exotic nuclei structure and reaction noyaux exotiques ... - IPN - IN2P3
exotic nuclei structure and reaction noyaux exotiques ... - IPN - IN2P3
exotic nuclei structure and reaction noyaux exotiques ... - IPN - IN2P3
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one of them is made with a neptunium of different<br />
origin, with a higher content of 241 Am. Any problem<br />
with the 235 U reference target can be discarded<br />
because it leads to the expected cross sections for<br />
234 U, as shown above, <strong>and</strong> also 233 U. The backing<br />
thicknesses have been measured by the slowing<br />
down of the α particles, <strong>and</strong> the O <strong>and</strong> H contents<br />
Fig. 2. Fission cross section of 234 U above the threshold, obtained<br />
from the measured ratio to 235 U <strong>and</strong> the 235 U cross section.<br />
lar for all targets, the ratio of efficiencies between<br />
targets is close to 1. This can be checked for the 4<br />
targets of 237 Np <strong>and</strong> also for the 2 targets of 234 U.<br />
As illustrated in figure 1 the efficiency is reproducible<br />
within 3%. The angular distribution of fission<br />
fragments affects the efficiency due to the truncation<br />
of the detectable angle range. This effect has<br />
been included as a correction on the ratio of efficiencies.<br />
Overall the systematic uncertainty is<br />
about 4%.<br />
Figure 2 shows the fission cross section of 234 U<br />
above 100 keV. The reference cross section for<br />
235 U is taken from ENDF-B7 up to 30 MeV <strong>and</strong><br />
from the high energy extension of JENDL-3.3<br />
above. The steep rises at 0.6, 7 <strong>and</strong> 15 MeV correspond<br />
to the openings of 1st, 2nd <strong>and</strong> 3rd chance<br />
Fig. 4. Fission cross section of 237 Np below the fission threshold<br />
have been assessed by RBS of 3 MeV protons. In<br />
addition the angular distribution varies with energy,<br />
but is similar for 237 Np <strong>and</strong> 235 U. All these effects<br />
have been included in the efficiency correction <strong>and</strong><br />
Fig. 5. Fission cross section of 209 Bi<br />
Fig. 3. Fission cross section of 237 Np above the threshold, obtained<br />
from the measured ratio to 235 U <strong>and</strong> the 235 U cross section.<br />
fission. Our data are in good agreement with previous<br />
measurements, but above 1 MeV we are lower<br />
than the data from Lisowski [2] which extend up to<br />
400 MeV.<br />
Similarly figure 3 shows the fission cross section of<br />
237 Np above 500 keV. Although the shape is very<br />
similar to the one derived from the most recent<br />
measurements (Shcherbakov [3], <strong>and</strong> also<br />
Lisowski not plotted in the figure), our data are systematically<br />
higher by 6 % above 1 MeV. It’s worth<br />
mentioning that these higher values are obtained<br />
equally with each of the 4 237 Np targets although<br />
we consider that our data are safe<br />
Figure 4 shows the cross section between 1 <strong>and</strong><br />
300 keV confirming the recent measurement from<br />
Tovesson which invalidates the ENDF-B6 database<br />
which is now correctly updated in ENDF-B7.<br />
Figure 5 shows the cross section obtained for 209 Bi.<br />
It’s worth stressing that our data are in agreement<br />
with previous measurements which lie essentially<br />
below 200 MeV. The systematics based on these<br />
measurements departs from our values above 200<br />
MeV where data were lacking At 1 GeV our data<br />
join the Prokofiev systematics [4] defined for proton-induced<br />
fission.<br />
References<br />
[1] L. Ferrant, University Thesis, Orsay, 7 Sept 2005<br />
[2] P. Lisowski et al., Conf. on Nucl. Data for Sci. <strong>and</strong><br />
Technol. Juelich p. p. 732 (1991).<br />
[3] O. Shcherbakov et al., J. Nucl. Sci. <strong>and</strong> Tech., Supplement<br />
Vol. 2 p. 230 (2002).<br />
[4] A. V. Prokofiev. NIM A, 463:557, 2001.<br />
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