ORNL-2106 - the Molten Salt Energy Technologies Web Site

ORNL-2106 - the Molten Salt Energy Technologies Web Site ORNL-2106 - the Molten Salt Energy Technologies Web Site

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ANP PROJECT PROGRESS REPORT Member NO.+ 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 TABLE 1.2.2. AVERAGE HEAT-GENERATION RATES IN MEMBERS OF ART NORTH HEAD Description Pressure shell (below sodium expansion tank) Liner Fuel-expansiorrtank baffle Fue I-exponsion-tank woll Upper deck (regions with sodium on both sides) Upper deck (regions with fuel on both sides) Sw irl-c hamber boff le Sw irl-c hamber wol I Lower deck (regions with fuel below and sodium above) Lower deck (regions with fuel on both sides) Copper-boron tiles F il Ier block Beryllium support struts Filler block Copper-boron tile Flat section of lower support ring Strut part of loww support ring Lower support ring *See Fig. 1.1.5, Chap. 1.1, this report, for location of member. The power-source distribution of the radioactive nuclides is found by multiplying their equilibrium concentration by their decay constant Ai and their average energy per disintegration. The total power and the power density in the gas space of the fuel expansion tank as a function of the volume of the gas and the helium flow rate are given in Fig, 1.2.3. For these calculations, A, was taken to be 5.82 x sec, which corresponds to a fuel flow rate of 22 gpm through the purging pumps. If the purging device is 36 Heat Generation (w/cm3) 4 6 w/cm3 + 16 w/cm2 on expansiondank surface due to beto roys 15 12 25 w/cm2*t + 6 w/cm3, where t = thickness of tiles (cm) 3 10 1 30 15 3 assumed to be 100% efficient, this means that the reactivity effect of the xenon is reduced to about 0.1% at equilibrium.’ The sweeping constant, A,, is dependent on the helium flow rate and the gas volume, and thus it is different for each point on the curves. In converting the STP values of the helium flow rate, the temperature of the gas was assumed to be 12OO0F, and the pressure in the expansion chamber and off-gas line was 1 e 5 18J. L. Meem, The Xenon Problem in the ART, ORNL CF-54-5-1 (May 3, 1954). P . s bi

h bd * W - EcBRc+ ORNL-LR-DWG I4918 35 I I I40 POWER DENSITY ---TOTAL WWER I - (20 I I I n 0 (00 200 300 400 500 600 700 800 VOLUME OF GAS SPACE (in3) I00 - 5 80 6 s P F 60 -1 Fig. 1.2.3. Total Power and Power Density in the Gas Space of the ART as a Function of the Gas Volume and the Helium Flow Rate for a Fuel Flow Rate of 22 gpm. taken to be 1.3 atm. The power of the reactor was assumed to be 60 Mw. In the calculation of the curves, the very short- and very long-lived nuclides of xenon and krypton (along with their decay products) were neglected. Since the fuel circulation time in the ART is less than 3 sec, nuclides with half lives less than this value will decay mostly in the fuel before it reaches the purging pumps. Thus very few atoms with half lives less than about 3 sec would get into the gas space. Also, for nuclides with long half lives (greater than about 100 hr), the number of disintegrations taking place in the fuel expansion chamber and small, since the dwell time at flow rates is very short, T may be neglected. In this study, 32 nuclides 16 of these being isotopes of and 16 being thei contributors to t daughter products themselves. In all cases, the daughter ntribute about 50 to 60% of bution. Of the total power, a is due to the beta-ray decays, with only 10% being due to gamma-ray decays. Thus, in determining the heating caused by these gases, it can be 40 20 e PERIOD ENDING JUNE 10, 1956 assumed that the heat deposition will occur mainly in a small surface layer of the materials surrounding the gases in the fuel expansion chamber and the off-gas line. The power density in the off-gas line as a function of time and gas volume for helium flow rates of 1000 and 3000 liters/day (STP) is given in Fig. 1.2.4. The time axis can be converted into lengths along the off-gas line by dividing the volume flow rate of the helium gas by the cross- sectional area of the off-gas pipe. Thus, Fig. 1.2.4 gives the power-source density of a cubic centi- meter of the gas at any position in the off-gas line. These plots were made by using the well-known equations of the decay of parent products and the buildup of their daughters as a function of time. The initial conditions at the beginning of the off-gas line were taken as the equilibrium con- ditions prevailing in the fuel expansion tank. ACTIVITIES OF NIOBIUM, MOLYBDENUM, RUTHENIUM, AND THEIR DAUGHTER PRODUCTSAFTER SHUTDOWN R. B. Stevenson The activities of the materials which will plate- out on the walls surrounding the fuel channel in the ART during reactor operation will, along with other factors, determine how long a period must elapse before reactor disassembly can proceed, The activities of the various radioactive nuclides of niobium, molybdenum, and ruthenium, and their daughter products have been determined for 100 and 300 days after shutdown and for reactor oper- ation periods of 500 and 1000 hr. These three fission products are expected to plate-out in large quantities, and therefore it has been assumed in this study that all the atoms of these elements created as fission products are plated-out. There is evidence that other fission products may plate- out; however, it is felt that the three taken into account here are the primary ones. The only isotopes of these elements that need to be considered at times greater than 100 days after shutdown are Nb95, Ru103, and Ru106. All the ather isotopes have sufficiently short half lives that they will decay appreciably in this time, and thus they may be neglected. The only daughter products that will have large activities after shutdown for more than 100 days will be Rh 03rn and Rh O6 (daughters of Ru O3 and Ru 06, respectively). 37

