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Neutron Scattering

Neutron Scattering - JuSER - Forschungszentrum Jülich

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21<br />

[ooç 1 " -<br />

19<br />

18<br />

17<br />

16<br />

"" 298 K<br />

4<br />

3<br />

O<br />

0 0.2 0.4 0 .6 0.8 1.0 0.8 0.6 0.4 0.2 0 0.1 0.2 0.3 0.4 0.3<br />

Reduced wave vector coordinate (c)<br />

Figure 13 Phonon dispersion of TaC, the dips, for example at (0 0 0 .7) andd at (0 .6 0 .6 0), indicate<br />

modes renormalized throiigh the electron phonon coiipling, from reference [2] .<br />

coupled spins the energy of the magnetic interaction amounts to<br />

n,<br />

U = -2J ~7 Sp - Sp+1 (13 .20) .<br />

p=1<br />

In the ground state all spins are parallel and Uo = -2NJS 2 ,<br />

this corresponds to figure<br />

14a . A possible excitation might consist in the flip of just one spin, like it is shown in<br />

figure 14b . 'This perturbation yields a finite increase in energy of 8JS 2 . However, the temperature<br />

dependence of several macroscopic properties like specific heat or magnetization<br />

does not correspond to an exponential law, as it<br />

has to be expected for a finite excitation<br />

energy.<br />

Spin waves (magnons) must have a much smaller energy than the single spin flip,<br />

like phonons may have lower energy than an ionic vacancy for instance .<br />

The distortion of the magnetic order corresponds to<br />

a plane magnetic wave (with<br />

propagation vector q and frequency w) and is drawn in Figure 14c .<br />

Spins are precessing<br />

around the direction of magnetic order (here z) with components<br />

Sp - u - exp[i(p(ja - wt)] (13 .21),<br />

13-20

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