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Neutron Scattering

Neutron Scattering - JuSER - Forschungszentrum Jülich

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times is performed at the detector distance dcp + L .<br />

A possible resulting "spectrum" is<br />

indicated on top of the detector distance line.<br />

The extrapolation of the dashed line to the<br />

detector position indicates the location of the "elastic line", i.e .<br />

the time channel where<br />

neutrons without energy transfer arrive 4 .<br />

The left vertical edge of the triangle defines<br />

the "beginning" of the time-of-flight spectrum, i .e .<br />

the earliest possible time of arrival<br />

occurring only for nearly infinite energy gain of the neutron .<br />

In reality there are no infinite<br />

large energy gains and the proper spectrum Starts somewhat later .<br />

The right edge of the<br />

"velocity fan" symbolized by the triangle is less well defined, in principle the neutron may<br />

transfer only a part of its energy but also virtually all of its energy to the Sample, thus<br />

virtually hortizontal path-time curves may result . Le . strictly speaking the spectrum does<br />

not end at some maximum channel number . However it is immediately recognizable that<br />

fortunately this effect goes along with a corresponding "dilution"<br />

of the intensity which<br />

becomes virtually structureless on the scale of the histogram channel Windows ("frames")<br />

causing a constant background in all channels of a "frame" that may be subtracted during<br />

data treatment . Thereby it becomes possible to repeat the uptake of a "frame" with a<br />

frequency S2 and to accumulate the spectra into the histograms mentioned above . Each<br />

chopper pulse resets the clock to time zero and the channels of the histogram cover the<br />

time interval T in terms of bins of width O7K ~ TIN .<br />

If due to resolution requirements<br />

5 or due to other technical demands 9 lias to be chosen such that the above discussed<br />

"frame"-overlap effect still distorts the spectra, it is possible, as indicated in fig . 10 .4, to<br />

use an additional coarse chopper to transmit only every 2nd or n-th pulse .<br />

By doing this<br />

sufficient spacing between "frames" may be gained to collect<br />

an undistorted spectrum,<br />

however with an n-fold reduction of effective data collection rate .<br />

10 .2 .2 Time-of-flight spectra<br />

In fig. 10 .5 several spectra as they are accumulated in the histogrammic memory are<br />

displayed .<br />

The time-of-flight scale of the horizontal axis refers to the distance L between<br />

Sample and detectors . This time-of-flight is directly proportional to the wavelength A'<br />

of the scattered neutrons as is indicated by the diagonal representing this linear relation<br />

4 Generally the scattering without (sizeable) energy transfer is the most probable process .<br />

5The pulse width (opening time) of a chopper depends -for a given design- on its rotation frequency.<br />

10-6

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