ANP PROJECT PROGRESS REPORT<br />

Member<br />

NO.+<br />

1<br />

2<br />

3<br />

4<br />

5<br />

6<br />

7<br />

8<br />

9<br />

10<br />

11<br />

12<br />

13<br />

14<br />

15<br />

16<br />

17<br />

18<br />

TABLE 1.2.2. AVERAGE HEAT-GENERATION RATES IN MEMBERS OF ART NORTH HEAD<br />

Description<br />

Pressure shell<br />

(below sodium expansion tank)<br />

Liner<br />

Fuel-expansiorrtank baffle<br />

Fue I-exponsion-tank woll<br />

Upper deck<br />

(regions with sodium on both sides)<br />

Upper deck<br />

(regions with fuel on both sides)<br />

Sw irl-c hamber boff le<br />

Sw irl-c hamber wol I<br />

Lower deck<br />

(regions with fuel below and sodium above)<br />

Lower deck<br />

(regions with fuel on both sides)<br />

Copper-boron tiles<br />

F il Ier block<br />

Beryllium support struts<br />

Filler block<br />

Copper-boron tile<br />

Flat section of lower support ring<br />

Strut part of loww support ring<br />

Lower support ring<br />

*See Fig. 1.1.5, Chap. 1.1, this report, for location of member.<br />

The power-source distribution of <strong>the</strong> radioactive<br />

nuclides is found by multiplying <strong>the</strong>ir equilibrium<br />

concentration by <strong>the</strong>ir decay constant Ai and <strong>the</strong>ir<br />

average energy per disintegration.<br />

The total power and <strong>the</strong> power density in <strong>the</strong><br />

gas space of <strong>the</strong> fuel expansion tank as a function<br />

of <strong>the</strong> volume of <strong>the</strong> gas and <strong>the</strong> helium flow rate<br />

are given in Fig, 1.2.3. For <strong>the</strong>se calculations,<br />

A, was taken to be 5.82 x sec, which<br />

corresponds to a fuel flow rate of 22 gpm through<br />

<strong>the</strong> purging pumps. If <strong>the</strong> purging device is<br />

36<br />

Heat Generation<br />

(w/cm3)<br />

4<br />

6 w/cm3 + 16 w/cm2 on expansiondank<br />

surface due to<br />

beto roys<br />

15<br />

12<br />

25 w/cm2*t + 6 w/cm3, where<br />

t = thickness of tiles (cm)<br />

3<br />

10<br />

1<br />

30<br />

15<br />

3<br />

assumed to be 100% efficient, this means that <strong>the</strong><br />

reactivity effect of <strong>the</strong> xenon is reduced to about<br />

0.1% at equilibrium.’ The sweeping constant,<br />

A,, is dependent on <strong>the</strong> helium flow rate and <strong>the</strong><br />

gas volume, and thus it is different for each point<br />

on <strong>the</strong> curves. In converting <strong>the</strong> STP values<br />

of <strong>the</strong> helium flow rate, <strong>the</strong> temperature of <strong>the</strong><br />

gas was assumed to be 12OO0F, and <strong>the</strong> pressure<br />

in <strong>the</strong> expansion chamber and off-gas line was<br />

1 e 5<br />

18J. L. Meem, The Xenon Problem in <strong>the</strong> ART,<br />

<strong>ORNL</strong> CF-54-5-1 (May 3, 1954).<br />

P<br />

.<br />

s<br />

bi

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