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PHYSICAL REVIEW B 70, 144524 (2004)<strong>Hofstadter</strong> <strong>butterflies</strong> <strong>in</strong> a <strong>modulated</strong> <strong>magnetic</strong> <strong>field</strong>: Superconduct<strong>in</strong>g wire networkwith <strong>magnetic</strong> decorationYasuhiro Iye,* Eiichi Kuramochi, Masahiro Hara, Akira Endo, and Sh<strong>in</strong>go KatsumotoInstitute for Solid State Physics, University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba 227-8581, Japan(Received 1 April 2004; published 29 October 2004)<strong>Hofstadter</strong> butterfly spectra of tight-b<strong>in</strong>d<strong>in</strong>g electron systems under spacially <strong>modulated</strong> <strong>magnetic</strong> <strong>field</strong>s arecalculated. The dependence of the spectrum on the symmetry and strength of the spatially vary<strong>in</strong>g <strong>magnetic</strong><strong>field</strong> is elucidated. The Little-Parks oscillation of the superconduct<strong>in</strong>g network under a spatially <strong>modulated</strong><strong>magnetic</strong> <strong>field</strong> produced by decoration with mesoscopic <strong>magnetic</strong> structure exhibits behavior reproduc<strong>in</strong>g theedge of the correspond<strong>in</strong>g <strong>Hofstadter</strong> spectra.DOI: 10.1103/PhysRevB.70.144524PACS number(s): 74.78.w, 74.81.Fa, 75.75.a, 73.21.bI. INTRODUCTIONThe exquisite structure of the energy diagram of a tightb<strong>in</strong>d<strong>in</strong>gelectron system on a two-dimensional (2D) squarelattice subjected to a uniform perpendicular <strong>magnetic</strong> <strong>field</strong>was first elucidated by the work of <strong>Hofstadter</strong> 1 and Wannier. 2The spectrum consists of q subbands, when the flux (<strong>in</strong> theunits of the flux quantum 0 =h/e) thread<strong>in</strong>g through eachplaquette is a rational number p/q. The spectra of this type,known as the <strong>Hofstadter</strong> butterfly, have s<strong>in</strong>ce been calculatedfor a variety of lattices, 3–5 and they have been discussed<strong>in</strong> various contexts of condensed-matter physics <strong>in</strong>clud<strong>in</strong>gthe quantum Hall effect 6,7 and the so-called flux phase <strong>in</strong> thet-J model. 8,9Observation of the butterfly spectra <strong>in</strong> real systems is aformidable task. For the ord<strong>in</strong>ary crystall<strong>in</strong>e lattices, the required<strong>magnetic</strong> <strong>field</strong> exceeds 1000 T, which is beyond thereach of the present technology. It is therefore natural to turnto the artificial periodic structures, such as lateral superlatticesbased on semiconductor two-dimensional electron systems.Recent work by Albrecht et al. 10 on magnetotransport<strong>in</strong> an antidot lattice seems to capture a certa<strong>in</strong> characteristicof the <strong>Hofstadter</strong> spectrum.Superconduct<strong>in</strong>g networks comprise another category ofsystems <strong>in</strong>timately related to the <strong>Hofstadter</strong> spectrum. Asdemonstrated by Pannetier et al., 11 the change <strong>in</strong> the transitiontemperature of a superconduct<strong>in</strong>g wire network with thefrustration parameter reproduces the f<strong>in</strong>e structure of theupper edge of the <strong>Hofstadter</strong> butterfly spectrum. This correspondencearises from the fact that the l<strong>in</strong>earized G<strong>in</strong>zburg-Landau equation for a superconductor near its transition hasthe same form as the Schröd<strong>in</strong>ger equation for the electronsystem. 12,13 Thus, with the advantage of macroscopic coherence,superconduct<strong>in</strong>g networks provide a convenient experimentalmodel of the <strong>Hofstadter</strong> butterfly, although admittedlythey can only probe the edge of the spectrum. This l<strong>in</strong>e ofstudy was subsequently extended to networks of various latticesymmetries, <strong>in</strong>clud<strong>in</strong>g triangular, honeycomb,Kagomé, 14 T 3 , 15 disordered, 16 quasiperiodic, 17 and fractal 18lattices.To the best of our knowledge, all of these previous studiesbasically employed a uniform external <strong>magnetic</strong> <strong>field</strong>. Itwould be <strong>in</strong>terest<strong>in</strong>g