Coherent Backscattering from Multiple Scattering Systems - KOPS ...

Coherent Backscattering from Multiple Scattering Systems - KOPS ... Coherent Backscattering from Multiple Scattering Systems - KOPS ...

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2 Theory cooperon 1 0.8 0.6 0.4 l abs = 10 −5 m l abs = 3 ⋅ 10 −5 m l abs = 10 −4 m no absorption 0.2 0 −90 −60 −30 0 30 60 90 scattering angle [deg] Figure 2.13: Coherent backscattering with absorption. The graph shows the cooperon α c (θ, l abs ) calculated with eqn. 2.18 for different absorption lengths l abs = 3Dτ/l ∗ with λ = 590 nm, kl ∗ = 5, and non-reflective sample surface. function of time or respectively the pathlength. The longest photon paths have the narrowest Gaussians, while short paths have wide distributions. An infinite series of Gaussians creates a triangular cusp at the tip of the coherent backscattering cone. However, absorption as well as localization introduce a cutoff length for the photon paths, so that the narrowest Gaussians are eliminated. This explains why one observes a rounded conetip for absorbing or localizing samples (figs. 2.13, 3.4). The effect of absorption can be handled mathematically by introducing a substitution q 2 → q 2 + (Dτ) −1 in the cooperon [38]. With the correct normalization the cooperon for absorbing samples becomes α c (θ, τ) = ( Dτ l ∗ + ( l ∗ l ∗ + √ ) 2 ( Dτ 1−e −2q abs z 0 ( 1 − e − 2z 0 q abs l ∗ + 2µ µ+1 ) ) ) √ √Dτ ( ) Dτ q abs l ∗ + µ+1 2 (2.18) 2µ with q abs = √ q 2 + (Dτ) −1 . Anderson localization can be modeled by a transition from a constant diffusion coefficient D to a time-dependent coefficient D(t) ∝ t −1 at the localization time t loc [45]. As the ‘cutoff’ mechanism is different, the resulting shape of the conetip also differs from that of a purely absorbing sample (fig. 3.4). 22

2.7 The theory of coherent backscattering cooperon [a.u.] 0.3 0.25 0.2 0.15 0.1 l abs = 10 −5 m l abs = 3 ⋅ 10 −5 m l abs = 10 −4 m no absorption 0.05 0 −90 −60 −30 0 30 60 90 scattering angle [deg] Figure 2.14: Coherent backscattering with absorption – unnormalized cooperon. The graph shows the unnormalized cooperon for different absorption lengths l abs = 3Dτ/l ∗ with λ = 590 nm, kl ∗ = 5, and non-reflective sample surface. Deviations from the non-absorptive case at the cone flanks can be observed only for very short absorption lengths, which are irrelevant for our experimental situations. Both absorption and localization not only cause a rounding of the conetip, they also widen the cooperon. However, in many experimental situations the normalization of the diffuson and the cooperon by ∫ j(⃗r ⊥ , θ = 0) d⃗r ⊥ is unnecessary, as the experimental data are also not normalized. Applying the above transformations only to the numerator of the cooperon in eqn. 2.13 results in a lowered cone enhancement instead of a widened cooperon (fig. 2.14), so that the cone flanks are unaffected by absorption or localization. In the measurement of kl ∗ , an imprecise rendition of the very tip of the backscattering cone – which is rather common for narrow cones – is therefore no major source of errors, as the theory can be fitted to the flanks of the cone. 23

2 Theory<br />

cooperon<br />

1<br />

0.8<br />

0.6<br />

0.4<br />

l abs<br />

= 10 −5 m<br />

l abs<br />

= 3 ⋅ 10 −5 m<br />

l abs<br />

= 10 −4 m<br />

no absorption<br />

0.2<br />

0<br />

−90 −60 −30 0 30 60 90<br />

scattering angle [deg]<br />

Figure 2.13: <strong>Coherent</strong> backscattering with absorption. The graph shows the cooperon<br />

α c (θ, l abs ) calculated with eqn. 2.18 for different absorption lengths l abs = 3Dτ/l ∗ with<br />

λ = 590 nm, kl ∗ = 5, and non-reflective sample surface.<br />

function of time or respectively the pathlength. The longest photon paths have the narrowest<br />

Gaussians, while short paths have wide distributions.<br />

An infinite series of Gaussians creates a triangular cusp at the tip of the coherent backscattering<br />

cone. However, absorption as well as localization introduce a cutoff length for the photon<br />

paths, so that the narrowest Gaussians are eliminated. This explains why one observes a<br />

rounded conetip for absorbing or localizing samples (figs. 2.13, 3.4).<br />

The effect of absorption can be handled mathematically by introducing a substitution q 2 →<br />

q 2 + (Dτ) −1 in the cooperon [38]. With the correct normalization the cooperon for absorbing<br />

samples becomes<br />

α c (θ, τ) =<br />

(<br />

Dτ l ∗ +<br />

(<br />

l ∗ l ∗ + √ ) 2 (<br />

Dτ 1−e<br />

−2q abs z 0<br />

(<br />

1 − e − 2z 0<br />

q abs l ∗ + 2µ<br />

µ+1<br />

)<br />

) )<br />

√ √Dτ ( )<br />

Dτ q abs l ∗ + µ+1 2<br />

(2.18)<br />

2µ<br />

with q abs = √ q 2 + (Dτ) −1 .<br />

Anderson localization can be modeled by a transition <strong>from</strong> a constant diffusion coefficient D<br />

to a time-dependent coefficient D(t) ∝ t −1 at the localization time t loc [45]. As the ‘cutoff’<br />

mechanism is different, the resulting shape of the conetip also differs <strong>from</strong> that of a purely<br />

absorbing sample (fig. 3.4).<br />

22

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