects is to lay the groundwork for future sustainable nuclear fuel cycle strategies involving transmutation in a dedicated waste-burning accelerator driven system (ADS) or in future Generation IV fast neutron reactors (FR). The Nuclear Energy Agency (NEA) has conducted a series of studies on P&T systems [3-5], which focused on a review of the progress in the separation of long-lived actinides and fission products, the options for their transmutation, and the possible benefit for the management of the radioactive waste. The International Atomic Energy Agency (IAEA) has published reports on the implications of P&T on nuclear fuel cycles and waste management [6,7]. Within the Generation IV International Forum [8], 141

Impact of Advanced Fuel Cycle Scenarios on Geological Disposal<br />

Summary<br />

Jan Marivoet 1 , Miguel Cuñado 2 , Simon Norris 3 , Eef Weetjens 1<br />

1 SCK·CEN, Mol, Belgium<br />

2 Enresa, Madrid, Spain<br />

3 NDA RWMD, Harwell, United Kingdom<br />

The impact of advanced nuclear fuel cycles on radioactive waste management and geological<br />

disposal has been evaluated within the Red-Impact project. Five representative fuel cycles,<br />

which were considered in equilibrium, were identified and the resulting waste volumes and<br />

compositions were estimated. Repository designs for disposal in hard rock and clay formations,<br />

developed by national radioactive waste management agencies for today's waste types,<br />

were used as reference concepts. After a 50 years cooling time, the heat generated in the highlevel<br />

radioactive waste arising from advanced fuel cycles is significantly lower than that in<br />

spent fuel from the present "once through" fuel cycle. This would allow the dimensions of a<br />

geological repository to be comparatively reduced. The impact of advanced fuel cycles on the<br />

radiological consequences in the case of the expected evolution or reference scenario is rather<br />

limited. This is because the maximum dose in this scenario, which is calculated to occur a few<br />

tens of thousands of years after the disposal of the waste and is associated with radionuclide<br />

transport in groundwater, is essentially due to mobile fission and activation products; as geological<br />

disposal systems are very effective at retarding the migration of actinides, the contribution<br />

of the actinides to the effective dose is limited. The associated intermediate-level waste<br />

contains considerable amounts of mobile activation products; these species persist in giving<br />

relatively high post-closure doses. On the other hand, for the variant human intrusion scenario,<br />

calculated doses to a geotechnical worker resulting from inadvertent intrusion into a<br />

high-level waste repository are significantly reduced in the case of advanced fuel cycles, because<br />

of the much lower actinide content of the waste. However, it should be noted that the<br />

realism of human intrusion scenarios, and the weight that could be placed on the associated<br />

outcome, is strongly debatable.<br />

1. Introduction<br />

During the last 15 years, various studies investigating the role and feasibility of partitioning and<br />

transmutation (P&T) within nuclear fuel cycles have been carried out. The European Commission<br />

(EC) has initiated several research projects within its various framework programmes on the possibilities<br />

of applying P&T techniques to reduce the inventories of long-lived isotopes in radioactive<br />

waste [1,2]. The final objective of these EC-funded research projects is to lay the groundwork for<br />

future sustainable nuclear fuel cycle strategies involving transmutation in a dedicated waste-burning<br />

accelerator driven system (ADS) or in future Generation IV fast neutron reactors (FR). The Nuclear<br />

Energy Agency (NEA) has conducted a series of studies on P&T systems [3-5], which focused on a<br />

review of the progress in the separation of long-lived actinides and fission products, the options for<br />

their transmutation, and the possible benefit for the management of the radioactive waste. The International<br />

Atomic Energy Agency (IAEA) has published reports on the implications of P&T on<br />

nuclear fuel cycles and waste management [6,7]. Within the Generation IV International Forum [8],<br />

141

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