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EXPERIMENTAL STUDY OF THE VAPOUR-LIQUID EQUILIBRIA OF HI-I 2-H 2O TERNARY MIXTURES Figure 4: Total pressure vs. [HI] molar for various [I 2 ] molar 2000 1500 130°C 39% Iodine 50% Iodine P (mbar) 1000 500 85% Iodine 65% Iodine 25% Iodine 12% Iodine 4% Iodine 0 0 2 4 6 8 10 12 14 16 18 %HI Figure 5 Measured total pressure (mbar) 1700 1600 1500 1400 1300 1200 1100 1000 900 800 700 600 500 400 300 200 100 0 Our measurements Prophy calculations Neumann value 9,5 10,0 10,5 11,0 11,5 12,0 12,5 13,0 [HI] molar % HI 1 0.0018 0.0019 0.002 0.0021 0.0022 0.0023 0.0024 0.0025 0.0026 Figure 6 H 2 O 1 0.0018 0.0019 0.002 0.0021 0.0022 0.0023 0.0024 0.0025 0.0026 I 2 1 0.0018 0.002 0.0022 0.0024 0.0026 0.1 0.1 0.1 C (mol/L 0.01 0.001 C (mol/L 0.01 C (mol/L) 0.01 (g) exp. (g) ProPhy 0.0001 0.00001 (g) exp. (h) exp. (i) exp. (g) ProPhy (h) ProPhy (i) ProPhy K -1 0.001 (g) exp. (h) exp. (i) exp. (g) PropHy (h) ProPhy (i) ProPhy K -1 0.001 (h) exp. (i) exp. (h) ProPhy (i) ProPhy K -1 196 NUCLEAR PRODUCTION OF HYDROGEN – © OECD/NEA 2010
EXPERIMENTAL STUDY OF THE VAPOUR-LIQUID EQUILIBRIA OF HI-I 2-H 2O TERNARY MIXTURES Figure 7 HI H 2 O I 2 T (°C) 1 120 170 220 270 T (°C) 1 120 170 220 270 T (°C) 0.1 120 170 220 270 0.1 0.1 C (mol/L) 0.01 0.001 C (mol/L) C (mol/L) 0.01 0.01 0.0001 0.00001 (a) exp. r=0.16 (a) ProPhy (b) exp. r= 0.19 (b) ProPhy (c ) exp. r= 0.22 (c ) ProPhy 0.001 (a) exp. r= 0.16 (a) ProPhy (b) exp. r= 0.19 (b) ProPhy (c ) exp. r= 0.22 (c ) ProPhy 0.001 (a) exp. r= 0.16 (a) ProPhy (b) exp. r= 0.19 (b) ProPhy (c ) exp. r= 0.22 (c ) ProPhy Figure 8 HI H 2 O I 2 T (°C) 1 90 110 130 150 170 190 210 230 T (°C) 1 90 110 130 150 170 190 210 230 T (°C) 0.1 90 110 130 150 170 190 210 230 0.1 0.1 0.01 C (mol/L) C (mol/L) C (mol/L) 0.01 0.01 0.001 0.001 (d) exp. r=0.16 (e) exp. r=0.18 (f) exp. r=0.22 (d) ProPhy (e) ProPhy (f) ProPhy 0.001 (d) exp. r=0.16 (d) ProPhy (e) exp. r= 0.18 (e) ProPhy (f) exp. r=0.22 (f) ProPhy 0.0001 (d) exp. r=0.16 (e) exp. r=0.18 (f) exp. r=0.22 (d) ProPhy (e) ProPhy (f) ProPhy References Belaissaoui, B., et al. (2008), Chemical Engineering and Processing: Process Intensification, Vol. 47, No. 3, 396-407. Bamberger, C.E. (1978), “Hydrogen Production from Water by Thermochemical Cycles: A 1977 Update”, Cryogenics, 170-183. Doizi, D., et al. (2007), “Total and Partial Pressure Measurements for the Sulphur-Iodine Thermochemical Cycle”, Int. J. Hydrogen Energy, 32 (9), 1183-1191. Doizi, D., et al. (2009), “Experimental Study of the Vapour-liquid Equilibria of HI-I 2 -H 2 O Ternary Mixtures. Part 1: Experimental Results Around the Atmospheric Pressure”, Int. J. Hydrogen Energy, forthcoming. NUCLEAR PRODUCTION OF HYDROGEN – © OECD/NEA 2010 197
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Nuclear Science 2010 Nuclear Produc
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ORGANISATION FOR ECONOMIC CO-OPERAT
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TABLE OF CONTENTS Table of contents
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TABLE OF CONTENTS Y. Gong, E. Chalk
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EXECUTIVE SUMMARY Executive summary
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EXECUTIVE SUMMARY steam turbine, in
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EXECUTIVE SUMMARY sulphur depositio
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EXECUTIVE SUMMARY affords saving 35
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EXECUTIVE SUMMARY safety assessment
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EXECUTIVE SUMMARY The question was
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CHANGING THE WORLD WITH HYDROGEN AN
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NUCLEAR HYDROGEN PRODUCTION PROGRAM
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NUCLEAR HYDROGEN PRODUCTION PROGRAM
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FRENCH RESEARCH STRATEGY TO USE NUC
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PRESENT STATUS OF HTGR AND HYDROGEN
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STATUS OF THE KOREAN NUCLEAR HYDROG
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THE CONCEPT OF NUCLEAR HYDROGEN PRO