to extend the study to more generalcases of spatially vary<strong>in</strong>g <strong>magnetic</strong> <strong>field</strong>. This is the subjectof the present study. More specifically, we have calculatedthe <strong>Hofstadter</strong> spectrum for a square lattice under spaciallyvary<strong>in</strong>g <strong>magnetic</strong> <strong>field</strong>s. We have also conducted experimentsus<strong>in</strong>g a superconductor/ferromagnet (S/F) hybrid systemconsist<strong>in</strong>g of a superconduct<strong>in</strong>g wire network and anarray of mesoscopic ferromagnets. An early version of ourstudy us<strong>in</strong>g an S/F hybrid system study has beenpublished. 19,20 An S/F hybrid system of a different type fromthe present one was studied by Nozaki et al. 21 The <strong>Hofstadter</strong>spectrum for a T 3 lattice under a <strong>modulated</strong> <strong>magnetic</strong> <strong>field</strong> istheoretically studied by Oh. 22The rema<strong>in</strong>der of this paper is organized as follows. Calculationsof the <strong>Hofstadter</strong> spectra for a square network undervarious patterns of a spatially vary<strong>in</strong>g <strong>magnetic</strong> <strong>field</strong> arepresented <strong>in</strong> the next section. Experiments us<strong>in</strong>g asuperconductor/ferromagnet hybrid system are described <strong>in</strong>Sec. III, and discussed <strong>in</strong> comparison with the calculatedspectra. F<strong>in</strong>ally, Sec. IV gives a summary of the presentwork and some remarks.II. CALCULATION OF THE HOFSTADTER SPECTRAA. The orig<strong>in</strong>al <strong>Hofstadter</strong> problemThe <strong>Hofstadter</strong> problem <strong>in</strong> its orig<strong>in</strong>al form, i.e., the tightb<strong>in</strong>d<strong>in</strong>gelectron spectrum on a 2D square lattice with latticeconstant a under a uniform <strong>magnetic</strong> <strong>field</strong> H, is obta<strong>in</strong>ed bysolv<strong>in</strong>g the follow<strong>in</strong>g Schröd<strong>in</strong>ger equation: n,m = t n−1,m + t n+1,m + te −2<strong>in</strong> n,m−1 + te 2<strong>in</strong> n,m+1 ,1where n,m represents the wave function at the latticesite n,m, t is the nearest-neighbor transfer-matrix element,and / 0 =eHa 2 /h is an avarage <strong>magnetic</strong> flux thread<strong>in</strong>ga unit square. The parameter is often called a frustrationparameter. The above equation can be reduced byputt<strong>in</strong>g n,m = e ik x na e ik y ma nto the follow<strong>in</strong>g one-dimensional Harper equation:21098-0121/2004/70(14)/144524(9)/$22.50 70 144524-1©2004 The American Physical Society


IYE et al. PHYSICAL REVIEW B 70, 144524 (2004) n = te −ik x a n−1 + te ik x a n+1 +2t cosk y a −2n n .3When is a rational number p/q, p and q be<strong>in</strong>gmutually prime, the size of the <strong>magnetic</strong> unit cell becomesqa,a, namely, x+qa,y=x,y and x,y+a=x,y.Figure 1 shows the tight-b<strong>in</strong>d<strong>in</strong>g square lattice withthe choice of gauge appropriate to = p/q. The energyeigenvalues are obta<strong>in</strong>ed by diagonaliz<strong>in</strong>g the follow<strong>in</strong>gmatrix:2t cosk y a −2 te ik x a 0 ¯ 0 e −ik x ate −ik x a 2t cosk y a −4 te ik x a 0 ¯ 00 4 0 00 ¯ 0 te −ik x a 2t cosk y a −2q −1 te ik x ate ik x a 0 ¯ 0 te −ik x a 2t cosk y a −2q.The result is the well-known butterfly spectrum, shown <strong>in</strong>the topmost panel of Fig. 3.B. Checkerboard <strong>magnetic</strong> <strong>field</strong>We consider a spatially vary<strong>in</strong>g <strong>magnetic</strong> <strong>field</strong> whichconsists of a uniform component and a component vary<strong>in</strong>g<strong>in</strong> a checkerboard pattern, as shown <strong>in</strong> Fig. 2. Here, denotes the flux per plaquette of the uniform componentof the <strong>magnetic</strong> <strong>field</strong>, and denotes the flux per plaquettewhich alternates <strong>in</strong> sign <strong>in</strong> the checkerboard pattern. Theassignment of the Peierls phase factor for this flux patternis shown <strong>in</strong> the figure. For = p/q, the system is <strong>in</strong>variantunder translation 2qa,0 or a,a. The relevant Schröd<strong>in</strong>gerequation reads n,m = t n−1,m + t n+1,m + te −2<strong>in</strong>−m+1 n,m−1+ te 2<strong>in</strong>−m e 2i n,m+1 n − m odd, 5 n,m = t n−1,m + t n+1,m + te −2<strong>in</strong>−m+1 e 2i n,m−1+ te 2<strong>in</strong>−m n,m+1 n − m even.Spectra obta<strong>in</strong>ed by diagonalization of the correspond<strong>in</strong>g2q2q matrix are shown <strong>in</strong> Fig. 3. The spectra are symmetricwith respect to transformations, →1±, so that calculationover the range =0– 1 2suffices. Five panels <strong>in</strong> Fig. 3correspond to =0, 1 8 , 1 4 , 3 8 , and 1 2, respectively. The topmostpanel =0 is the orig<strong>in</strong>al <strong>Hofstadter</strong> butterfly spectrum.Introduction of nonzero deforms the spectrum <strong>in</strong> such away that, for <strong>in</strong>stance, the spectral weight at the band center(van Hove s<strong>in</strong>gularity at =0) for =0 is smeared, and aquasigap develops there with <strong>in</strong>creas<strong>in</strong>g . The bottommostpanel = 1 2is identical to the topmost one except that thespectrum is shifted by 1 2along the horizontal axis. Thatthis should be so can be readily understood by recall<strong>in</strong>g thefollow<strong>in</strong>g: At = 1 2 , two adjacent cells enclose + 1 2 and − 1 2flux, respectively. Addition of a uniform flux = 1 2to thesystem changes them to 1 and 0, which is equivalent to the=0,=0 configuration. The same relation (shift by halfperiod)holds between the spectra for = 3 8[panel (d)] andfor = 1 8 [panel (b)].At= 1 4[panel (c)], the periodicity <strong>in</strong> becomes half the orig<strong>in</strong>al one. In other words, the states at=<strong>in</strong>teger and at =half-<strong>in</strong>teger become equivalent for= 1 4. Aga<strong>in</strong>, this can be easily understood by recall<strong>in</strong>g thatthe flux configuration of two adjacent cells is +34 ,+1 4at= 1 4 ,= 1 2, which is equivalent to −14 ,+1 4, and hence to +14 ,−1 4at = 1 4 ,=0 .FIG. 1. Tight-b<strong>in</strong>d<strong>in</strong>g square lattice with assignment of thePeierls phase factor to each bond, for a uniform external <strong>magnetic</strong>flux = p/q.FIG. 2. Square lattice subjected to a spatially vary<strong>in</strong>g <strong>magnetic</strong><strong>field</strong> <strong>in</strong> a checkerboard pattern and a uniform <strong>field</strong> .The assignment of the Peierls phase factor is <strong>in</strong>dicated bythe arrows.144524-2


HOFSTADTER BUTTERFLIES IN A MODULATED… PHYSICAL REVIEW B 70, 144524 (2004)FIG. 3. <strong>Hofstadter</strong> spectra for a square lattice subjected to a checkerboard <strong>field</strong> and a uniform <strong>field</strong> . Five panels shows spectrafor different amplitudes of the checkerboard <strong>field</strong>: (a) =0, (b) = 1 8 , (c) = 1 4 , (d) = 3 8 , and (e) = 1 2 , respectively.C. Stripe <strong>magnetic</strong> <strong>field</strong>We next consider the case of a stripe pattern of <strong>field</strong>modulation, as shown <strong>in</strong> Fig. 4. Here, denotes the flux perplaquette, which alternates <strong>in</strong> sign for every other column.The assignment of the Peierls phase factor for this fluxpattern is shown <strong>in</strong> the figure. The <strong>magnetic</strong> unit cell for= p/q is 2qa,a, i.e., the system is <strong>in</strong>variant under translationby 2qa,0 or 0,a. The relevant Schröd<strong>in</strong>ger equationreads n,m = t n−1,m + t n+1,m + te −2<strong>in</strong> e 2i n,m−1+ te 2<strong>in</strong> e 2i n,m+1 n odd, 6 n,m = t n−1,m + t n+1,m + te −2<strong>in</strong> n,m−1+ te 2<strong>in</strong> n,m+1 n even.The spectra obta<strong>in</strong>ed by diagonalization of the correspond<strong>in</strong>g2q2q matrix are shown <strong>in</strong> Fig. 5. Only the spectrafor = 1 8 and 1 4are shown, s<strong>in</strong>ce the spectra for =0and = 1 2 are identical to those for =0 and = 1 2<strong>in</strong> Fig. 3,and the spectrum for = 3 8is none other than thatfor = 1 8 shifted by 1 2along the horizontal axis. Wecan immediately note the differences between the spectrafor a stripe <strong>field</strong> and those for a checkerboard <strong>field</strong>. Introductionof nonzero (stripe <strong>field</strong>) causes lift<strong>in</strong>g of degeneracy144524-3


