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<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Light Amplification by <strong>Stimulated</strong> <strong>Emission</strong> of Radiation<br />

Erasmus Intensive Program <strong>OREA</strong> <strong>2011</strong><br />

4 – 15 July <strong>2011</strong>, Department of Electronics<br />

TEI of Crete, Chania, Crete, Greece<br />

Dr Kostantinos Petridis


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

• Lasers: An invention that many of us take it as granted because we have<br />

grown up with, and has always been a part of our everyday lives.<br />

• The development of lasers has changed science forever and its various<br />

forms continue to have considerable impact in many areas of science,<br />

technology and industry.<br />

• 50 th anniversary of the laser invention (16 th of May 1960).


An Introduction – Fifty Brilliant Years<br />

In 1958 A.L.Schalow and C.H.<br />

Townes published the first theoretical<br />

work concerning laser operational<br />

principles.<br />

They expanded their research from<br />

microwave frequencies operated<br />

devices (masers) to optical frequency<br />

operated devices (lasers)<br />

The consequent development of the<br />

laser changed science forever.<br />

Arthur L. Schawlow Semiconductor lasers have<br />

revolutionized telecoms. Nd:YAG<br />

lasers have changed the way we<br />

perform material processing. Excimer<br />

lasers drive the semiconductor<br />

industry. Ti:Sapphire lasers enable<br />

ultrafast studies of matter<br />

Charles H. Townes<br />

Both scientists awarded with the<br />

Nobel prize for their work.<br />

7 7/3/11


An Introduction – Fifty Brilliant Years<br />

In 1960 Maiman build the<br />

first operational laser device.<br />

It was a ruby laser<br />

In 1984 he awarded with the<br />

Nobel prize.<br />

8 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

• Schalow & Townes back in 1958 : “The laser is a solution in search of problem”<br />

• Lasers have gone on to be one of the outstanding success stories in physics<br />

• Federico Capasso (inventor of QCL’s): “Laser is a solution of many problems”<br />

• Lasers were changing how we live, sometimes in ways so dramatic that one might<br />

ask, which is truth and which is the fiction?<br />

• The impact of the laser on many areas of research is very evident, making it one of<br />

the greatest achievements in modern science.<br />

• The use of lasers has become widespread not only in commercial applications but<br />

also in areas ranging from fundamental physics to chemistry, biology and medical<br />

research.<br />

• The laser technology is still rejuvenated in comparison with other great inventions.<br />

1 Maiman T.H., Nature 187, 493 – 494 (1960)


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

• It was an idea that there was on human’s mind even before its invention<br />

• Even after the construction of the laser this technology immediately hosted by the<br />

Hollywood movie producers (see Goldfinger 1964)


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

• Lasers have demonstrated a versatility & capability for constant innovation that surpasses many<br />

other main scientific discoveries:<br />

(a) Matter Lasers in Bose – Einstein condensates 1<br />

(b) The phonon laser 2 & nanolasers (10 nm thick) 6<br />

(c) Attosecond 3 & zeptosecond 4 laser pulses push the extremes of physics<br />

(d) New types of lasers: “Anything will lase if pumped hard enough”: Organic lasers (Brock<br />

et.al. 1961) & Single cell biological lasers !!!<br />

(e) High power lasers (ELI – 200 petawatts – attosecond pulses).<br />

(f) Laser facilities as PETAL that will drive the European effort to produce energy through laser<br />

fusion 5 .<br />

• 14 physics Nobel prizes have been awarded for achievements directly related or linked to<br />

lasers.<br />

1 Nature Materials 9, 374 – 375 (2010)<br />

2 Nature Physics 5, 682 – 686 (2009)<br />

3 Journal of Physics: Conference Series 194 (2009)<br />

7 http://www.nature.com/milestones/photons/<br />

8 http://www.hiper-laser.org<br />

9 Science vol 328 14 May 2010


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

• Lasers in BioPhysics: study of molecules of life such us the proteins, nucleic<br />

acids, carbonhydrates and other chemicals – see optical tweezers!!<br />

• High energy laser weapons: ABL project (equipped with a megawatt chemical<br />

oxygen – iodine laser. The new version will use diode pumped alkali metal<br />

vapours) (see video)<br />

• Solid state lasers (CW or pulsed operation 100 kW) can neutralize IED’s<br />

from a safe distance.<br />

• Free electron lasers: use special relativity to provide tunable electromagnetic<br />

radiation from a relativistic free electrons as they move through a transverse<br />

spatially periodic applied magnetic field. (see video)


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

• Lasers ( 5- 15 W) in astronomy in combination with adaptive optics


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

• The ABL project: The HiPER project:


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

• The free electron laser:


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

1) O. Svelto: Principles of Lasers<br />

2) Siegman: Lasers<br />

3) William T. Silfvast: Laser Fundamentals<br />

Historical Review<br />

1) C.H. Townes: “How the laser happened”<br />

2) M. Bertollotti: “The history of the laser”<br />

18 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

The present state of the art includes:<br />

(a) Peak powers > 10 12 W<br />

(b) Pulses shorter than 10 -15 sec


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

• Laser light unique properties: A laser is a specialized light source that should be used only<br />

when its unique properties are required.<br />

(a) Monochromatic light: (b) Spatial and temporal coherence:<br />

(c) Directional light: (d) High intensity light:


• Monochromatic:<br />

<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

Do not forget: Almost monochromatic broadening homogeneous & inhomogeneous<br />

The spectral linewidth of a laser beam it will be much narrower than the atomic<br />

transition. This is because the emission is affected by the optical cavity.<br />

• Coherence:<br />

Spatial coherence refers to whether there are irregularities in the optical phase in a<br />

cross sectional slice of the beam.<br />

Temporal coherence refers to the time duration over which the phase of the beam is<br />

well defined.<br />

t c = 1<br />

Δν


• Directionality:<br />

<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

The light comes out as a highly directional beam.<br />

• Brightness:<br />

The power per unit area is very high<br />

• Ultrashort Pulse Generation:<br />

The power duration of a laser pulse is defined by the uncertainty principle:<br />

t p ∝ 1<br />

Δν


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years


10 -21<br />

Nuclear<br />

Dynamics<br />

10-18 Atomic<br />

Dynamics<br />

10 -15<br />

Molecular<br />

Dynamics<br />

<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

10 -10<br />

Photon<br />

Creation<br />

10 -6<br />

Brown<br />

Motion<br />

Seconds<br />

10 -3<br />

10 -1<br />

Acoustics<br />

Earthquakes<br />

109 Human Life 10 16<br />

Star Life<br />

10<br />

Universe Life<br />

18


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty Brilliant Years<br />

• Gain Medium ( something to amplify the light)<br />

• Resonator (something to provide suitable optical feedback)<br />

• Pump Source (something to create the population inversion)<br />

Pump Source<br />

100% Reflector Gain Medium 98% Reflector<br />

Output beam<br />

25 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

An Introduction – Fifty brilliant years<br />

• The device consists of three essential elements:<br />

(a) External energy source or pump (b) A gain medium (c) An optical cavity or resonator<br />

• The pump is an external source that produces a population inversion in the laser gain<br />

medium.<br />

• Pumps could be: (1) Electrical (diode lasers), (2) chemical, (3) thermal , (4) optical (solid<br />

and liquid lasers)<br />

• The participating energy levels in the gain medium determine the wavelength of the laser<br />

radiation. Only in gases they have been discovered 1000 laser transitions.<br />

• Gain medium could be solid, semiconductor crystal, gas or liquid.<br />

• The most important requirement of the amplifying medium is its ability to support a<br />

population inversion between two energy levels of the laser atoms.<br />

• Due to different lifetimes of the available atomic energy levels only certain pairs of<br />

energy levels with appropriate spontaneous lifetimes can be inverted even with vigorous<br />

pumping.


• The various interactions that occur inside the atom has as a result the creation of the following energy<br />

states:<br />

Gross structure effects (1 – 10 eV)<br />

a) the kinetic energy of the electrons in their orbits around the nucleus<br />

b) the attractive electrostatic potential between the positive nucleus and the negative<br />

electrons<br />

c) the repulsive electrostatic interaction between the different electrons in the multi<br />

- electron atom<br />

Fine structure effects (0.001 – 0.01 eV): The spectral lines reveals that often coma as multiplets.<br />

a) Spin – orbit interaction<br />

Hyperfine structure effects (10 -6 – 10 -5 eV): Fine structure lines are also split into more multiplets.<br />

This splitting is due to interaction between the nucleus (spin of nucleus) and the electrons magnetic<br />

moment due to its orbital motion.<br />

<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain medium – Energy Levels


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain medium – Energy Levels<br />

• Atoms are composed by charged particles so interact with E/M radiation.<br />

• The atoms and the molecules that constitute matter have discrete energy<br />

levels (electronic, vibrational, rotational).


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Energy Levels<br />

• Laser light is the manifestation of a particular interaction between charged particles and E/<br />

M fields: An understanding of this necessitates a study of the quantization of energies of E/<br />

M fields and atoms.<br />

• The energy of E/M radiation of frequency ν is quantized in units of hν which are called<br />

photons.<br />

• The total energy stored in an E/M field of frequency ν is given by:<br />

E = 1<br />

hν + nhν<br />

2<br />

where the first right term is energy that corresponds to the electromagnetic vacuum.


