exotic nuclei structure and reaction noyaux exotiques ... - IPN - IN2P3

exotic nuclei structure and reaction noyaux exotiques ... - IPN - IN2P3 exotic nuclei structure and reaction noyaux exotiques ... - IPN - IN2P3

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X direction (mm) Y direction (mm) Figure 2 : Vertical section of the 130 kV Pegase platform with the main elements umn including the ion source, the lens, the Wien filter, and which duplicates the Orion facility working at the Tandem terminal since 1993 at around 10 MeV. The focusing of the new equipment will be, however, much improved in order to reach the micron objective. This set up is then connected to a diagnostic chamber containing deflection plates, a collimator holder with different size collimators and a Faraday cup. The collimator position is precisely adjustable and the Faraday cup measures the intensity of the beam selected by the Wien filter and passing through the collimator chosen by the user at the platform level. All the power supplies and the electronics are set on this platform, driven and controlled via about thirty optical fibers. The acceleration occurs after the diagnostic chamber through an accelerator gap made of 2 tubes one of which is a “trumpet” calculated by J. Arianer (fig 2) In the first experiments, we use the focusing properties of this gap. The future focusing beam line incorporates a “Russian” quadruplet with weak aberrations [7] which permits to obtain one µm beam spot (fig 3). This PEGASE project submitted in July 2007 by E.A. Schweikert to the NSF was accepted in February 2008. The realization started at the end of June 2008 and was finished at the end of November 2009 when the platform was transferred to the Texas A&M University, after it was delivered and tested at the IPN in October. The IPN tests went up to 100 kV and gave a total beam intensity of 300 nA. The transmission is better than 80 %. A selected Au 400 4+ beam was accelerated at 480 keV with a 1 nA intensity. The first gold nanodroplets beam at 35 km/s was obtained on October the 22 nd . The first experiments started in February 2010, at Texas A&M University, the Pegase platform being connected to a Time-of-Flight mass spectrometer. The first secondary ions spectra have been obtained from a silicon wafer and a CsI target. These first experiments permitted to test the transmission of the cluster beams and simultaneously the ToF mass spectrometer and the first stage of the electron emission microscope. 10 5 0 5 10 0 500 1000 1500 2000 Beam line distance from the source (mm) Figure 3: An example of simulation of the Pegase Beam line from the LMISource to the Russian quadrupoles with the full cluster beam. There are clearly two focussing points one behind the 130 kV acceleration lens (Pegase first step) and the other behind the Russian quadrupoles After these tests the experiments in progress concern the measurement of the massive cluster energy losses. At Orsay with 200 keV/atom massive cluster ions we showed that there was no pronounced coherent effect after the passage through 25 nm of matter, the zone close to the surface where the coherent effect is strongest is thus negligible with respect to the total range [8]. 101

But at 80 keV total energy ( 200 eV/atom) we observed a full coherent effect [9] with a projected range increased by a factor of almost 6 to 8 because of the clearing the way effect (the first cluster atoms entering in the solids push away the target atoms and so open an easy path for their followers). It is thus important to control in the range from 40 keV to 400 keV of total energy what is the contribution of the coherent motion on the energy loss, the part of the clearing the way effect versus the friction processes (effect of the charge at the surface Coulomb explosion etc) observed between 200 keV per charge and 4 MeV per charge [2]. The targets are carbon foils of 5, 10, 15 nm. The reference of these measurements are the 20-100 keV beams of Au 1-5 [10]. The secondary ion and electron emission are measured from the backside of the target and simultaneously we measure the velocity of the projectiles or fragments by time of flight. The first results show that the massive cluster passes through 15 nm of carbon at 80 keV per charge and produces an ion emission of carbon clusters; It is important to notice that an atomic ion with the same velocity is stopped by 3 nm of carbon and that 15 nm is the range of atomic gold at 27 keV or Au 3 at 80 keV; this has been controlled experimentally. These measurements will allow to establish the transition between coherent effect and independent atomic interaction and also to know the energy deposited in the first 10 nm of matter which contributes to the secondary emission from the solid. References [1] S. Bouneau, et al , Nucl. Instr. And Meth. B225, 579-589, 2004. [2] A.Tempez, et al, Rapid Comm; in Mass Spectrom. 18 371- 376, 2004. [3] C. Guillermier, et al, Applied Surface Science 252, 6529- 6532, 2006. [4] C. Guillermier, et al, Int. Journal of Mass Spect., Volume 263, Issues 2-3, 5, 298-303, 2007. [5]C.Guillermier, et al, Int. Journal of Mass Spect., 275, 86-90, 2008. [6]S. Della-Negra, et al, Surface and Interface Analysis, accepted, 2010. [7]A.D.Dymnikov and S.Y. Yavor.,Sov. Phys. Techn. Phys., 8- 7, 639, 1964. [8]S. Bouneau, et al,. Nucl. Instr. And Meth. B 251, 383-389, 2006. [9] S. Della-Negra, M. Pautrat, G. Rizza, In preparation [10]H.H. Andersen, et al, Nucl. Instr. and Meth. B212, 56, 2003. 102