IYE et al. PHYSICAL REVIEW B 70, 144524 (2004)FIG. 4. Square lattice subjected to a spatially vary<strong>in</strong>g <strong>magnetic</strong><strong>field</strong> <strong>in</strong> a stripe pattern and a uniform <strong>field</strong> . The assignmentof the Peierls phase factor is <strong>in</strong>dicated by the arrows.at =0 for = 1 2, while the splitt<strong>in</strong>g occurs at <strong>in</strong>teger for the checkerboard <strong>field</strong>, as seen earlier. It is evidentthat the spectra for stripe <strong>field</strong>s are considerably “darker”(more bands and fewer gaps) as compared with thosefor checkerboard <strong>field</strong>s. This is <strong>in</strong> l<strong>in</strong>e with a generaltrend that the <strong>Hofstadter</strong> spectrum becomes “darker”as one <strong>in</strong>troduces rectangular anisotropy <strong>in</strong> the squarelattice. 9D. Comparison with a honeycomb latticeAlthough it is a k<strong>in</strong>d of excursion to a side road,it is <strong>in</strong>terest<strong>in</strong>g to compare the spectra for the checkerboardFIG.FIG. 5. <strong>Hofstadter</strong> spectra for different values of , the strengthof the stripe pattern <strong>field</strong>. (a) = 1 8 and (b) = 1 4. The spectra for=0 and = 1 2are identical with Figs. 3(a) and 3(e), respectively.The spectrum for = 3 8 is the same as the one for = 1 8except it isshifted by 1 2along the horizontal axis.6. (a) A square lattice with different transfer <strong>in</strong>tegralst and t. When t=0 [panel (b)], it is topologically equivalentto a honeycomb lattice [panel (c)]. Panel (d) shows unit “brick” ofthis lattice and the one for a square lattice under checkerboard <strong>field</strong>(Fig. 2).<strong>field</strong> shown <strong>in</strong> Fig. 3 with that for a honeycomb latticeunder a uniform <strong>magnetic</strong> <strong>field</strong>. Let us consider a squarelattice shown <strong>in</strong> Fig. 6(a), <strong>in</strong> which the transfer <strong>in</strong>tegralfor every other vertical bond t (dotted l<strong>in</strong>es) can take adifferent value from that for the rest of the bonds t (solidl<strong>in</strong>es).The relevant Schröd<strong>in</strong>ger equation reads n,m = t n−1,m + t n+1,m + te −2<strong>in</strong> n,m−1 + te 2<strong>in</strong> n,m+1 .7Sett<strong>in</strong>g t=t reduces the system to a simple square lattice.On the other hand, sett<strong>in</strong>g t=0 [Fig. 6(b)] makes it topologicallyequivalent to a honeycomb lattice [Fig. 6(c)].Therefore, by chang<strong>in</strong>g the parameter t from t to 0, thesystem evolves cont<strong>in</strong>uously from a square to a honeycomblattice.Figure 7 shows calculated spectra for (a) t=0.5t and (b)t=0 (honeycomb lattice). It is seen that they exhibit a resemblance<strong>in</strong> overall shape with the spectra for = 1 8 and 1 4for the checkerboard <strong>field</strong> [panels (b) and (c) of Fig. 3]. Theresemblance actually runs over the whole range of the twomodels, i.e., between the checkerboard <strong>field</strong> [Eq. (6)] with chang<strong>in</strong>g from 0 to 1 2and the square-to-honeycomb evolution[Eq. (7)] with t chang<strong>in</strong>g from t through 0 to −t. Thespectra at both ends are <strong>in</strong>deed identical: =0⇔t=t and=1/2⇔t=−t.In retrospect, this resemblance is someth<strong>in</strong>g one shouldhave anticipated, because <strong>in</strong> both cases the structural unitis a rectangle consist<strong>in</strong>g of two adjacent unit squares, asshown <strong>in</strong> Fig. 6(d). Both Fig. 2 and Fig. 6(a) are thenconstructed by bricklay<strong>in</strong>g these unit rectangles <strong>in</strong> the144524-4


HOFSTADTER BUTTERFLIES IN A MODULATED… PHYSICAL REVIEW B 70, 144524 (2004)FIG. 7. Spectra for the model def<strong>in</strong>ed <strong>in</strong> Fig. 6. The panels (a)and (b) are for t=0.5t and 0 (honeycomb lattice), respectively. Thespectra for t=t and t=−t are the same as the panels (a) and (e) ofFig. 3, respectively.pattern shown <strong>in</strong> Fig. 6(b). It is also <strong>in</strong>terest<strong>in</strong>g to notethat the spectra shown <strong>in</strong> Fig. 3 resemble those obta<strong>in</strong>ed fora lattice fermion model <strong>in</strong> the context of two-dimensionald-wave superconductivity. 