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Energy Levels<br />

Bohr’s theory tried to explain the discrete emission lines of hydrogen spectrum:<br />

1. The hydrogen atom included a positively charged nucleus (proton) and a negatively charged electron<br />

orbiting in a circular motion around the nucleus.<br />

2. The electron could temporarily remain in a particular orbit if its angular momentum is a integral<br />

multiple of<br />

3. Radiation is emitted from the atom when the electron jumps from a higher energy to a lower<br />

energy level<br />

1. When a radiation is emitted its frequency can be determined by the Einstein’s equation:<br />

hν 21 = E 2 − E 1<br />

30 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Energy Levels<br />

De Broglie suggested that an electron should have wavelike properties. Thus an electron<br />

is characterised by a wavelength λ e and is rotating in orbits whose radius is an integer<br />

multiple of the electron’s wavelength.<br />

λ e = h<br />

p e<br />

The double slit experiment showed us that the electrons are not oscillating in the classical<br />

trajectories that Bohr theory suggested earlier. There is an uncertainty where the electrons<br />

are.<br />

Heisenberg’s Uncertainty Principles:<br />

31 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Energy Levels<br />

The matter consists from atoms around which the electrons move (Bohr model).<br />

The matter stability reveals that a) the electrons energy can take only specific<br />

values (quantized energy levels) and b) they move across specific orbits that<br />

each one have a specific energy.<br />

According to Schrodinger, Dirac and Heisenberg the electrons are particles<br />

with some energy and are accompanied by a probability wave function that<br />

describes the probability the electron to be in a specific orbit (eigenstate) .<br />

Each eigenstate is determined fully by three quantum numbers n, l, m<br />

32 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Energy Levels<br />

The quantum mechanics provides the appropriate probability distribution functions<br />

for the quantities of position, momentum, energy and time.<br />

Wave functions Ψ are used in order to describe various atomic parameters including<br />

the electron’s properties in an atom.<br />

The wave function by it self has no physical meaning. Multiplied by its conjugate<br />

function and a variable under consideration (e.g. position or momentum or energy)<br />

provides the probability distribution function associated with these variables.<br />

The insertion of the term of the wave-function agrees with the uncertainty principles<br />

and the wavelike properties of the electrons.<br />

33 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Energy Levels<br />

The time independent Schrodinger equation:<br />

The solutions of ψ of the Schrodinger equation are known as eigenfunctions.<br />

The time dependent Schrodinger equation describes the non stationary functions<br />

and has the following form:<br />

34 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Energy Levels<br />

Two kind of quantum states exist: The stationary and the coherent states.<br />

Each quantum state is related with an energy E n<br />

The stationary states are described by the Bohr theory. Each stationary energy<br />

state is described by its wave-function Ψ n that informs for the probability the<br />

electron to be found on a specific specific orbit around the nucleus.<br />

The time dependence of a wave function is of the form of<br />

The wave – function of a stationary state has the following form:<br />

35 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Energy Levels<br />

When the electron is in mode from changing from one specific state to lower state, the<br />

wave function must incorporate both the initial state and the final state. Thus,<br />

The probability for the electron to be in this coherent state can be represented by<br />

Ψ * * * * * *<br />

Ψ = C1 C1ψ 1ψ1<br />

+ C2C2ψ 2ψ<br />

2 + C1 C2ψ 1ψ 2e −iω 21t *<br />

+ C2C1ψ 1ψ 2e −iω 21t The solution of the Schrodinger equation allows to connect the energy of a coherent<br />

state with the corresponding wave – function.<br />

36 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Energy Levels<br />

How strong two eigenstates are related depends on the interaction among them. That<br />

interaction involves the computation of the electric dipole matrix element M if .<br />

∞<br />

Mif = ∫<br />

*<br />

Ψf erΨidV −∞<br />

The above integral is calculated over the entire volume V associated with the radiating<br />

atom. The factor er represents the electric dipole moment of the electron – proton system.<br />

The transition probability λ if depends on how well the two eigenstates interact<br />

(overlap) and on the number of various ways the transition can be occurred (is expressed<br />

by the density of the final eigenstates ρ f ).<br />

37 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Rate equations


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Rate equations<br />

• Rate equations relate the population densities to the properties of the<br />

electromagnetic field that interacts with the gain medium.<br />

• Rate equations together with equations representing the effect of a cavity on<br />

an E/M field, are used to develop a relation that predicts the output irradiance<br />

as a function of the pump, gain medium and cavity that comprises the laser<br />

system.<br />

• The Einstein coefficients are characteristic of the two energy states.


