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2.1 Ultrafast solid-state lasers - ETH - the Keller Group

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Ref. p. 134] <strong>2.1</strong> <strong>Ultrafast</strong> <strong>solid</strong>-<strong>state</strong> <strong>lasers</strong> 93<br />

Table <strong>2.1</strong>.6. Sellmeier equations for different materials. The wavelength λ is given in units of μm.<br />

Material Defining Sellmeier equation Constants<br />

Fused quartz n 2 =1+ Aλ2 + Bλ2 + Cλ2<br />

λ 2 − λ 2 1 λ 2 − λ 2 2 λ 2 − λ 2 3<br />

A =0.6961663<br />

λ 1 =0.0684043<br />

B =0.4079426<br />

λ 2 =0.1162414<br />

C =0.8974794<br />

λ 3 =9.896161<br />

SF10 glass<br />

a 0 =2.8784725<br />

n 2 = a 0 + a 1λ 2 + a2<br />

λ + a3<br />

2 λ + a4<br />

4 λ + a5<br />

a 1 = −0.010565453<br />

6 λ 8 a 2 =3.327942 × 10 −2<br />

a 3 =2.0551378 × 10 −3<br />

a 4 = −1.1396226 × 10 −4<br />

a 5 =1.6340021 × 10 −5<br />

Sapphire n 2 =1+ a1λ2<br />

+<br />

a2λ2<br />

+<br />

λ 2 − b 1 λ 2 − b 2<br />

a 1 =1.023798<br />

a 2 =1.058264<br />

a3λ2<br />

a 3 =5.280792<br />

λ 2 − b 3<br />

b 1 =0.00377588<br />

b 2 =0.0122544<br />

b 3 = 321.3616<br />

Here, <strong>the</strong> derivatives are evaluated at ω 0 . ∂φ/∂ω is <strong>the</strong> group delay T g , ∂ 2 φ/∂ω 2 <strong>the</strong> <strong>Group</strong> Delay<br />

Dispersion (GDD), ∂ 3 φ/∂ω 3 <strong>the</strong> Third-Order Dispersion (TOD). The GDD describes a linear<br />

frequency dependence of <strong>the</strong> group delay and thus tends to separate <strong>the</strong> frequency components of<br />

a pulse: For positive GDD, e.g., <strong>the</strong> components with higher frequencies are delayed with respect<br />

to those with lower frequencies, which results in a positive “chirp” (“up-chirp”) of <strong>the</strong> pulse.<br />

Higher orders of dispersion generate more complicated distortions. Material dispersion is normally<br />

described with Sellmeier equations for <strong>the</strong> refractive index as a function of <strong>the</strong> wavelength, i.e.<br />

n (λ). With <strong>the</strong> Sellmeier equations (Table <strong>2.1</strong>.6) all <strong>the</strong> necessary dispersive quantities can be<br />

calculated (Table <strong>2.1</strong>.7). An example is given in Table <strong>2.1</strong>.8.<br />

The broader <strong>the</strong> bandwidth of <strong>the</strong> pulse (i.e., <strong>the</strong> shorter <strong>the</strong> pulse duration), <strong>the</strong> more terms<br />

of this expansion are significant. GDD which acts on an initially unchirped Gaussian pulse with<br />

Full-Width-at-Half-Maximum (FWHM) pulse duration τ 0 , increases <strong>the</strong> pulse duration according<br />

to [86Sie]<br />

√<br />

( )<br />

τ p (z)<br />

4ln2d2 φ/d ω<br />

= 1+<br />

2 2<br />

, (<strong>2.1</strong>.20)<br />

τ 0<br />

τ 2 0<br />

where it is assumed that <strong>the</strong> incident pulse is transform-limited, i.e. <strong>the</strong> time–bandwidth product of<br />

<strong>the</strong> Gaussian pulse is τ 0 Δ ν p =0.4413, where Δ ν p is <strong>the</strong> Full-Width-at-Half-Maximum (FWHM)<br />

spectral width of <strong>the</strong> pulse intensity (Fig. <strong>2.1</strong>.15). Only second-order dispersion (i.e. ∂ 2 φ/∂ ω 2 )<br />

and higher orders are broadening <strong>the</strong> pulse. The first-order dispersion gives <strong>the</strong> group delay, i.e.<br />

<strong>the</strong> delay of <strong>the</strong> peak of <strong>the</strong> pulse envelope. It is apparent that <strong>the</strong> effect of GDD becomes strong<br />

if GDD >τ 2 0 . Similarly, TOD becomes important if TOD >τ 3 0 . It is important to note that<br />

for dispersive pulse broadening (which is in <strong>the</strong> linear pulse propagation regime) <strong>the</strong> spectrum<br />

of <strong>the</strong> pulse remains unchanged, only <strong>the</strong> spectral content of <strong>the</strong> pulse is redistributed in time.<br />

With positive dispersion <strong>the</strong> long-wavelength part of <strong>the</strong> spectrum is in <strong>the</strong> leading edge of <strong>the</strong><br />

pulse and <strong>the</strong> short-wavelength part in <strong>the</strong> trailing edge of <strong>the</strong> pulse, i.e. “red is faster than blue”<br />

(Fig. <strong>2.1</strong>.15). In <strong>the</strong> regime of strong pulse broadening, i.e. d 2 φ/d ω 2 ≫ τ 2 0 , we can reduce (<strong>2.1</strong>.20)<br />

Landolt-Börnstein<br />

New Series VIII/1B1

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