Nuclear Production of Hydrogen, Fourth Information Exchange ...
Nuclear Production of Hydrogen, Fourth Information Exchange ... Nuclear Production of Hydrogen, Fourth Information Exchange ...
CONCEPTUAL DESIGN OF THE HTTR-IS NUCLEAR HYDROGEN PRODUCTION SYSTEM Introduction Japan Atomic Energy Agency (JAEA) has been conducting R&D on both high-temperature reactors and hydrogen production technologies. Concerning reactor technology, an HTTR was constructed at Oarai, Japan and successfully delivered 950°C heat outside its reactor vessel (Fujikawa, 2004). Regarding hydrogen production technology, JAEA has been conducting R&D for a thermochemical water-splitting iodine-sulphur process (IS process), and achieved a continuous hydrogen production of 31 NL/h for 175 hours using a bench-scale apparatus in 2004 (Kubo, 2004). Followed by pilot plant experiment, JAEA plans to construct a hydrogen production system with the IS process utilising heat from the HTTR (HTTR-IS system), which is expected to be the world’s first demonstration on hydrogen production utilising heat directly supplied from a nuclear reactor (Sakaba, 2007). One of the key issues for the nuclear hydrogen demonstration is the IHX tube rupture scenario (IHXTR). In case of the HTTR design, the secondary cooling system is included in the containment vessel (CV), and cooling ability is sufficient by secondary pressurised water cooling system during the scenario. Hence, there is no significant impact on either reactor safety or public exposure. In contrast, the secondary cooling system of HTTR-IS system penetrates the CV and reactor building in order to provide heat to the hydrogen production plant. Thus the containment isolation valves should be automatically closed detecting an appropriate signal from engineered safety features actuation system in order to reduce radionuclide transportation from primary to secondary cooling system. Furthermore, core cooling and component integrity should be reinvestigated due to the procedure change in IHXTR. This paper summarises the HTTR-IS nuclear hydrogen production system and discusses detection method of heat transfer tube rupture of IHX and system analysis results during IHXTR. Conceptual design of the HTTR-IS system A tentative flow diagram of the HTTR-IS system is shown in Figure 1 and the major design specifications are shown in Table 1. The HTTR-IS system consists of the reactor, primary cooling system, secondary cooling system and IS process. At rated operation of the HTTR-IS system, primary pressurised water cooler (PPWC) and IHX are used in parallel and remove the heat of the reactor core. The heat produced by the reactor core transfers to the secondary cooling system at the IHX. Secondary cooling system penetrates CV and flows through the inner tube of the concentric hot gas duct in order to provide heat to the IS process. At the IS process, secondary helium gas provides heat to process heat exchangers, etc., such as a H 2 SO 4 decomposer, a HI decomposer, and a re-boiler of the HI distillation column. Downstream of the IS process, a steam generator and a helium gas cooler are installed as a thermal buffer. Finally, the helium gas is compressed by a secondary helium circulator and flows through the outer tube of the concentric hot gas duct and flows back to the IHX. Figure 1: Flow diagram of the HTTR-IS system Containment vessel Containment isolation valves Auxiliary cooling system Reactor IHX Concentric -hot gas duct IS process Steam generator PPWC Secondary helium circulator Helium cooler 388 NUCLEAR PRODUCTION OF HYDROGEN – © OECD/NEA 2010
CONCEPTUAL DESIGN OF THE HTTR-IS NUCLEAR HYDROGEN PRODUCTION SYSTEM Table 1: Major specifications of the HTTR-IS system Item Value Reactor power 30 MWt Thermal load of IS process Ca. 8 MWt Reactor outlet temperature 950°C Primary Reactor inlet temperature 395°C cooling system Reactor inlet pressure 4.0 MPa Reactor inlet flow rate 10.1 kg/s IS process inlet temperature 880°C Secondary IS process outlet temperature 253°C cooling system IHX inlet pressure 4.0 MPa IHX inlet flow rate 2.5 kg/s Figure 2 shows a schematic diagram of the helium pressure control system in the HTTR-IS system. The primary coolant pressure is controlled by the primary helium pressure control system at about 4.0 MPa with actuating valves of the helium storage and supply system. Secondary coolant pressure is controlled higher than primary helium pressure at about 0.07 MPa by primary-secondary differential pressure control system in order to prevent radionuclide transportation from the primary to secondary cooling system with actuating valves of the secondary helium storage and supply system. The flow meter is installed at the inlet and outlet of the primary and secondary helium storage and supply systems. In the current HTTR, the integral flow rate of the primary helium gas supply is calculated by the software in order to detect the leakage