23E. Relation to superconduct<strong>in</strong>g networksThe transition temperature of a superconduct<strong>in</strong>g wire networkunder a uniform <strong>magnetic</strong> <strong>field</strong> H is related with theeigenvalue max correspond<strong>in</strong>g to the upper edge of the energyspectrum for the tight-b<strong>in</strong>d<strong>in</strong>g model by the follow<strong>in</strong>grelation: 11–13T c HT c0= 2 0a 2arccos 2 maxz. 8Here, z is the number of nearest-neighbor nodes. Typically,the relative change <strong>in</strong> the transition temperature is smallT c T c0 , and T c is l<strong>in</strong>early related with max .Figure 8 shows the evolution of the lower edgeof the <strong>Hofstadter</strong> spectra as a function of the amplitude (a) of the checkerboard <strong>field</strong> and (b) of the stripe <strong>field</strong>.(S<strong>in</strong>ce the upper and the lower edge are identical, weshow the latter for the sake of ease of visual comparisonwith the experimental data to be shown later.) The curveon the front-left face ( or =0) represents the loweredge of the orig<strong>in</strong>al <strong>Hofstadter</strong> butterfly spectrum. In Fig. 9,the same set of data are presented as a gray-scale plot.A notable difference between the checkerboard and stripeFIG. 8. Stereo plot of the m<strong>in</strong>imum energy as a function of and (or ). Namely, these figures show evolution of the bottomedge of the <strong>Hofstadter</strong> spectrum with the amplitude of the spatiallyvary<strong>in</strong>g <strong>magnetic</strong> <strong>field</strong> of (a) the checkerboard pattern and (b) thestripe pattern.<strong>field</strong> case is manifest upon comparison of the curves on thefront-right face =<strong>in</strong>teger. The curve <strong>in</strong> Fig. 8(a) has acusp at = 1 2 , while that <strong>in</strong> Fig. 8(b) is rounded at = 1 2 .Correspond<strong>in</strong>gly, the latter rises more steeply near the orig<strong>in</strong>than the former. These features are to be compared with theexperimental results <strong>in</strong> the next section. An <strong>in</strong>terest<strong>in</strong>g featureof the energy landscape shown <strong>in</strong> Fig. 8(a) is that theenergy at = 1 4 and 3 4 is constant =−2 2 irrespective of thevalue of , which can be seen more clearly <strong>in</strong> the contourplot of Fig. 9(a).FIG. 9. Contour plot of the same set of data as Fig. 8.144524-5


IYE et al. PHYSICAL REVIEW B 70, 144524 (2004)FIG. 10. Structure of the samples. (a) Sample A for the checkerboard<strong>field</strong>. (b) Sample B for the stripe <strong>field</strong>. The external <strong>field</strong>parallel to the network plane controls the magnetization of the ferro<strong>magnetic</strong>array. The amplitude of the spatially <strong>modulated</strong> <strong>magnetic</strong><strong>field</strong> can be changed by the azimuthal angle of the parallel<strong>field</strong>.III. EXPERIMENT WITH SUPERCONDUCTINGWIRE NETWORKSA. Experimental methodThe samples used <strong>in</strong> the present study were fabricated onsilicon substrates by the follow<strong>in</strong>g steps.(i) Electrode pads were first formed by electron beam lithographyand gold evaporation.(ii) The network pattern (square lattice) was def<strong>in</strong>ed byelectron beam lithography and the niobium wire networkwas formed by ion-beam sputter<strong>in</strong>g deposition and the liftoffprocess.(iii) A protect<strong>in</strong>g layer of germanium was deposited ontop of the wire network, so as to prevent oxidation of niobiumand to keep it from direct contact with the ferro<strong>magnetic</strong>material to be deposited next.FIG. 11. Magnetoresistance traces at different temperatures forsample A. These data were taken at =0, i.e., =0.FIG. 12. Evolution of the Little-Parks oscillation for sample Awith the value of (checkerboard <strong>field</strong>). The traces are verticallyoffset for clarity.