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Three - University of Arkansas Physics Department

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VOLUME 78, NUMBER 5 PHYSICAL REVIEW LETTERS 3 FEBRUARY 1997<br />

Experimental Observation <strong>of</strong> the Continuous Pulse-Train Soliton Solution<br />

to the Maxwell-Bloch Equations<br />

John L. Shultz and Gregory J. Salamo<br />

<strong>University</strong> <strong>of</strong> <strong>Arkansas</strong>, <strong>Physics</strong> <strong>Department</strong>, Fayetteville, <strong>Arkansas</strong> 72701<br />

(Received 23 February 1996; revised manuscript received 2 July 1996)<br />

We report the first experimental observation <strong>of</strong> the evolution <strong>of</strong> an arbitrarily shaped input optical<br />

pulse train to the analytic, shape-preserving, Jacobi elliptic pulse-train solutions to the Maxwell-Bloch<br />

equations including relaxation. [SO03 1-9007(96)02261-21<br />

PACS numbers: 42.65.Tg<br />

Coherent propagation <strong>of</strong> trains <strong>of</strong> optical pulses through<br />

a two-level absorber has been investigated, from a theoretical<br />

viewpoint, by many researchers. These investigations<br />

have been based on the self-induced transparency<br />

(SIT) equations [I], both with [2-51 and without [6] the<br />

assumption <strong>of</strong> zero relaxation. Without relaxation, analytic<br />

shape-preserving pulse-train solutions to the SIT<br />

equations were found although they did require a rather<br />

complicated initial atomic state which appeared difficult<br />

to produce experimentally. Specifically, the necessary initial<br />

state for each atom in a Doppler-broadened pr<strong>of</strong>ile is<br />

composed <strong>of</strong> a different superposition <strong>of</strong> ground and excited<br />

states depending on the resonant frequency <strong>of</strong> the<br />

atom. With relaxation, however, it was shown that the<br />

atomic variables relax to the correct values needed to allow<br />

shape-preserving propagation <strong>of</strong> the analytic pulsetrain<br />

envelopes found as solutions to the zero-relaxation<br />

problem. In this sense, the presence <strong>of</strong> relaxation effects<br />

makes possible the experimental observation <strong>of</strong> the analytic<br />

shape-preserving optical pulse-train solutions predicted<br />

by the SIT equations with zero relaxation.<br />

While these theoretical studies have been very thorough,<br />

and experimental studies have demonstrated the features<br />

<strong>of</strong> breakup and delay [7-91, the predicted Jacobi elliptic<br />

soliton pulse-train solution has never been observed. In<br />

this Letter we report the first experimental observation<br />

<strong>of</strong> the Jacobi elliptic soliton shape-preserving solution to<br />

the SIT equations including relaxation. In particular, it is<br />

shown via experiment that an input train <strong>of</strong> optical pulses,<br />

with rather arbitrary input envelope shape and input area<br />

between rr and 37r, evolves through the interaction with<br />

a two-level absorber to the analytical, shape-preserving,<br />

Jacobi elliptic soliton-train solution to the SIT equations.<br />

This is true, as predicted, even though the optical train<br />

has been allowed to come to equilibrium for a time much<br />

longer than the two-level atomic absorber relaxation time.<br />

The basic apparatus consisted <strong>of</strong> a homemade modelocked<br />

dye laser and sodium absorption cell. The number<br />

<strong>of</strong> oscillating longitudinal modes in the cavity was controlled<br />

using several intracavity etalons. For the experiment<br />

these were limited to three longitudinal modes whose<br />

separation was 167 MHz as determined by the cavity configuration<br />

and monitored using a Fabry-Perot scan. The<br />

phase locking <strong>of</strong> these three modes resulted in an optical<br />

pulse train consisting <strong>of</strong> 2.9 ns (FWHM) pulses separated<br />

by 5.8 ns, peak to peak. This approach to producing an optical<br />

pulse train was chosen over using a cw laser coupled<br />

with a nonlinear optical modulator to ensure the production<br />

<strong>of</strong> an optical pulse train with both strong modulation and a<br />

high repetition rate. An example <strong>of</strong> the three laser modes,<br />

used to produce the input pulse train, as seen on an oscilloscope<br />

display <strong>of</strong> a Fabry-Perot scan is shown in Fig. l (a)<br />

along with a corresponding input optical pulse train in<br />

Fig. l(b). A computer simulation <strong>of</strong> the pulse train using<br />

the three mode-locked modes <strong>of</strong> relative amplitude shown<br />

in Fig. l(a), and fixed relative phase, is shown in Fig. I (c).<br />

The good agreement between Figs. l(b) and l(c) supports<br />

the assumption that the train <strong>of</strong> optical pulses is produced<br />

by mode locking three modes with fixed relative phase.<br />

The output optical pulse train was then gated through a<br />

Glan prism by a Pockels cell. This resulted in a train <strong>of</strong><br />

optical pulses that was about 1 ps long and was repeated<br />

every millisecond. The long time between successive<br />

pulse trains ensured that the experiment could be considered<br />

as starting over every millisecond. Meanwhile,<br />

the long length <strong>of</strong> the optical train, when compared to<br />

the atomic relaxation times <strong>of</strong> TI and Ti, guaranteed that<br />

equilibrium would be reached. The optical pulse train<br />

was then focused by an f = 41 cm lens into a 5 mm<br />

sodium cell. The sodium cell was housed in an oven and<br />

placed in a magnetic field which could be varied from 0 to<br />

10 kG. With a large magnetic field the sodium transitions<br />

<strong>of</strong> different Mj are well resolved, but several MI transitions<br />

are excited as a result <strong>of</strong> the large Doppler width.<br />

However, since the dipole moments are independent <strong>of</strong><br />

MI, simultaneous excitation <strong>of</strong> several MI levels with the<br />

same Mj quantum number can be treated as the excitation<br />

<strong>of</strong> a single state. For our experiment we excited the<br />

2~1/2 -+ 2~3/2 transition in sodium. In particular, using<br />

circularly polarized light we selectively excited only the<br />

3<br />

+<br />

2S~/2(~~ = 2 ~312(~J = Z) transition which could<br />

I<br />

then only decay back to the 2S1/2(~J = Z) ground state.<br />

In this way we avoid optical pumping complications. For<br />

this transition the energy decay time TI is equal to 16 ns<br />

while the dipole dephasing time T; is equal to 32 ns. This<br />

means that for our experiment the relaxation time is much<br />

003 1 -9007/97/ 78(5)/855(4)$10.00 0 1997 The American Physical Society 855

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