X direction (mm)<br />

Y direction (mm)<br />

Figure 2 : Vertical section of the 130 kV Pegase<br />

platform with the main elements<br />

umn including the ion source, the lens, the Wien<br />

filter, <strong>and</strong> which duplicates the Orion facility working<br />

at the T<strong>and</strong>em terminal since 1993 at around<br />

10 MeV. The focusing of the new equipment will<br />

be, however, much improved in order to reach the<br />

micron objective. This set up is then connected to<br />

a diagnostic chamber containing deflection plates,<br />

a collimator holder with different size collimators<br />

<strong>and</strong> a Faraday cup. The collimator position is precisely<br />

adjustable <strong>and</strong> the Faraday cup measures<br />

the intensity of the beam selected by the Wien filter<br />

<strong>and</strong> passing through the collimator chosen by the<br />

user at the platform level. All the power supplies<br />

<strong>and</strong> the electronics are set on this platform, driven<br />

<strong>and</strong> controlled via about thirty optical fibers. The<br />

acceleration occurs after the diagnostic chamber<br />

through an accelerator gap made of 2 tubes one of<br />

which is a “trumpet” calculated by J. Arianer (fig 2)<br />

In the first experiments, we use the focusing properties<br />

of this gap.<br />

The future focusing beam line incorporates a<br />

“Russian” quadruplet with weak aberrations [7]<br />

which permits to obtain one µm beam spot (fig 3).<br />

This PEGASE project submitted in July 2007 by<br />

E.A. Schweikert to the NSF was accepted in February<br />

2008. The realization started at the end of<br />

June 2008 <strong>and</strong> was finished at the end of November<br />

2009 when the platform was transferred to the<br />

Texas A&M University, after it was delivered <strong>and</strong><br />

tested at the <strong>IPN</strong> in October.<br />

The <strong>IPN</strong> tests went up to 100 kV <strong>and</strong> gave a total<br />

beam intensity of 300 nA. The transmission is better<br />

than 80 %. A selected Au 400 4+ beam was accelerated<br />

at 480 keV with a 1 nA intensity. The first<br />

gold nanodroplets beam at 35 km/s was obtained<br />

on October the 22 nd .<br />

The first experiments started in February 2010, at<br />

Texas A&M University, the Pegase platform being<br />

connected to a Time-of-Flight mass spectrometer.<br />

The first secondary ions spectra have been obtained<br />

from a silicon wafer <strong>and</strong> a CsI target. These<br />

first experiments permitted to test the transmission<br />

of the cluster beams <strong>and</strong> simultaneously the ToF<br />

mass spectrometer <strong>and</strong> the first stage of the electron<br />

emission microscope.<br />

10<br />

5<br />

0<br />

5<br />

10<br />

0 500 1000 1500 2000<br />

Beam line distance from the source (mm)<br />

Figure 3: An example of simulation of the Pegase<br />

Beam line from the LMISource to the<br />

Russian quadrupoles with the full cluster<br />

beam. There are clearly two focussing<br />

points one behind the 130 kV acceleration<br />

lens (Pegase first step) <strong>and</strong> the other behind<br />

the Russian quadrupoles<br />

After these tests the experiments in progress concern<br />

the measurement of the massive cluster energy<br />

losses. At Orsay with 200 keV/atom massive<br />

cluster ions we showed that there was no pronounced<br />

coherent effect after the passage through<br />

25 nm of matter, the zone close to the surface<br />

where the coherent effect is strongest is thus negligible<br />

with respect to the total range [8].<br />

101

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