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ORNL-4191 - the Molten Salt Energy Technologies Web Site

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23. Steady-State Fission Product Concentrations and<br />

Heat Generation in an MSBR and Processing Plant<br />

Concentrations of fission products and <strong>the</strong> heat<br />

generation associated with <strong>the</strong>ir decay are re-<br />

quired for design of systems €or processing <strong>the</strong><br />

fuel and fertile streams of an MSBR. A method<br />

for calculating <strong>the</strong> steady-state concentration of<br />

fission products in an MSBR will be described,<br />

and heat-generation rates in <strong>the</strong> fuel stream will<br />

be given. Changes in heat-generation rate re-<br />

sulting from removal of fission products in both<br />

<strong>the</strong> reactor and <strong>the</strong> fuel-stream processing system<br />

will be shown.<br />

Several simplifying assumptions were made in<br />

calculating <strong>the</strong> concentration of fission products<br />

in <strong>the</strong> fuel stream of an MSBR. The differential<br />

equation used to define <strong>the</strong> concentration of a<br />

given isotope was<br />

where<br />

J. S. Watson L. E. McNeese W. L. Carte1<br />

Nz,A = number of atoms of an isotope with<br />

atomic number 2 and mass number A, . .. .. . .-<br />

Vc/V, = core volume/total fuel volume,<br />

T - processing cycle time €or isotopes<br />

z with atomic number 2 (sec),<br />

t : time (sec).<br />

The reactor was assumed to be at steady state<br />

with respect to all fission products. At steady<br />

state, dN /dt -: 0; so <strong>the</strong> differential equation<br />

reduces to<br />

Z,A<br />

which defines <strong>the</strong> steady-state Concentration of<br />

each isotope. This equation was solved for each<br />

isotope using an IHM 7090. The calculations used<br />

235U yields given by Blomeke and Todd;' yields<br />

for 233U were obtained by distributing "mass<br />

yields" reported by England' among <strong>the</strong> isotopes<br />

in each mass chain so that each isotope had <strong>the</strong><br />

same fraction of <strong>the</strong> mass yield as reported for<br />

235U. Decay chains were simplified and approxi-<br />

mated by "straight" chains considering only beta<br />

decay. Where isomeric transitions or o<strong>the</strong>r<br />

complications were noted, personal judgment was<br />

used to approximate <strong>the</strong> res1 process with straight<br />

beta decay.<br />

P - power (w),<br />

Y = primary yield of isotope of atomic<br />

number and number A (atoms/<br />

' 1. 0. Rlomeke . and Marv ,- F. Todd. Umninm-235<br />

~<br />

Fission-Product Production as a Function of Thermal<br />

Neutron I'lux, Irradiation Time, and Decay Time. 1.<br />

Atomic Coricentrafions and Gross Totals, <strong>ORNL</strong>-2127<br />

f iss i on),<br />

+ = flux (neutrons sec-' cm-'),<br />

(part I.), vol. 1.<br />

'T. R. England, Time-Dependent Fission-Product<br />

(2 7 cross section of isotope with atomic<br />

%,A<br />

number 2 and mass number A (cm'),<br />

'~liemia? andKesonance Absorption Cross Sections<br />

matil Revisions azld Colculationa1 Extensions), WAPD-<br />

TM-333, addendum No. 1.<br />

245

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