(iv) An array of mesoscopic ferromagnets (cobalt ornickel) was placed on top by electron beam lithography, ionbeamsputter deposition, and liftoff.The crucial po<strong>in</strong>t <strong>in</strong> the fabrication was to achievegood positional and angular registration between thesuperconduct<strong>in</strong>g network and the overlaid ferromagnetarray.Two samples (A and B) were <strong>in</strong>tensively studied. Thesesamples represent the checkerboard <strong>field</strong> case (sample A)and the stripe <strong>field</strong> case (sample B), respectively. Thesuperconductor part of the sample consisted of a squarenetwork of 100100 unit cells, made of niobium wire150 nm wide and 40 nm thick. The lattice period was500 nm for sample A and 750 nm for sample B. For sampleA, 150200 nm 2 rectangular dots of 80-nm-thick cobaltwere placed on top of the center of every other bond wires<strong>in</strong> the y direction, as shown <strong>in</strong> Fig. 10(a). For sample B,250-nm-wide strips of 60-nm-thick nickel were placedon top of every other l<strong>in</strong>es <strong>in</strong> the y direction as shown <strong>in</strong>Fig. 10(b).Measurements of the superconduct<strong>in</strong>g properties wereconducted by use of a cross-coil superconduct<strong>in</strong>g magnetsystem, consist<strong>in</strong>g of a 6 T Helmholtz coil and a 1 Tsolenoid. The horizontal <strong>field</strong> was used to fix the magnetizationof the ferro<strong>magnetic</strong> array and thereby controlthe strength of the spatially vary<strong>in</strong>g <strong>field</strong> (parameter or ).The vertical <strong>field</strong> supplied the uniform <strong>field</strong> (parameter )for the network. The four-term<strong>in</strong>al resistance of the networkwas measured by a standard ac lock-<strong>in</strong> technique. Cryogeniccontrol was achieved by a variable temperature <strong>in</strong>sert Dewar144524-6


HOFSTADTER BUTTERFLIES IN A MODULATED… PHYSICAL REVIEW B 70, 144524 (2004)FIG. 13. Evolution of the Little-Parks oscillation for sample Bwith the value of (stripe <strong>field</strong>). The traces are vertically offset forclarity.and a feedback circuit for heater power. Use of a sampleholder with rotat<strong>in</strong>g stage enabled us to precisely align theorientation of the network sample with respect to the <strong>magnetic</strong><strong>field</strong>.The plane of the wire network was adjusted so as to makeit parallel to the horizontal <strong>magnetic</strong> <strong>field</strong>. The horizontal<strong>magnetic</strong> <strong>field</strong> was typically set at 1 T, which was strongenough to fully saturate the magnetization of the ferromagnet.The value of for the checkerboard <strong>field</strong> (or for stripe <strong>field</strong>) was varied by chang<strong>in</strong>g the azimuthalangle of the horizontal <strong>field</strong>. As is clear from the configurationshown <strong>in</strong> Fig. 10, when =0 the total flux dueto the stray <strong>field</strong> from the mesoscopic magnets adds upto zero for each plaquette (provided that the lithographicalsymmetry is perfect), so this corresponds to =0. Asthe horizontal <strong>field</strong> is rotated from =0, the flux pierc<strong>in</strong>geach plaquette grows <strong>in</strong> magnitude, and the sign alternatesbetween adjacent cells. The value of could thus becontrolled <strong>in</strong> a contiunuous manner (roughly proportionalto for small ). A typical set of measurements consistedof sweep<strong>in</strong>g the vertical <strong>magnetic</strong> <strong>field</strong> for different sett<strong>in</strong>gsof .B. Results and discussionFigure 11 shows a series of magnetoresistance tracesfor sample A under =0 at different temperatures belowT c . Little-Parks oscillations with period 7.7 mT, whichagrees well with the unit-cell area 0.25 m 2 , are clearlyseen with additional dips at half-<strong>in</strong>tegers. The small shiftFIG. 14. Comparison of T c with the edge of the <strong>Hofstadter</strong>spectra for (a) checkerboard and (b) stripe <strong>field</strong>. The symbols represent−T c obta<strong>in</strong>ed from the resistance change as a function of or . The curves represent the bottom edge of the correspond<strong>in</strong>g<strong>Hofstadter</strong> spectra scaled to fit with the experimental data. The solidsymbols and the solid curve correspond to =0. The open symbolsand the dashed curve correspond to = 1 2 .of zero <strong>magnetic</strong> <strong>field</strong> is due to residual misalignmentbetween the horizontal <strong>magnetic</strong> <strong>field</strong> and the film plane.The f<strong>in</strong>e structures at rational values of other than12 (and weaker features at 1 3 and 2 3) were not clearly observed<strong>in</strong> this sample. This is probably attributable to