rate of primary cooling system. Figure 2: Schematic diagram of the helium pressure control system in the HTTR-IS system Primary He pressure control system 1 Secondary He storage & supply system Primarysecondary differential pressure control system Primary He storage & supply system Secondary He purification system 2 Primary He purification system 2 ? P IS process IHX Auxiliary heat exchanger Reactor P 1 PPWC Description of IHXTR In the current HTTR, the whole secondary cooling system is involved in the CV so that there is no need for considering radionuclide transportation outside of the CV in case of IHXTR. Also, the safety analysis result showed that there are no significant impacts on reactor cooling ability and therefore the scenario is not identified as a selected event in the safety evaluation. NUCLEAR PRODUCTION OF HYDROGEN – © OECD/NEA 2010 389
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CONCEPTUAL DESIGN OF THE HTTR-IS NUCLEAR HYDROGEN PRODUCTION SYSTEM<br />
Introduction<br />
Japan Atomic Energy Agency (JAEA) has been conducting R&D on both high-temperature reactors and<br />
hydrogen production technologies. Concerning reactor technology, an HTTR was constructed at Oarai,<br />
Japan and successfully delivered 950°C heat outside its reactor vessel (Fujikawa, 2004). Regarding<br />
hydrogen production technology, JAEA has been conducting R&D for a thermochemical water-splitting<br />
iodine-sulphur process (IS process), and achieved a continuous hydrogen production <strong>of</strong> 31 NL/h for<br />
175 hours using a bench-scale apparatus in 2004 (Kubo, 2004). Followed by pilot plant experiment,<br />
JAEA plans to construct a hydrogen production system with the IS process utilising heat from the HTTR<br />
(HTTR-IS system), which is expected to be the world’s first demonstration on hydrogen production<br />
utilising heat directly supplied from a nuclear reactor (Sakaba, 2007).<br />
One <strong>of</strong> the key issues for the nuclear hydrogen demonstration is the IHX tube rupture scenario<br />
(IHXTR). In case <strong>of</strong> the HTTR design, the secondary cooling system is included in the containment<br />
vessel (CV), and cooling ability is sufficient by secondary pressurised water cooling system during the<br />
scenario. Hence, there is no significant impact on either reactor safety or public exposure. In contrast,<br />
the secondary cooling system <strong>of</strong> HTTR-IS system penetrates the CV and reactor building in order to<br />
provide heat to the hydrogen production plant. Thus the containment isolation valves should be<br />
automatically closed detecting an appropriate signal from engineered safety features actuation system<br />
in order to reduce radionuclide transportation from primary to secondary cooling system. Furthermore,<br />
core cooling and component integrity should be reinvestigated due to the procedure change in IHXTR.<br />
This paper summarises the HTTR-IS nuclear hydrogen production system and discusses detection<br />
method <strong>of</strong> heat transfer tube rupture <strong>of</strong> IHX and system analysis results during IHXTR.<br />
Conceptual design <strong>of</strong> the HTTR-IS system<br />
A tentative flow diagram <strong>of</strong> the HTTR-IS system is shown in Figure 1 and the major design specifications<br />
are shown in Table 1. The HTTR-IS system consists <strong>of</strong> the reactor, primary cooling system, secondary<br />
cooling system and IS process. At rated operation <strong>of</strong> the HTTR-IS system, primary pressurised water<br />
cooler (PPWC) and IHX are used in parallel and remove the heat <strong>of</strong> the reactor core. The heat produced<br />
by the reactor core transfers to the secondary cooling system at the IHX. Secondary cooling system<br />
penetrates CV and flows through the inner tube <strong>of</strong> the concentric hot gas duct in order to provide heat<br />
to the IS process. At the IS process, secondary helium gas provides heat to process heat exchangers,<br />
etc., such as a H 2 SO 4 decomposer, a HI decomposer, and a re-boiler <strong>of</strong> the HI distillation column.<br />
Downstream <strong>of</strong> the IS process, a steam generator and a helium gas cooler are installed as a thermal<br />
buffer. Finally, the helium gas is compressed by a secondary helium circulator and flows through the<br />
outer tube <strong>of</strong> the concentric hot gas duct and flows back to the IHX.<br />
Figure 1: Flow diagram <strong>of</strong> the HTTR-IS system<br />
Containment vessel<br />
Containment<br />
isolation valves<br />
Auxiliary<br />
cooling<br />
system<br />
Reactor<br />
IHX<br />
Concentric<br />
-hot gas<br />
duct<br />
IS process<br />
Steam<br />
generator<br />
PPWC<br />
Secondary<br />
helium<br />
circulator<br />
Helium<br />
cooler<br />
388 NUCLEAR PRODUCTION OF HYDROGEN – © OECD/NEA 2010