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Marine Ecosystems Research Department - jamstec japan agency ...

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JAMSTEC 2002 Annual Report<br />

Frontier <strong>Research</strong> System for Global Change<br />

TRACE-P campaign was conducted. For evaluating<br />

the model performance, modeled concentrations of OH<br />

and HO were compared with observational data<br />

obtained onboard the DC- and P-B during the campaign.<br />

Comparison shows that simulated OH and HO <br />

concentrations agree reasonably well with observations,<br />

while calculated values are generally higher than<br />

the observed values. Fig. shows calculated regional<br />

distribution of OH and HO radicals in East Asia in the<br />

daytime on March , .<br />

The Air Quality Prediction Modeling System<br />

(AQPMS) is used to perform year-long, quantitative<br />

simulation of rainwater pH in East Asia. Monitoring<br />

data of EANET (the Acid Deposition Monitoring<br />

Network in East Asia) in addition to the field observation<br />

data of SEPA (State Environmental Protection<br />

Administration) of China are used to evaluate the<br />

model, and a reasonable agreement is obtained.<br />

c. Greenhouse Gases Modeling Group<br />

Using inverse model techniques, we select most<br />

effective procedures for future atmospheric CO observations.<br />

An assessment of the utility of CO vertical<br />

profile measurements by a solar occultation based<br />

satellite sensor is made. We have compared the<br />

impacts of these possible vertical profile observations<br />

and optimal extensions of the present surface measurement<br />

network on the estimation of CO regional<br />

sources from annual average CO concentration patterns<br />

by an inverse model. The satellite measurements<br />

are valuable to constrain the CO source uncertainties<br />

for the tropical lands with no existing observations.<br />

The optimal extension of the surface network appears<br />

to be the more effective way to reduce average inverse<br />

model uncertainty; however, in high resolution inversion<br />

the relative merit of the satellite data is higher<br />

than that in the low-resolution case. We show that the<br />

systematic errors in satellite observations can lead to<br />

significant shifts in the inverse model-estimated fluxes.<br />

Parallel version of the atmospheric transport model<br />

has been developed for high-resolution, long-term,<br />

multiple tracer simulations necessary for forward and<br />

inverse model analysis. CO fluxes, simulated with<br />

ecosystem model Biome-BGC, were prepared. We also<br />

continue developing and improving data analysis software,<br />

incorporating data fitting and filtering, editing<br />

and visualization. The analysis system was applied to<br />

shipboard measurement data of atmospheric N O over<br />

the Pacific Ocean.<br />

d. Atmospheric Composition Data Analysis Group<br />

Carbon monoxide total column amount is regularly<br />

measured over Hokkaido since and over Russia<br />

since . A comparison of these total columns<br />

reveals a systematic CO surplus over Hokkaido in<br />

summer months. Calculations based on isentropic trajectories<br />

and inventories of CO sources show that forest<br />

fires and combustion processes in populated areas<br />

contribute to this surplus (Fig.).<br />

The surface O and CO data from continuous meas-<br />

Fig.12 Simulated regional distribution of a) OH and b) HO 2 radicals in East Asia at 13Z<br />

on March 7, 2001 during TRACE-P campaign period.<br />

130

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