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ORNL-4191 - the Molten Salt Energy Technologies Web Site

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HFIR FUEL ELLEMENT ,EXPERIMEUT<br />

194<br />

<strong>ORNL</strong>-DMIG 67-11834<br />

Fig. 15.9. Equipment Layout for Gamma Irradiation Experiment in an HFIR Fuel Element.<br />

The gamma flux of <strong>the</strong> spent fuel element used<br />

for <strong>the</strong> irradiation experiment was measured by<br />

<strong>the</strong> reduction of a 0.07. M Ce(SO,), solution irradiated<br />

in <strong>the</strong> center of <strong>the</strong> fuel element. Such measurements<br />

indicated that <strong>the</strong> gamma intensity was<br />

8.06 x lo7 dhr before <strong>the</strong> start of irradiation (6<br />

days decay time) and 2.23 x IO7 r/hr after temination<br />

of irradiation (30 days decay time).<br />

The capsule assembly was placed in <strong>the</strong> center<br />

of HFIR fuel element 9 on July 20, 1967. This<br />

element had been removed from <strong>the</strong> reactor on<br />

July 7, 1967, after 23 days of operation at 100 Mw.<br />

The salt temperature reached 32OOC from gamma<br />

heat alone (calculated to be 0.2 w/g). The assembly<br />

was removed on August 14, 1967, after<br />

600 hr (25 days) of irradiation, accumulating an<br />

estimated absorbed dose of 1.5 x ev per g of<br />

salt based on <strong>the</strong> irradiation intensity measurements<br />

described above. The temperature of <strong>the</strong><br />

fuel salt was held constant at 320GC throughout<br />

<strong>the</strong> irradiation period by adding furnace heat as<br />

<strong>the</strong> fucl element gamma flux decayed. No significant<br />

pressure change was noted; a decrease from<br />

-19 psia to I-u 18 psia appeared to be associated<br />

with <strong>the</strong> change from internal gamma heating to<br />

external electrical heating. Analysis of a sample<br />

of <strong>the</strong> argon cover gas obtained during postirradiation<br />

examination showed no evidence of radiolysis<br />

products.

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