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Rate equations<br />

• Absorption<br />

An incoming photon can be absorbed by the system and an electron will be excited from<br />

the lower to the upper state.<br />

The frequency of the photon should be such that<br />

The rate at which the electrons occupy state 2 due to absorption of ‘suitable’ photon is<br />

dN 1<br />

dt = B 12ρ(ν)N 1<br />

where ρ(ν) is the photon energy density at frequency ν<br />

Β 12 is the Einstein coefficient for stimulated absorption.<br />

v 12 = E 2 − E 1<br />

h<br />

40 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium - Rate equations


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Rate equations<br />

• <strong>Stimulated</strong> <strong>Emission</strong><br />

An incoming ‘suitable’ photon can cause an electron in the upper state too relax and an<br />

additional photon with the same frequency and phase will be emitted.<br />

The stimulated emission flow of electrons from state 2 to state 1 is given by<br />

dN 2<br />

dt = −B 21ρ ν<br />

( )N 2<br />

where B 21 is the Einstein coefficient of stimulated emission.<br />

The stimulated emission is the key to the laser action but not the only action!!!.<br />

43 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Rate equations<br />

Under thermodynamic equilibrium the population of the atomic energy levels is<br />

determined by the Boltzmann distribution,<br />

N 2<br />

N 1<br />

= g 2<br />

g 1<br />

k is known as the Boltzmann constant and its value is equal to 1.38×10 -23 joule/Kelvin<br />

where g 1,2 are the degeneracies of state 1 and 2<br />

exp − E ⎡ ⎛ 2 − E1⎞ ⎤<br />

⎢<br />

⎣ ⎝ kT ⎠ ⎥<br />

⎦<br />

44 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Rate equations<br />

In thermal equilibrium the rate of change of upper and lower populations must be zero i.e.<br />

dN1 dt = dN2 dt<br />

Using the rates of the absorption, spontaneous and stimulated emission for the upper<br />

and lower energy levels in equilibrium we get<br />

ρ( ν)<br />

=<br />

A 2<br />

B12 B21 = 0<br />

B 21<br />

N 1<br />

N 2<br />

−1<br />

46 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Rate equations<br />

Replacing the Boltzmann distribution and equating the result with the density of<br />

states of the Blackbody we get,<br />

Conclusions:<br />

A 2<br />

B 21<br />

= 8πn 3 hν 3<br />

c 3 ⇒ A2 B21ρ ν<br />

g 1 B 12 = g 2 B 21<br />

(a) In order to increase substantially the stimulated emission over the spontaneous<br />

the emitted photons should be limited to a very fine spectrum region: increase<br />

( )<br />

⎛ hν⎞<br />

= exp<br />

⎝ kT⎠<br />

−1<br />

the spectral density energy. Contain the medium within a cavity!!<br />

(b) Increase the population density of the upper energy<br />

47 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Rate equations<br />

• Conclusions:<br />

(a) For stimulated emission in order to overcome photon absorption we<br />

need to achieve population inversion .<br />

(b) For stimulated emission in order to exceed spontaneous emission<br />

we must have large photon concentration which is achieved by<br />

building an optical cavity to contain photons.<br />

• Population inversion means that we depart from the situation of the<br />

thermal equilibrium. So the laser principle is based on non-thermal<br />

equilibrium.


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain medium – Small Gain Coefficient


The photons that are emitted spontaneously are incoherent to the incoming radiation and<br />

therefore they do not give useful output. The rate of change of the photons number is given<br />

by<br />

<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Small Gain Coefficient<br />

dD ν<br />

dt<br />

= ρ ν ( )B21 N2 − N [ ] 1<br />

The change of photons due to the processes of the absorption and stimulated emission is:<br />

ΔD ν =<br />

ΔD ν<br />

dt<br />

( ) − ρ( x)<br />

ρ x + dx<br />

hν<br />

= −aρ ν<br />

c<br />

( )<br />

n<br />

1<br />

hν<br />

= dI ν<br />

dx<br />

Δx n<br />

hν c = −aIνΔt 1<br />

hν ⇔<br />

52 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Small Gain Coefficient<br />

So the small gain or the absorption coefficient can be evaluated thought:<br />

Conclusion:<br />

a = B 21hνn<br />

c<br />

[ N2 − N ] 1<br />

(a) Population inversion should be established<br />

(b) A pumping source is needed<br />

(c) Gain > Loss


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Pumping Source<br />

In order to amplify the incident radiation population inversion is required .<br />

To overcome the thermal distribution of the energy states we create population<br />

inversion by pumping.<br />

The various types of pumping are:<br />

(a) Optical Pumping<br />

(b) Pumping through the energy that an exothermic chemical reaction releases<br />

(c) Electrical discharge<br />

(d) Electrical pumping<br />

54 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Laser Energy Systems<br />

Impossible to obtain population inversion with a two energy system !!! Why?


