Itinerant Spin Dynamics in Structures of ... - Jacobs University
Itinerant Spin Dynamics in Structures of ... - Jacobs University Itinerant Spin Dynamics in Structures of ... - Jacobs University
26 Chapter 3: WL/WAL Crossover and Spin Relaxation in Confined Systems precession axis and the amplitude of the total precession field is changing, since | B+B SO (−p) |=| B−B SO (p) |≠| B+B SO (p) |, resulting in spin dephasing and relaxation, as the sign of the momentum changes randomly. 3.1.2 Wires with W > λ F In this Chapter, we show, however, that the condition for a coherent spin precession is not only the 1d wire, 1/τ s is already strongly reduced in much wider wires: as soon as the wire width W is smaller than bulk spin precession length L SO , which is the length on which the electron spin precesses a full cycle. This explains the reduction of the spin relaxation rate in quantum wires for widths exceeding both the elastic mean-free path l e and λ F , as observed with optical[HSM + 06] as well as with WL measurements[DLS + 05, LSK + 07, SGP + 06, WGZ + 06, KKN09]. As an example we show two experiments in Fig.3.1, where the significant dimensional reduction has been observed. Since L SO can be several µm and is not changed significantly as the wire width W is reduced, such a reduction of spin relaxation can be very useful for applications: the spin of conduction electrons precesses coherently as it moves along the wire on length scale L SO . It becomes randomized and relaxes on the longer length scale L s (W) = √ D e τ s only [D e = v F l e /2 (v F , Fermi velocity) is the 2D diffusion constant]. To understand the connection between the conductivity measurements and spin relaxation we recall that quantum interference of electrons in low-dimensional, disordered conductors is known to result in corrections to the electrical conductivity ∆σ. This quantum correction, the WL effect, is a very sensitive tool to study dephasing and symmetry-breaking mechanisms in conductors.[AAKL82, Ber84, CS86] The entanglement of spin and charge by SO interaction reverses the effect of WL and thereby enhances the conductivity. This WAL effect was predicted by Hikami et al.[HLN80] for conductors with impurities of heavy elements. As conduction electrons scatter from such impurities, the SO interaction randomizes their spin. The resulting spin relaxation suppresses interference in spin triplet configurations. Sincethetime-reversal operation changes not only thesign of momentum but also the sign of the spin, the interference in singlet configuration remains unaffected. Since singlet interference reduces the electron’s return probability, it enhances the conductivity, which is named the WAL effect. In weak magnetic fields, the singlet contributions are suppressed. Thereby, the conductivity is reduced and the magnetoconductivity becomes negative. The
Chapter 3: WL/WAL Crossover and Spin Relaxation in Confined Systems 27 magnetoconductivity of wires is thus related to the magnitude of the spin relaxation rate. InSec.3.2, we firstderive thequantumcorrections to theconductivity for wires with general bulk SO interaction and relate it to the Cooperon propagator. In Sec.3.3, we diagonalize the Cooperon for two-dimensional (2D) electron systems with Rashba SO interaction. We compare the spectrum of the triplet Cooperon with the one of the spin-diffusion equation. InSec.3.4, we presentthesolution of the Cooperonequation for awiregeometry. We review the solutions of the spin-diffusion equation in the wire geometry and compare the resulting spin relaxation rate with the one extracted from the Cooperon equation. Then we proceed to calculate the quantum corrections to the conductivity using the exact diagonalization of the Cooperon propagator. In the last part of this section, we consider two other kinds of boundary conditions. We calculate the spin relaxation rate in narrow wires with adiabatic boundaries, which arise in wires with smooth lateral confinement and regard also tubular wires. In Sec.3.5, we study the influence of the Zeeman coupling to a magnetic field perpendicular to the quantum well in a system with sharp boundaries and analyze how the magnetoconductivity is modified. In Sec.3.6, we draw the conclusions and compare with experimental results. In AppendixC.2, we give the derivation of the non-Abelian Neumann boundary conditions for the Cooperon propagator. In AppendixC.3, we show the connection between the effective vector potential A S due to SO coupling and the spin relaxation tensor. InAppendixC.4, we give theexact quantumcorrection totheelectrical conductivity in 2D. In AppendixC.5, we detail the diagonalization of the Cooperon propagator. 