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Scientific Report 2007-2009<br />

Laboratories and Facilities of the Department of Physics<br />

L14. Laboratory for Ultrafast Spectroscopy<br />

The laboratory for Ultrafast Spectroscopy, inaugurated in March 2009, is a newcomer among the experimental facilities<br />

of the Physics Department. Built up from scratch thanks to an ERC-IDEAS Starting Grant project, the lab is powered by<br />

an ultrafast 80 Mhz Ti:Sa oscillator (Coherent MICRA) and a regenerative amplifier able to deliver 800nm, 1Khz pulses<br />

with dual option for 35 fs and 120 fs duration (Coherent LEGEND). The lab is currently involved in two main experimental<br />

activities based on Pump&Probe protocol applied in different time domains:<br />

Femtosecond Stimulated Raman Scattering We study photoinduced<br />

effects in molecular and supra molecular structures such as<br />

isomerization reactions, ligand dynamics in proteins, vibrational<br />

energy redistribution. The system is pumped in an out of equilibrium<br />

state by an ultrashort tunable laser pulse produced with an<br />

Optical Parametric Amplifier (pump), and the wavepacket evolution<br />

is probed at variable time delays tracking ultrafast dynamics<br />

by means of Stimulated Raman Scattering. A combination of a<br />

narrowband, highly tunable (330 ÷ 520 nm and 790÷810 nm)<br />

pulse and a ultrashort white light continuum allows broadband<br />

stimulated Raman scattering resulting in a probe with sub ps<br />

time resolution and few wavenumbers frequency resolution.<br />

Picosecond acoustics We study acoustic properties (sound<br />

propagation) in disordered materials in the 10 ÷ 100 picosecond<br />

time domain (corresponding to 50-500 Ghz range), which is unaccessible<br />

ordinary frequency domain techniques such as light and<br />

neutrons/xrays scattering. The sample needs to be prepared as<br />

a film ( 100 ÷ 1000 nm thickness) with a 10nm metallic coating<br />

on a surface. An ultrashort 800nm pulse impinges in the metallic<br />

Figure 1: Ultrafast Spectroscopy Laboratory<br />

surface producing an impulsive thermal expansion launching a strain wave. A second broadband pulse (white light continuum)<br />

is reflected by the metallic surface and by the moving acoustic wave, resulting into a time dependent modulated signal<br />

with periodicity and damping related to sound velocity and attenuation.<br />

http://femtoscopy.phys.uniroma1.it/<br />

Related research activities: C28.<br />

L15. Macroscopic Quantum Coherence Lab<br />

The The Macroscopic Quantum Coherence (MQC) group aims to study the behaviour<br />

of macroscopic systems at very low temperatures, where the thermal effects<br />

are negligible, being dominated by quantum effects. In particular we study superconducting<br />

non linear systems realized with Jopsephson junctions in various configurations<br />

and topology. These systems are studied also in view of the realization of a Quantum<br />

Computer made of superconducting qubits. The laboratory is equipped with a Leiden<br />

Cryogenics He3-He4 dilution refrigerator, having a base temperature of 10mK and<br />

200microW of power dissipation capability at 120 mK. The system is equipped with<br />

36 low frequency filtered lines (dc-1 MHz) and very high frequency rigid coaxial lines<br />

(30 GHz).<br />

For the high frequency signals we use two CW signal generators Anritsu Mg3694A<br />

10 MHz-40 GHz and HP 8673G 2-26GHZ. For low frequency signal generators<br />

and the detection system we use low noise commercial equipments driven by lab<br />

View custom designed virtual instruments. Devices pre-test are performed using<br />

standard liquid helium immersion dewars and a Heliox He3 system with operating<br />

temperature of 0,3K (at IFN- CNR lab in Rome). The devices are designed by the<br />

low temperature group collaborating with the experiment (IFN-CNR) and realized in<br />

the CNR nano-micro fabrication facility, or by external factories.<br />

Figure 2: Picture of the lower part<br />

of the dilution refrigerator.<br />

http://www.roma1.infn.it/exp/webmqc/home.htm/<br />

Related research activities: P33.<br />

<strong>Sapienza</strong> Università di Roma 187 Dipartimento di Fisica

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