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Laser energy systems<br />

Transition a: The pump transfers population from the ground state to the higher<br />

energy level<br />

Transition b: The excited population through non radiative decay from energy<br />

level 3 to energy level 2. The lifetime of 3 is very short and all the<br />

population in state 3 decays to state 2.<br />

Transition c: <strong>Stimulated</strong> emission from state 2 to state 1. The lifetime of energy<br />

state 2 is long so population inversion to be achieved with respect to<br />

state 1. Once an inversion is obtained, stimulated emission will give<br />

optical gain<br />

56 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Laser Energy Systems<br />

In order to achieve population inversion in a three level laser system we need to<br />

pump at least the half population of the ground state to the upper laser energy level<br />

(level 2).<br />

This means that<br />

N 2 ≥ N tot<br />

2<br />

The minimum rate at which the active medium should be pumped is<br />

The main disadvantage of the three laser level system is that requires at least the half<br />

population of the ground state to be excited.<br />

R th = N tot<br />

2<br />

57 7/3/11<br />

1<br />

τ 2


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Laser Energy Systems<br />

4 Energy Level


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Laser Energy Systems<br />

The terminal state of the laser transition in a four level laser system is not the<br />

ground state and so is easier, compared to a three level system, to maintain the<br />

population inversion.<br />

It is easily observable that population inversion between states 1 and 2 can be<br />

obtained even for small populations in state 2.<br />

The required level of pumping is:<br />

R th = N th<br />

1<br />

τ 2<br />

59 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium - Threshold Point


Considering that all the losses are included into a coefficient γ the single round trip gain through<br />

the resonator and gain media is:<br />

where r 1,2 are the reflectivities of the cavity mirrors and L is the length of the gain medium.<br />

The parameter γ includes all the losses except the transmittance of the mirrors.<br />

• Loss sources:<br />

(a) Transparency of the cavity mirrors<br />

(b) Absorption and scattering in the gain medium<br />

(c) Diffraction<br />

At threshold, where G ain equals unity, the small gain coefficient can be calculated, using the<br />

above equation , as follows<br />

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Gain Medium – Threshold Point<br />

Gain = r1r2 exp{ 2(kgain − γ )L}<br />

k th = γ − 1<br />

2L ln(r 1r 2)<br />

61 7/3/11


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Gain Medium – Threshold Point<br />

The exponential gain of a laser beam is<br />

The exponential loss is defined as:<br />

Where t c is the loss cavity time. The time t is related to the length that the beam<br />

propagates through the cavity as follows,<br />

At the threshold the gain equals unity and so:<br />

k tht c<br />

I = Io exp(kx)<br />

I = Io exp(− t<br />

)<br />

τ c<br />

c<br />

n = 1 ⇒ k th = n<br />

ct c<br />

62 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain Medium – Threshold Point<br />

By manipulating the previous relations an expression for the threshold population<br />

inversion can be extracted:<br />

ΔNth = ( N2 − N ) 1 =<br />

where ΔΝ th is the inversion population at threshold.<br />

1<br />

B 21 hνt c<br />

= 8πn 3 ν 2 τ 2<br />

c 3 t c<br />

For some lasers the pump power required to attain a threshold can only be achieved for<br />

short time. These lasers are pulsed lasers.<br />

If the inversion can be maintained indefinitely the output is continuous, Such lasers are<br />

called CW lasers.<br />

63 7/3/11


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Gain Medium - Saturation<br />

If in the rate equations of the upper and lower laser levels include the effect of pumping<br />

through the pumping rate R the population inversion under thermal equilibrium is :<br />

ΔN = N 2 − N 1 =<br />

R 1− τ ⎛ ⎞ l<br />

⎜ ⎟<br />

⎝ τ u ⎠<br />

Iν 1<br />

Bul +<br />

c τ u<br />

As now the beam travels through a long length gain medium the intensity of the beam<br />

according to the Beer law will increase continuously. This means that the left factor of the<br />

denominator will continuously take higher and higher values. At a specific length<br />

(saturation length L sat ) it will reach a value that is comparable to the value of the right<br />

denominators’ parameter. At this distance from the beginning the beams’ intensity is equal<br />

to I sat (saturation intensity). 65 7/3/11<br />

≈<br />

B ul<br />

I ν<br />

c<br />

R<br />

+ 1<br />

τ u


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Gain Medium - Saturation<br />

• When saturation occurs the upper energy level population would decrease by a factor of<br />

two to a value:<br />

• From Beer’s law we know that the exponential is analogous to the population inversion.<br />