3.2 Quantum Transport Corrections 3.2.1 Diagrammatic Approach As the temperature is lowered, we expect quantum mechanical coherence to be more important: The phase coherence length l ϕ increases with decreasing temperature. If l ϕ is much larger then the elastic scattering length but smaller then the sample size one would expect that all interference effects disappear due to self-averaging. However, it was found that one process seems to survive, as measurements show in logarithmically increasing resistance as temperature decreases, Fig.3.2. In order to introduce the problem of dephasing and WL, we begin with a semiclassical picture of how an electron propagates from a point r to r ′ : The corresponding probability amplitude P is given as the sum over
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26 Chapter 3: WL/WAL Crossover and <strong>Sp<strong>in</strong></strong> Relaxation <strong>in</strong> Conf<strong>in</strong>ed Systems<br />
precession axis and the amplitude <strong>of</strong> the total precession field is chang<strong>in</strong>g, s<strong>in</strong>ce<br />
| B+B SO (−p) |=| B−B SO (p) |≠| B+B SO (p) |,<br />
result<strong>in</strong>g <strong>in</strong> sp<strong>in</strong> dephas<strong>in</strong>g and relaxation, as the sign <strong>of</strong> the momentum changes randomly.<br />
3.1.2 Wires with W > λ F<br />
In this Chapter, we show, however, that the condition for a coherent sp<strong>in</strong> precession<br />
is not only the 1d wire, 1/τ s is already strongly reduced <strong>in</strong> much wider wires:<br />
as soon as the wire width W is smaller than bulk sp<strong>in</strong> precession length L SO , which is<br />
the length on which the electron sp<strong>in</strong> precesses a full cycle. This expla<strong>in</strong>s the reduction<br />
<strong>of</strong> the sp<strong>in</strong> relaxation rate <strong>in</strong> quantum wires for widths exceed<strong>in</strong>g both the elastic<br />
mean-free path l e and λ F , as observed with optical[HSM + 06] as well as with WL<br />
measurements[DLS + 05, LSK + 07, SGP + 06, WGZ + 06, KKN09]. As an example we show<br />
two experiments <strong>in</strong> Fig.3.1, where the significant dimensional reduction has been observed.<br />
S<strong>in</strong>ce L SO can be several µm and is not changed significantly as the wire width W is reduced,<br />
such a reduction <strong>of</strong> sp<strong>in</strong> relaxation can be very useful for applications: the sp<strong>in</strong><br />
<strong>of</strong> conduction electrons precesses coherently as it moves along the wire on length scale<br />
L SO . It becomes randomized and relaxes on the longer length scale L s (W) = √ D e τ s only<br />
[D e = v F l e /2 (v F , Fermi velocity) is the 2D diffusion constant].<br />
To understand the connection between the conductivity measurements and sp<strong>in</strong> relaxation<br />
we recall that quantum <strong>in</strong>terference <strong>of</strong> electrons <strong>in</strong> low-dimensional, disordered conductors<br />
is known to result <strong>in</strong> corrections to the electrical conductivity ∆σ. This quantum correction,<br />
the WL effect, is a very sensitive tool to study dephas<strong>in</strong>g and symmetry-break<strong>in</strong>g<br />
mechanisms <strong>in</strong> conductors.[AAKL82, Ber84, CS86] The entanglement <strong>of</strong> sp<strong>in</strong> and charge by<br />
SO <strong>in</strong>teraction reverses the effect <strong>of</strong> WL and thereby enhances the conductivity. This WAL<br />
effect was predicted by Hikami et al.[HLN80] for conductors with impurities <strong>of</strong> heavy elements.<br />
As conduction electrons scatter from such impurities, the SO <strong>in</strong>teraction randomizes<br />
their sp<strong>in</strong>. The result<strong>in</strong>g sp<strong>in</strong> relaxation suppresses <strong>in</strong>terference <strong>in</strong> sp<strong>in</strong> triplet configurations.<br />
S<strong>in</strong>cethetime-reversal operation changes not only thesign <strong>of</strong> momentum but also the<br />
sign <strong>of</strong> the sp<strong>in</strong>, the <strong>in</strong>terference <strong>in</strong> s<strong>in</strong>glet configuration rema<strong>in</strong>s unaffected. S<strong>in</strong>ce s<strong>in</strong>glet<br />
<strong>in</strong>terference reduces the electron’s return probability, it enhances the conductivity, which is<br />
named the WAL effect. In weak magnetic fields, the s<strong>in</strong>glet contributions are suppressed.<br />
Thereby, the conductivity is reduced and the magnetoconductivity becomes negative. The