lithographicalimperfection, especially nonperfect registry betweenthe superconduct<strong>in</strong>g wire network and the mesoscopicmagnet array, which tends to smear the higher-orderstructures.Then the temperature was fixed at a po<strong>in</strong>t where thesample resistance was about 0.01R n , and a series of magnetoresistancetraces were taken by sweep<strong>in</strong>g the vertical <strong>field</strong>for different sett<strong>in</strong>gs of . Figure 12 shows the traces thusobta<strong>in</strong>ed. Here, successive traces correspond to <strong>in</strong>crementsof by 1 degree, and they are vertically offset for clarity.The horizontal axis is converted to , with a proper correctionfor the above-mentioned zero-<strong>field</strong> shift.The trace marked A corresponds to =0. With <strong>in</strong>crementsof , the dips at half-<strong>in</strong>tegers deepen and those at <strong>in</strong>tegersbecome shallow, until they become equal for the traceB. Here, the period of oscillation becomes half the orig<strong>in</strong>alone. This corresponds to = 1 4. With a further <strong>in</strong>crease144524-7


IYE et al. PHYSICAL REVIEW B 70, 144524 (2004)of , the dips at half-<strong>in</strong>teger and <strong>in</strong>teger ’s change over<strong>in</strong> depth. The trace C, which corresponds to = 1 2, is shiftedby a half-period from the orig<strong>in</strong>al one (trace A). Theevolution with thus goes on and completes one cycle atthe trace E.Figure 13 shows a similar set of traces for sample B,represent<strong>in</strong>g the stripe <strong>field</strong> case. 24 Although the overall evolutionof the trace with is similar to Fig. 12, there are twodist<strong>in</strong>ct features to be noted. First, compar<strong>in</strong>g the traces B <strong>in</strong>the two figures, the relative amplitude of oscillation at thepo<strong>in</strong>t of half-periodicity for sample B = 1 4is muchsmaller than the correspond<strong>in</strong>g one for sample A = 1 4. Secondly,although difficult to see directly from Figs. 12 and 13,there is a substantial difference <strong>in</strong> the way the depth of <strong>in</strong>tegerdips (and that of the half-<strong>in</strong>teger dips) evolves with or, between the two cases. This is more clearly seen <strong>in</strong> Fig.14, which shows the shift <strong>in</strong> the transition temperature with (or ) for the two cases. The values of T c were obta<strong>in</strong>edfrom the experimentally measured changes <strong>in</strong> resistance byconvert<strong>in</strong>g them with use of the resistive transition curveRT. The amplitude T c is consistent with Eq. (8) with030 nm. The difference <strong>in</strong> T c by a factor of 2 betweensamples A (checkerboard) and B (stripe) is chiefly due to thedifference <strong>in</strong> the unit-cell area a 2 . The curves <strong>in</strong> the figurerepresent the shape of the bottom edge of the correspond<strong>in</strong>g<strong>Hofstadter</strong> spectra, seen on the front-right facet of the stereoplot <strong>in</strong> Fig. 8. The solid symbols and the solid curve correspondto =0. The open symbols and the dashed curve correspondto = 1 2. The agreement between the experimentaldata and the calculated curves <strong>in</strong>dicates that the present systemof a superconduct<strong>in</strong>g network with <strong>magnetic</strong> decorationcaptures some of the characteristic features of the <strong>Hofstadter</strong>spectra under the spatially <strong>modulated</strong> <strong>magnetic</strong> <strong>field</strong> discussed<strong>in</strong> this paper.IV. CONCLUSIONWe have calculated the <strong>Hofstadter</strong> butterfly spectra for a2D tight-b<strong>in</strong>d<strong>in</strong>g square lattice subjected to a spatially <strong>modulated</strong><strong>magnetic</strong> <strong>field</strong>. The correspond<strong>in</strong>g experimental situationsare realized by fabricat<strong>in</strong>g a superconduct<strong>in</strong>g wire networkdecorated with a mesoscopic ferromagnet array. Theevolution of Little-Parks oscillation with the amplitude of the<strong>modulated</strong> <strong>magnetic</strong> <strong>field</strong> <strong>in</strong> these samples exhibits characteristicfeatures of the two different types of modulation, thatis, checkerboard