So at the saturation length the intensity of the beam will be reduced since the population<br />

inversion reduced.<br />

• Further increase in I would further decrease the gain in regions where the beam<br />

propagates further into the medium!!<br />

• As the saturation intensity we define the beam’s intensity where the stimulated emission<br />

rate becomes equal to the spontaneous emission rate, so:<br />

I sat =<br />

N u = R uτ u<br />

2<br />

c<br />

nB ul (ν)τ u<br />

66 7/3/11


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Gain Medium - Saturation<br />

67 7/3/11


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Gain medium – Saturation


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain medium – Spectral Broadening<br />

• The energy levels of atoms is not exactly discrete but they have a finite energy width<br />

ΔΕ. This width arises from the interaction of the atom with its environment.<br />

• Typical value of the energy level width is 10 -7 eV.<br />

• This energy width relaxes the restriction for a photon in order to interact with an<br />

electron should have a frequency that matches exactly the energy difference between<br />

these energy levels.<br />

• So in order to interact a photon should have an energy within the range:<br />

hν = E n − E m − ΔE n + ΔE ( m )<br />

2<br />

to hν = E n − E m + ΔE n + ΔE m<br />

( )<br />

2


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Gain medium – Spectral Broadening<br />

• From the last relationship is easily can be extracted that:<br />

ν = E n − E m<br />

h<br />

± ΔE ( n + ΔE m )<br />

2<br />

= ν o ± Δν<br />

2<br />

• The likelihood of the atom with energy levels E n and E m interacting with a photon of<br />

frequency ν is proportional to a lineshape function g(ν). It is valid that:<br />

∞<br />

∫ g( ν)<br />

dν = 1<br />

−∞


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Gain medium – Spectral Broadening


In a homogeneously broadened laser all the<br />

atoms contribute to the gain at all frequencies. As<br />

the population inversion is reduced the gain is<br />

reduced at all frequencies.<br />

The laser will oscillate at the frequency<br />

corresponding to the longitudinal mode closest<br />

to the gain maximum. When the steady state is<br />

reached only one mode will oscillate.<br />

Homogeneously broadened lasers oscillate with a<br />

single longitudinal mode.<br />

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Gain medium – Spectral Broadening<br />

72 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Gain medium – Spectral Broadening<br />

In a inhomogeneously broadened<br />

laser transition the gain saturation is<br />

stronger near the wavelength of the<br />

laser beam that is amplified<br />

through the laser gain medium.<br />

73 7/3/11


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Gain medium – Spectral Broadening


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Gain medium – Spectral Broadening<br />

75 7/3/11


From equation is easily observed that in order to increase the stimulated emission rate<br />

we need to feedback into the gain medium some of the previously emitted light e.g.<br />

increase ρ ν .<br />

<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Optical Resonator<br />

In order to provide this feedback the laser gain medium is enclosed into a laser cavity.<br />

76 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Optical Resonator<br />

Usually in the design of laser cavities curved mirrors are used instead of plane mirrors<br />

since the former laser cavities are more stable.<br />

77 7/3/11


What are the conditions for a) mirror curvature and b) mirror separation for a stable cavity?<br />

The condition, known as the stability criterion, that should be satisfied for a stable laser<br />

cavity is the following:<br />

<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Optical Resonator<br />

0 ≤ g g ≤ 1 ⇒ 0 ≤ 1− 1 2 d ⎛ ⎞<br />

⎜ ⎟ 1−<br />

⎝ ⎠<br />

d ⎛ ⎞<br />

⎜ ⎟ ≤ 1<br />

⎝ ⎠<br />

where R1,2 are the radii of curvature of the cavity mirrors, d is the length of the laser<br />

cavity and f1,2 are the focal lengths of the cavity mirrors.<br />

R 1<br />

R 2<br />

79 7/3/11


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Optical Resonator<br />

80 7/3/11


• Why Gaussian Beams?<br />

The light propagation within an cavity corresponds to a propagation<br />

through apertures that are in a distance d. The diameter of each aperture equals<br />

the mirror diameter. The beam propagation includes diffraction effects every time<br />

the beam incidents on a mirror. These diffraction affects add each other.<br />

Thus the form of the initial plane wave is altered and the initial intensity drops<br />

off due to the diffraction.<br />

Using the Fresnel – Kirchoff theory results that the above behavior is described<br />

by Gaussian shape beams.<br />

The beam maintains its Gaussian shape even during its propagation outside of the<br />

resonator.<br />

<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Optical Resonator – Stable Resonators & Gaussian Beams


A wave with a transverse Gaussian intensity propagates in a different fashion to a<br />

spherical beam. Two are the key parameters a) the beam size and b) the wave-front<br />

curvature.<br />

<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Optical Resonator – Stable Resonators & Gaussian Beams<br />

