Three - University of Arkansas Physics Department
Three - University of Arkansas Physics Department
Three - University of Arkansas Physics Department
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Journal <strong>of</strong> Electronic Materials, Vol. 27, No. 7, 1998<br />
Regular Issue Paper<br />
Evaluation <strong>of</strong> 1nP:Fe Parameters by Measurement <strong>of</strong> Two<br />
Wave Mixing Photorefractive and Absorptive Gain<br />
M. CHAUVET,' G.J. SALAMO,' D.F. BLISS,^ and G. BRYANT~<br />
1.-<strong>University</strong> <strong>of</strong> <strong>Arkansas</strong>, <strong>Physics</strong> <strong>Department</strong>, Fayetteville, AK 72701, 2.-Rome Laboratory,<br />
U.S.A.F., Hanscom AFB, MA 01731<br />
In this paper, we present two-wave mixing absorption gain measurements in<br />
1nP:Fe in the 960-1035 nm wavelength range. The measured absorption gain is<br />
shown to be positive for long wavelength but changes sign for shorter wavelength.<br />
By simultaneously measuring the photorefractive gain and the absorption<br />
gain, we deduce the values <strong>of</strong> the photo-ionization cross sections related to<br />
the iron deep level trap. Finally, the study <strong>of</strong> the temperature dependence <strong>of</strong> the<br />
absorption gain allows us to evaluate a temperature shift <strong>of</strong> the iron level with<br />
respect to the conduction band <strong>of</strong> -4 x lo4 eV/K.<br />
Key words: Absorptive gain, InP:Fe, photorefractivity, two wave mixing<br />
INTRODUCTION<br />
Semi-insulating iron doped indium phosphide<br />
(1nP:Fe) is <strong>of</strong> interest for the development <strong>of</strong> optoelectronic<br />
components. For this reason, it is important<br />
to understand the role <strong>of</strong> iron on the electronic<br />
and optical performance <strong>of</strong> 1nP:Fe devices. This role is<br />
strongly related to the position and behavior <strong>of</strong> the<br />
iron level, as well as to the iron optical cross sections.<br />
In this paper, we exploit photorefractive two wave<br />
mixing (TWM) experiments to determine the optical<br />
cross sections as well as the temperature dependence<br />
<strong>of</strong> the iron energy level. These TWM experiments are<br />
based on observing the mutual influence <strong>of</strong> two coherent<br />
beams <strong>of</strong> unequal intensity crossing in a 1nP:Fe<br />
crystal. We measure the change <strong>of</strong> intensity level <strong>of</strong><br />
the weaker beam (signal beam) after propagation in<br />
the crystal under the presence <strong>of</strong> the strong beam<br />
(pump beam). A TWM gain r can then be calculated<br />
assuming that the intensity <strong>of</strong> the weak beam follows<br />
the solution:<br />
Where Iso and I,, are the intensity <strong>of</strong> the signal in the<br />
(Received August 25, 1997; accepted January 26, 1998)<br />
absence and in the presence <strong>of</strong> the strong beam,<br />
respectively. The TWM gain is composed <strong>of</strong> rEO, the<br />
electro-optic gain, Ta, the absorption gain and T, the<br />
absorption-induced index gain. These gains all come<br />
initially from a redistribution <strong>of</strong> the charges on the<br />
iron deep level under the influence <strong>of</strong> the interference<br />
grating formed by the two beams. Specifically, rEO is<br />
the electro-optic gain that is measured when the<br />
energy coupling is created by the space charge field<br />
associated with the linear electro-optic effect. This<br />
electro-o tic gain has been extensively studied in<br />
1nP:Fe<br />
1s<br />
as well as in numerous photorefractive<br />
and is commonly named the photorefractive<br />
gain. The absorptive gain5 ra takes place<br />
because <strong>of</strong> the absorption grating formed by the ~ e"<br />
and ~ e sinusoidal ~ ' redistribution resulting in a spatial<br />
modulation <strong>of</strong> the absorption. The absorption<br />
gain is usually neglected but it has been reported for<br />
photorefractive crystal such as6 BaTi03 and G~As.~"<br />
This absorption grating is accompanied by an index<br />
grating giving energy coupling or a gain T,. The total<br />
gain is simply the sum <strong>of</strong> the contribution <strong>of</strong> each<br />
individual gain: r = rEO + ra + ran<br />
THEORY<br />
The photorefractive effect is present in 1nP:Fe<br />
because <strong>of</strong> a spatial redistribution <strong>of</strong> the free carriers