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CANADIAN NUCLEAR HYDROGEN R&D PROGR
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APPLICATION OF NUCLEAR-PRODUCED HYD
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STATUS OF THE INL HIGH-TEMPERATURE
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HIGH-TEMPERATURE STEAM ELECTROLYSIS
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MATERIALS DEVELOPMENT FOR SOEC Mate
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A METALLIC SEAL FOR HIGH-TEMPERATUR
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DEGRADATION MECHANISMS IN SOLID OXI
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Page 149 and 150: CAUSES OF DEGRADATION IN A SOLID OX
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Page 157 and 158: NUCLEAR HYDROGEN USING HIGH TEMPERA
Page 167: SESSION III: THERMOCHEMICAL SULPHUR
Page 170 and 171: CEA ASSESSMENT OF THE SULPHUR-IODIN
Page 181: STATUS OF THE INERI SULPHUR-IODINE
Page 184 and 185: INFLUENCE OF HTR CORE INLET AND OUT
Page 194 and 195: EXPERIMENTAL STUDY OF THE VAPOUR-LI
Page 203: DEVELOPMENT OF HI DECOMPOSITION PRO
Page 206 and 207: SOUTH AFRICA’S NUCLEAR HYDROGEN P
Page 216 and 217: INTEGRATED LABORATORY SCALE DEMONST
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Page 229 and 230: RECENT CANADIAN ADVANCES IN THE THE
Page 237 and 238: AN OVERVIEW OF R&D ACTIVITIES FOR T
Page 245 and 246: STUDY OF THE HYDROLYSIS REACTION OF
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STUDY OF THE HYDROLYSIS REACTION OF
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STUDY OF THE HYDROLYSIS REACTION OF
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DEVELOPMENT OF CuCl-HCl ELECTROLYSI
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EXERGY ANALYSIS OF THE Cu-Cl CYCLE
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CaBr 2 HYDROLYSIS FOR HBr PRODUCTIO
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SESSION V: ECONOMICS AND MARKET ANA
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DEVELOPMENT OF THE HYDROGEN ECONOMI
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NUCLEAR H 2 PRODUCTION - A UTILITY
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ALKALINE AND HIGH-TEMPERATURE ELECT
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THE PRODUCT OF HYDROGEN BY NUCLEAR
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SUSTAINABLE ELECTRICITY SUPPLY IN T
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PROHYTEC, THE FRENCH INDUSTRIAL PLA
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NHI ECONOMIC ANALYSIS OF CANDIDATE
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MARKET VIABILITY OF NUCLEAR HYDROGE
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POSSIBILITY OF ACTIVE CARBON RECYCL
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NUCLEAR SAFETY AND REGULATORY CONSI
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TRANSIENT MODELLING OF S-I CYCLE TH
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PROPOSED CHEMICAL PLANT INITIATED A
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CONCEPTUAL DESIGN OF THE HTTR-IS NU
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USE OF PSA FOR DESIGN OF EMERGENCY
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HEAT PUMP CYCLE BY HYDROGEN-ABSORBI
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HEAT EXCHANGER TEMPERATURE RESPONSE
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ALTERNATE VHTR/HTE INTERFACE FOR MI
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POSTER SESSION CONTRIBUTIONS Poster
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ACTIVITIES OF NUCLEAR RESEARCH INST
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ACTIVITIES OF NUCLEAR RESEARCH INST
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A URANIUM THERMOCHEMICAL CYCLE FOR
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A URANIUM THERMOCHEMICAL CYCLE FOR
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MEETING ORGANISATION Annex 1: Meeti
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LIST OF PARTICIPANTS REYTIER, Magal
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LIST OF PARTICIPANTS BROWN, Nichola
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LIST OF PARTICIPANTS SINK, Carl US
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