and stripe pattern. These results establishthe consistency of the calculated <strong>Hofstadter</strong> spectra with thechange <strong>in</strong> T c , although there is a fundamental limitation thatonly the edge of the spectrum can be probed by the superconduct<strong>in</strong>gsystem.Control of flux distribution <strong>in</strong> the superconduct<strong>in</strong>g networkby mesoscopic <strong>magnetic</strong> decoration may prove to be auseful technique <strong>in</strong> the development of devices us<strong>in</strong>g superconduct<strong>in</strong>gflux quanta. It should be of much <strong>in</strong>terest to explorethe vortex dynamics <strong>in</strong> these artificial potential landscapes.More generally, the mesoscopic ferromagnet/superconductor hybrid system may provide a wider arena forthe exploration of vortex physics and possible device applications.ACKNOWLEDGMENTSWe thank Professor D. Yoshioka, Professor H. Aoki, ProfessorH. Fukuyama, Professor S. Maekawa, Professor F.Nori, and Dr. M. Kosh<strong>in</strong>o for helpful conversations. Thiswork has been supported by a Grant-<strong>in</strong>-Aid for COE Research“Quantum Dot and Its Application” (No. 12CE2004),and by a Grant-<strong>in</strong>-Aid for Scientific Research (No.13304025), from the M<strong>in</strong>istry of Education, Culture, Sports,Science and Technology (MEXT), Japan.*Electronic address: iye@issp.u-tokyo.ac.jp1 D.R. <strong>Hofstadter</strong>, Phys. Rev. B 14, 2239 (1976).2 G.H. Wannier, Phys. Status Solidi B 88, 757 (1978).3 F.H. Claro and G.H. Wannier, Phys. Rev. B 19, 6068 (1979).4 Y. Hatsugai and M. Kohmoto, Phys. Rev. B 42, 8282 (1990).5 Ch. Kreft and R. Seiler, J. Math. Phys. 37, 5207 (1996).6 D.J. Thouless, M. Kohmoto, M.P. Night<strong>in</strong>gale, and M. den Nijs,Phys. Rev. Lett. 49, 405 (1982).7 A.H. MacDonald, Phys. Rev. B 28, 6713 (1983).8 P. Lederer, D. Poilblanc, and T.M. Rice, Phys. Rev. Lett. 63,1519 (1989).9 Y. Hasegawa, Y. Hatsugai, M. Kohmoto, and G. Montambaux,Phys. Rev. B 41, 9174 (1990).10 C. Albrecht, J.H. Smet, K. von Klitz<strong>in</strong>g, D. Weiss, V. Umansky,and H. Schweizer, Phys. Rev. Lett. 86, 147 (2001).11 B. Pannetier, J. Chaussy, R. Rammal, and J.C. Villegier, Phys.Rev. Lett. 53, 1845 (1985); see also B. Pennetier, <strong>in</strong> QuantumCoherence <strong>in</strong> Mesoscopic Systems, edited by B. Kramer, NATOAdvanced Study Institute Series Vol. 254 (Plenum Press, NewYork, 1991), p. 457.12 S. Alexander, Phys. Rev. B 27, 1541 (1983).13 R. Rammal, T.C. Lubensky, and G. Toulouse, Phys. Rev. B 27,2820 (1983).14 M.J. Higg<strong>in</strong>s, Y. Xiao, S. Bhattacharya, P.M. Chaik<strong>in</strong>, S. Sethuraman,R. Bojko, and D. Spencer, Phys. Rev. B 61, R894 (2000).15 C.C. Abilio, P. Butaud, Th. Fournier, B. Pannetier, J. Vidal, S.Tedesco, and B. Dalzotto, Phys. Rev. Lett. 83, 5102 (1999).16 M.A. Itzler, A.M. Behrooz, C.W. Wilks, R. Bojko, and P.M.Chaik<strong>in</strong>, Phys. Rev. B 42, 8319 (1990).17 M.A. Itzler, R. Bojko, and P.M. Chaik<strong>in</strong>, Phys. Rev. B 47, 14 165(1993).18 B. Doucot, W. Wang, J. Chaussy, B. Pannetier, R. Rammal, A.Vareille, and D. Henry, Phys. Rev. Lett. 57, 1235 (1986).19 S. Ito, M. Ando, S. Katsumoto, and Y. Iye, J. Phys. Soc. Jpn. 68,3158 (1999).20 M. Ando, S. Ito, S. Katsumoto, and Y. Iye, J. Phys. Soc. Jpn. 68,3462 (1999).21 Y. Nozaki, Y. Otani, K. Runge, H. Miyajima, B. Pannetier, J.P.Nozieres, and G. Fillion, J. Appl. Phys. 79, 8571 (1996).22 G.-Y. Oh, Phys. Rev. B 62, 4567 (2000).144524-8


HOFSTADTER BUTTERFLIES IN A MODULATED… PHYSICAL REVIEW B 70, 144524 (2004)23 Y. Morita and Y. Hatsugai, Phys. Rev. Lett. 86, 151 (2001).24 The reason why the range of for Fig. 13 is wider than for Fig.12 is simply due to the difference <strong>in</strong> the <strong>magnetic</strong> decoration.First, the ferro<strong>magnetic</strong> material for sample B was nickel <strong>in</strong>contrast to cobalt for sample A. Secondly, the distance betweenthe ferromagnet array and the superconduct<strong>in</strong>g network wasabout five times larger for sample B than sample A. These twofactors made the value of required for the same amplitude of<strong>magnetic</strong> <strong>field</strong> modulation much larger for sample B than forsample A.144524-9

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