Euradwaste '08 - EU Bookshop - Europa

Euradwaste '08 - EU Bookshop - Europa Euradwaste '08 - EU Bookshop - Europa

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agreed for support through an integrated effort at the European level despite the diversity among the Member States in terms of the fuel cycle policy. A key criterion for the selection of projects and activities to be co- funded by the European Union is the “European Added Value”. As shown in Fig.1 the projects are organised coherently to provide all elements necessary for a better understanding and control over the various components required for the deployment of P&T at an industrial scale level in the 2020 to 2040 time scale. Fig. 1 EC co-funded P&T projects 2.1 The Coordinated Action PATEROS This Coordinated Action aims at the establishment of a European vision for the deployment of P&T up to the level of industrial implementation. It should serve as a basis for decisions on advanced fuel cycles leading to a sustainable nuclear energy and thus is intended to provide input for the structuring of the corresponding part of the Sustainable Nuclear Energy Technology Platform (SNE-TP). Performance characteristics of various options for transmutation systems were evaluated e.g. Multi recycling in fast reactors (FR) of TRU unloaded from LWRs and, successively, from FRs. Reduction of TRU inventory in fuels unloaded from LWRs. Reduction of MA inventory. Use of different fuel types and coolants in critical systems as well as the impact of different recycling (e.g. homogeneous and heterogeneous MA recycling) has been studied [1]. Such strategies necessitate fuels with variable amounts of MA incorporated in conventional fuels. The results of the PATEROS programme have been complemented by those obtained in the EISOFAR project for sodium cooled systems and the ELSY project for lead cooled systems. Though dependent on design optimisation, the generic transmutation characteristics for different coolants and homogeneous re- 114

cycling fuels do not vary significantly for critical low conversion ratio systems. In general, the introduction of MA leads to a beneficial effect on the reactivity variation with burn-up but results in slightly worse reactivity feedback effects concerning the Doppler and the void reactivity. For large size sodium cooled reactors (SFR) with about 3000 MWt a maximum MA content of 2.5 to 3.5 % is acceptable from a safety point of view. In the case of a large gas cooled fast reactor (GFR), this upper limit could become higher i.e. up to about 5 to 7 %. A yet higher MA content (e.g. for U-free fuels with a MA content > 40 %) can result in a very significant decrease of the delayed neutron fraction which might result in problems regarding safety. Heterogeneous actinide recycling provides the possibility to circumvent this disadvantage and - more importantly - to disconnect the minor actinide cycle from the conventional fuel cycle. 2.2 Fuels for homogeneous recycling The incorporation of minor actinides into fuels for fast reactors represents an immense challenge. The reprocessing plants must deliver actinide streams suitable for conversion to solid and further processing. Traditionally, mixed oxide fast reactor fuels have been prepared from UO2 and PuO2 powders fed from the separated U and Pu streams in the PUREX process enabling flexibility in preparing fuels with varying Pu enrichment via standard powder metallurgical routes. Introduction of minor actinides (MA) will immediately require full automation of the entire fabrication process, including assembly production, transport and storage. Research on minor actinide bearing fuels is still in its infancy; and major experimental programmes are needed before such fuels can be licensed for industrial application. The SUPERFACT experiment [2, 3] represented the first major milestone in this area. A total of eight fuel pins with pair wise four fuels were manufactured at the JRC-ITU using the sol gel liquid to solid conversion route, as this method has the distinct advantage that it is nearly dust free, and thereby minimises radiation dose risk within the facility. The selected compositions represent both homogeneous and heterogeneous (MA targets) minor actinide recycling in fast reactors (see Table 1). The irradiation was performed during 360 EFPD (equivalent full power days) in a standard Phenix bundle, within which the standard MOX fuel operated at linear powers of 430 and 370 at beginning and end of life (BOL and EOL), respectively. 115

agreed for support through an integrated effort at the European level despite the diversity among the<br />

Member States in terms of the fuel cycle policy. A key criterion for the selection of projects and<br />

activities to be co- funded by the European Union is the “European Added Value”. As shown in<br />

Fig.1 the projects are organised coherently to provide all elements necessary for a better understanding<br />

and control over the various components required for the deployment of P&T at an industrial<br />

scale level in the 2020 to 2040 time scale.<br />

Fig. 1 EC co-funded P&T projects<br />

2.1 The Coordinated Action PATEROS<br />

This Coordinated Action aims at the establishment of a European vision for the deployment of P&T<br />

up to the level of industrial implementation. It should serve as a basis for decisions on advanced<br />

fuel cycles leading to a sustainable nuclear energy and thus is intended to provide input for the<br />

structuring of the corresponding part of the Sustainable Nuclear Energy Technology Platform<br />

(SNE-TP).<br />

Performance characteristics of various options for transmutation systems were evaluated e.g.<br />

Multi recycling in fast reactors (FR) of TRU unloaded from LWRs and, successively, from<br />

FRs.<br />

Reduction of TRU inventory in fuels unloaded from LWRs.<br />

Reduction of MA inventory.<br />

Use of different fuel types and coolants in critical systems as well as the impact of different recycling<br />

(e.g. homogeneous and heterogeneous MA recycling) has been studied [1]. Such strategies<br />

necessitate fuels with variable amounts of MA incorporated in conventional fuels. The results of the<br />

PATEROS programme have been complemented by those obtained in the EISOFAR project for sodium<br />

cooled systems and the ELSY project for lead cooled systems. Though dependent on design<br />

optimisation, the generic transmutation characteristics for different coolants and homogeneous re-<br />

114

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