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Itinerant Spin Dynamics in Structures of ... - Jacobs University

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22 Chapter 2: <strong>Sp<strong>in</strong></strong> <strong>Dynamics</strong>: Overview and Analysis <strong>of</strong> 2D Systems<br />

Perturbation theory yields then directly the correspond<strong>in</strong>g sp<strong>in</strong> relaxation rate<br />

1 ∑<br />

∫ dθ<br />

= πνn i<br />

τ s 2π (1−cosθ) | V SO(k,k ′ ) αβ | 2 , (2.34)<br />

α,β<br />

proportional to the concentration <strong>of</strong> impurities n i . Here α,β = ± denotes the sp<strong>in</strong> <strong>in</strong>dices.<br />

S<strong>in</strong>cethesp<strong>in</strong>-orbit<strong>in</strong>teraction <strong>in</strong>creases withtheatomic numberZ <strong>of</strong>theimpurityelement,<br />

this sp<strong>in</strong> relaxation <strong>in</strong>creases as Z 2 , be<strong>in</strong>g stronger for heavier element impurities.<br />

2.4.5 Bir-Aronov-Pikus <strong>Sp<strong>in</strong></strong> Relaxation<br />

Theexchange<strong>in</strong>teraction J betweenelectrons andholes<strong>in</strong>p-dopedsemiconductors<br />

results <strong>in</strong> sp<strong>in</strong> relaxation, as well.[BAP76] Its strength is proportional to the density <strong>of</strong><br />

holes p and depends on their it<strong>in</strong>erancy. If the holes are localized they act like magnetic<br />

impurities. If they are it<strong>in</strong>erant, the sp<strong>in</strong> <strong>of</strong> the conduction electrons is transfered by the<br />

exchange <strong>in</strong>teraction to the holes, where the sp<strong>in</strong>-orbit splitt<strong>in</strong>g <strong>of</strong> the valence bands results<br />

<strong>in</strong> fast sp<strong>in</strong> relaxation <strong>of</strong> the hole sp<strong>in</strong> due to the Elliott-Yafet, or the D’yakonov-Perel’<br />

mechanism.<br />

2.4.6 Magnetic Impurities<br />

Magnetic impurities have a sp<strong>in</strong> S which <strong>in</strong>teracts with the sp<strong>in</strong> <strong>of</strong> the conduction<br />

electrons by the exchange <strong>in</strong>teraction J, result<strong>in</strong>g <strong>in</strong> a spatially and temporarily fluctuat<strong>in</strong>g<br />

local magnetic field<br />

B MI (r) = − ∑ i<br />

Jδ(r−R i )S, (2.35)<br />

where the sum is over the position <strong>of</strong> the magnetic impurities R i . This gives rise to sp<strong>in</strong><br />

relaxation <strong>of</strong> the conduction electrons, with a rate given by<br />

1<br />

τ Ms<br />

= 2πn M νJ 2 S(S +1), (2.36)<br />

where n M is the density <strong>of</strong> magnetic impurities, and ν is the DOS at the Fermi energy.<br />

Here, S is the sp<strong>in</strong> quantum number <strong>of</strong> the magnetic impurity, which can take the values<br />

S = 1/2,1,3/2,2.... Antiferromagnetic exchange <strong>in</strong>teraction between the magnetic impurity<br />

sp<strong>in</strong> and the conduction electrons results <strong>in</strong> a competition between the conduction<br />

electrons to form a s<strong>in</strong>glet with the impurity sp<strong>in</strong>, which results <strong>in</strong> enhanced nonmagnetic<br />

and magnetic scatter<strong>in</strong>g. At low temperatures the magnetic impurity sp<strong>in</strong> is screened by

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