82 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Optical Resonator – Stable Resonators & Gaussian Beams<br />

The position that the beam has got the minimum transverse half width, w = w o , is<br />

called the Beam waist.<br />

The half width of a Gaussian beam across the path of propagation can be calculated<br />

through the relationship<br />

w(z) = wo 1 + λz ⎛<br />

⎜<br />

⎝<br />

2<br />

πwo where the distance z r is called the Rayleigh range where the beam waist equals the<br />

⎞<br />

⎟<br />

⎠<br />

2<br />

83 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Optical Resonator – Stable Resonators & Gaussian Beams<br />

Other useful relationships that describe the parameters of a Gaussian beam are<br />

Radius of curvature R w :<br />

Rayleigh range z r :<br />

Far field divergence angle θ:<br />

Rw ( z)<br />

= z 1 + z 2<br />

r<br />

z 2<br />

⎛ ⎞<br />

⎜ ⎟<br />

⎝ ⎠<br />

zr = πw 2<br />

on<br />

λo θ =<br />

λ o<br />

πw o n<br />

84 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Optical Resonator – Stable Resonators & Gaussian<br />

Beams<br />

For stable cavity configuration, the mirrors should be placed in a such way<br />

that they reflect the Gaussian wave-front without changing the beam<br />

parameter.<br />

The curvature of the mirrors should fit with the wavefront curvature. In<br />

other words<br />

The mirror curvature must match with the mode curvature!!<br />

85 7/3/11


Within a resonator they do not oscillate all the frequencies emitted from the<br />

transitions in the laser gain medium.<br />

The reflections back and forth result in a standing wave field to be set up within the<br />

resonator. The wavelength of the standing wave has to ‘fit’ exactly within the cavity,<br />

e.g.<br />

<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Optical Resonator - Longitudinal Modes<br />

m λ<br />

= L<br />

2<br />

86 7/3/11


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Optical Resonator - Longitudinal Modes<br />

The allowed cavity frequencies are defined from equation and are<br />

The frequency spacing between adjacent longitudinal modes of a cavity, called the<br />

Free Spectral Range (FSR) is<br />

ν m = mc<br />

2L<br />

Δν =<br />

c<br />

2nL<br />

87 7/3/11


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Optical Resonator - Longitudinal Modes<br />

88 7/3/11


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Optical Resonator - Longitudinal Modes<br />

The various mechanisms of broadening mean that the gain medium will give<br />

optical gain over continuous range of frequencies. However, the resonator will only<br />

provide feedback at the cavity mode frequencies.<br />

The output will be at one or more of the specific frequencies dictated by the cavity<br />

modes within the gain profile of the laser.<br />

A laser in which only one longitudinal mode oscillates is called SLM laser.<br />

89 7/3/11


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Optical Resonator - Longitudinal Modes<br />

90 7/3/11


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Optical Resonator - Longitudinal Modes


The intensity distribution across the width of the cavity is the Transverse Mode pattern.<br />

The transverse mode determines the beam shape. The transverse mode type depends on<br />

the cavity dimensions, reflector sizes, and other limiting apertures that may present in the<br />

cavity.<br />

The general form for the transverse electric modes is: TEM pq where p is the number on<br />

nodes in x- direction and q the respectively number of nodes in y direction.<br />

The proffered transverse mode that oscillates within the cavity depends and on:<br />

the radial dependence of the gain.<br />

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Optical Resonator - Transverse Modes<br />

A single transverse mode laser is restricted to give TEM 00 output.<br />

92 7/3/11


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Optical Resonator - Transverse Modes


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Optical Resonator - Transverse Modes<br />

94 7/3/11


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<strong>Stimulated</strong> <strong>Emission</strong> and Photon Amplification


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Pulsed Operation<br />

• Pulsed Laser Operation:<br />

(a) Observation of fast inter - atomic processes (lifetime of an excited state)<br />

(b) High Intensities (NIF & HiPER projects)


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Pulsed Operation – Q Switching<br />

• Q –Switching is a technique to produce laser pulses.<br />

• There are two types of Q-Switching: Passive & Active Q-Switching<br />

Initially:<br />

Finally:


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Pulsed Operation – Q Switching Configurations<br />

(a) Cavity dumping configuration:<br />

(b) Pocket Cell configuration:


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Pulsed Operation – Q Switching Configurations<br />

• Acousto – optic modulator:<br />

• Passive Q- Swiching:


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Pulsed Operation – Q Switching


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Pulsed Operation – Q Switching


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Pulsed Laser devices – Beyond ultrafast


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Pulsed Laser devices – Beyond ultrafast<br />

• Laser systems have steadily improved due to progress to material science<br />

and mirror technology.<br />

• Incredibly powerful lasers have been developed or are under development<br />

for laser fusion and other lasers with ultra - short pulses (attoseconds 10 -18<br />

sec) are constructing in order to monitor fast procedures within the atom!!<br />

• Attosecond technology can be used in order to monitor the charge carrier<br />

movement inside a photovoltaic cell or a transistor. This will aid to the<br />

improvement of the photovoltaic cell efficiency and the transistor speed.


