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JAERI 1287 JNDC Nuclear Data Library of Fission Products Fir

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10 <strong>JNDC</strong> Nucleai <strong>Data</strong> <strong>Library</strong> <strong>of</strong> <strong>Fission</strong> <strong>Products</strong> <strong>JAERI</strong> <strong>1287</strong><br />

values when evaluated for the whole nuclides but not the individual. The adopted data <strong>of</strong> Qp,<br />

£>and Er are given in Ref. 39 for these 87 nuclides as well as those with unknown data.<br />

2.4 <strong>Fission</strong> Yields<br />

<strong>Data</strong> <strong>of</strong> independent and cumulative yields <strong>of</strong> fission products are very important in<br />

calculation <strong>of</strong> the decay power. The experimental data are, however, far from complete,<br />

because the measured yields are a very complicated function <strong>of</strong> independent yields <strong>of</strong> the<br />

preceding nuclides in the decay chain including many short-lived nuclides. Thus it is usually<br />

difficult to compare and evaluate many measured data on yields in a region <strong>of</strong> interest even<br />

for the case <strong>of</strong> thermal-neutron fission <strong>of</strong> 235 U. Generally the individual yields have been<br />

evaluated empirically by using an appropriate theoretical assumption.<br />

The fission yield data included in the present library are based on those compiled by<br />

Rider and Meek 41) . When a new isomer is found or some isomer adopted proves not to exist,<br />

the independent yield given by Rider and Meek should be revised as will be described in this<br />

section. The cumulative yields have been calculated from the independent yields using the<br />

branching ratios adopted in our decay scheme evaluation. The fission yield data thus evaluated<br />

are those for thermal neutron fissions <strong>of</strong> 235 U, 239 Pu, 241 Pu and 233 U, fast neutron fissions <strong>of</strong><br />

235U; 238U> 239Pu and 232Th) and high-energy neutron fissions <strong>of</strong> 235 U and 238 U.<br />

In the compilation work in 1977, Rider and Meek 41) postulated that the independent<br />

yields were expressed as the symmetric Gaussian charge distribution with even-odd effects<br />

in proton and neutron pairing. They made further adjustment by taking account <strong>of</strong> available<br />

experimental data. The results were adopted in ENDF/B-IV. In the present work most <strong>of</strong> the<br />

yield data has been taken from the compilation by Rider and Meek. However it requested<br />

further information about short-lived nuclides far from stability line than theirs and up to<br />

date data on isomeric state. Thus we calculated the necessary yield values by following the<br />

treatment described in Ref. 41. The main items <strong>of</strong> the revision are summarized as follows.<br />

1) The distribution <strong>of</strong> independent yield strength between ground and isomeric states <strong>of</strong><br />

primary fission products was evaluated by Madland and England method with recent<br />

experimental data <strong>of</strong> the spin-parity values 42 ^. The values <strong>of</strong> fraction at yields for a total<br />

<strong>of</strong> 191 nuclides are tabulated in Table 2.4.1. We have used these values for all yields <strong>of</strong><br />

relevant nuclides in our file, while Rider and Meek used only a part <strong>of</strong> them.<br />

2) The increase in number <strong>of</strong> nuclides in this library is about 140 and their yields have been<br />

estimated.<br />

3) Recent experiments have denied the existence <strong>of</strong> the isomeric state <strong>of</strong> 74 As, 85 Se, 86 Rb,<br />

109 162<br />

Rh and Tb adopted in Ref. 41. Thus these isomeric states were removed and their<br />

yields were added to those <strong>of</strong> the ground states.<br />

4) The increase in number <strong>of</strong> isomeric states is 68 and the nuclides are expressed with<br />

asterisk at upper right <strong>of</strong> the names in Table 2.4.1.<br />

The equations and the parameter values used in the present evaluation will be briefly<br />

described in the following. In a given mass chain <strong>of</strong> mass number A the fractional independent<br />

yield <strong>of</strong> an isobar <strong>of</strong> atomic number Z is approximated by the symmetric Gaussian<br />

function 43 >44) as follows:<br />

o.s r (Z-Zp(A)) 2<br />

[ ^ ]dZ. (2.4.1)<br />

5 e x p [ ^<br />

where Zp (A) is the most probable charge and a the Gaussian width. The sum is given by the

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