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A Review of Criticality Accidents A Review of Criticality Accidents

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The accident investigation determined that the<br />

excursions had occurred in the vacuum pump oil<br />

reservoir (Figure 16). The gamma exposure rate on<br />

contact was measured daily at the midpoint <strong>of</strong> the oil<br />

reservoir for five days using a PMR-1 instrument.<br />

Results <strong>of</strong> these measurements are shown in Table 7. A<br />

total <strong>of</strong> 42.95 l <strong>of</strong> oil were drained into 5 l bottles on<br />

18 and 19 July. Analysis <strong>of</strong> the oil using the luminescent<br />

method indicated a uranium concentration <strong>of</strong><br />

173 g/ l with an uncertainty <strong>of</strong> ±30% to 40% (the<br />

luminescent method involved introducing a liquid<br />

luminescing agent into the solution and estimating the<br />

concentration from the intensity <strong>of</strong> the emitted light).<br />

The uranium enrichment was uniformly 22.6% by<br />

weight.<br />

The time evolution <strong>of</strong> the excursions had several<br />

unusual features. The UF 6 had been accumulating at a<br />

normal rate until four days before the accident when a<br />

large increase occurred. There was no delay in the<br />

initiation <strong>of</strong> the chain reaction due to the very slow<br />

Figure 16. Oil reservoir (Dimensions are in mm).<br />

reactivity insertion rate and the relatively large neutron<br />

source (~1.3 × 10 4 n/s from α,n reactions). Consequently,<br />

the first excursion on 14 July (04:45) was very<br />

small and probably did not exceed 2 × 10 14 fissions.<br />

After this excursion terminated, the oil in the reservoir<br />

probably remained only slightly subcritical. It should<br />

be emphasized that the concentration, solution volume,<br />

and material configuration at the time <strong>of</strong> this burst are<br />

not well known. Furthermore, it is not known if the<br />

vacuum pump was operating during this first excursion.<br />

When the pump was turned on at 07:30, the oil in<br />

the pump’s cavities was forced out into the central pipe<br />

<strong>of</strong> the oil reservoir. This sudden injection <strong>of</strong> oil<br />

containing uranium led to the second and much larger<br />

excursion. The shutdown <strong>of</strong> this excursion was due to a<br />

combination <strong>of</strong> temperature rise and radiolytic gas<br />

generation, which caused ejection <strong>of</strong> the oil from this<br />

central pipe back into the pump’s cavities and the gas<br />

purification equipment. As with the first excursion, the<br />

25

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