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Pulsed Laser devices – Beyond ultrafast<br />

• The pulsed lasers in comparison with the continuous wave systems emit<br />

over a broad range of frequencies – billions in fact. These frequencies are<br />

timed exactly so that their electric fields nearly cancel each other except for<br />

during one tiny period of time when they constructively interfere.


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Pulsed Laser devices – Beyond ultrafast


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Pulsed Laser devices – Beyond ultrafast<br />

• The frequencies of light that exist in a laser’s resonant cavity are determined by:<br />

(a) Lasing transitions within the laser medium: is selected a medium with many<br />

different lasing transitions.<br />

From the Heisenberg’s energy time uncertainty principle, a broad band width<br />

of laser energies or frequencies is required to produce a short pulse: the greater<br />

the bandwidth, the shorter the pulse.<br />

(b) The cavity dimensions only allow light frequencies for which the electric<br />

field has nodes at the cavity’s end mirrors.


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Pulsed Laser devices – Beyond ultrafast


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Pulsed Laser devices – Beyond ultrafast<br />

• Since the pulsed lasers are alternate between a a short burst of light, known as<br />

pulse, and a much longer downtime in between, pulsed lasers can produce high<br />

peak powers (10 12 watts) : since a fixed amount of energy can be emitted<br />

within 10 -18 s<br />

• Very fast stroboscopic photography (attosecond)<br />

• Pulsed laser technology is hand to hand with non-linear optics.<br />

• Pulsed operation techniques: Mode locking & Q – Switching<br />

• In a pulsed laser system light appears at the output as pulses separated by the<br />

cavity round trip.


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Pulsed Laser devices – Beyond ultrafast


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Pulsed Laser devices – Beyond ultrafast<br />

• Shorter pulses means shorter wavelengths!!<br />

• Light pulses can not be shorter than one oscillation of the<br />

carrier electric field. At 750 nm the shortest pulse has duration<br />

equal to 2.5 fs and at XUV (12 nm) the pulse duration is<br />

smaller than 100 attosecond!!<br />

• In order to produce high power laser pulses the latter must be<br />

amplified from the nanojoules to milijoule level: Chirped<br />

Pulse Amplification


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Pulsed Laser devices – Beyond ultrafast


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Pulsed Laser devices – Attosecond Science<br />

From 1964 laser pulse duration has been<br />

decreased by about three orders of<br />

magnitude.


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Pulsed Laser devices – Attosecond Science<br />

• Attosecond science arises from research of the early 1990s into intense ultrashort – pulse atomic<br />

physics.<br />

• There are three important characteristics of the current generation of attosecond technology that imply<br />

new directions in science:<br />

(a) The technology of the electron physics can be integrated with optical<br />

technology. Spatial resolution of an electron is of the order of 1 A.<br />

(b) Attosecond photon or electron pulses are accompanied by a synchronized<br />

visible pulse of control waveform. Thus attosecond technology extends<br />

conventional ultrafast spectroscopy.<br />

(c) Attosecond photon or electron pulses have energies of 10 eV to 1 keV or beyond. Core level and<br />

multi – electron dynamics or even nuclear dynamics can be time – resolved.


<strong>Stimulated</strong> <strong>Emission</strong> <strong>Devices</strong> <strong>LASERS</strong><br />

Pulsed Laser devices – Attosecond Science<br />

Step 1: (see figure a) Ionization induced by<br />

strong NIR laser field.<br />

Step 2: (see figure b) An electron will gain<br />

kinetic energy equal to 50 – 1000 eV from the<br />

field during its first femtosecond of freedom.<br />

The kinetic energy of the electrons will determine<br />

the maximum photon energy in the emitted<br />

attosecond photon pulse. The gained kinetic<br />

energy is proportional to laser wavelength and the<br />

laser electric field amplitude.<br />

Step 3: (see figure e) Recollision. On re-<br />

encountering the core, the electron scatters from<br />

its parent ion. In addition , the recollision electron<br />

may give rise to the emission of an attosecond<br />

burst


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Pulsed Laser devices – Attosecond Science<br />

• Controlling the shape and the wavefrom of the optical pulse controls the<br />

attosecond pulse.<br />

• The above effect is depicted below:

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