Spatial Characterization Of Two-Photon States - GAP-Optique

Spatial Characterization Of Two-Photon States - GAP-Optique Spatial Characterization Of Two-Photon States - GAP-Optique

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4. OAM transfer in noncollinear configurations ing induced by the spatial walk-off. The symmetry breaking implies that the correlations between oam modes do not follow the relationship lp = ls + li. Figure 4.7 also shows that for larger pump beams the azimuthal changes are smoothened out. The insets in figure 4.7 show the oam decomposition at α = 90 ◦ and at α = 360 ◦ . At α = 90 ◦ , the walk-off effect compensates the noncollinear effect, and the weight of the ls = 0 mode is larger than the weight of any other mode. This angle is optimal for the generation of heralded single photons with a Gaussian shape. The degree of spatial entanglement between the photons also exhibits az- imuthal variations depending on their emission direction. Figure 4.8 shows the ] as a function of the azimuthal angle α with and with- signal purity T r[ρ2 signal out walk-off, for a pump beam waist wp = 100 µm with collection modes of ws = wi = 50 µm. When considering the walk-off, the degree of entanglement increases and becomes a function of the azimuthal angle. The purity has a minimum for α = 0◦ and α = 180◦ and maximum for α = 90◦ and α = 270◦ . The spatial azimuthal dependence affects especially those experimental configurations where photons from different parts of the cone are used, as in the case in the experiment reported in reference [12] for the generation of photons entangled in polarization. Using two identical type-i spdc crystals with the optical axes rotated 90◦ with respect to each other, the authors generated a space-frequency quantum state given by |Ψ〉 = 1 √ dqsdqi Φ 2 1 q(qs, qi)|H〉s|H〉i + Φ 2 q(qs, qi)|V 〉s|V 〉i (4.8) where Φ 1 q(qs, qi) is the spatial mode function of the photons generated in the first crystal Φ 1 q(qs, qi) = Φq(qs, qi, α = 0 ◦ ) exp [iL tan ρ0(q y s + q y i )], (4.9) and Φ 2 q(qs, qi) is the spatial mode function of the photons generated in the second crystal Φ 2 q(qs, qi) = Φq(qs, qi, α = 90 ◦ ). (4.10) Since the photons generated in the first crystal are affected by the walk-off as they pass by the second crystal, the mode functions are different. Following chapter 2, the polarization state of the generated photons is calculated by tracing out the spatial variables from equation 4.8. The resulting state is described by the density matrix where 46 ˆρp = 1 |H〉s|H〉i〈H|s〈H|i + |V 〉s|V 〉i〈V |s〈V |i 2 +c|H〉s|H〉i〈V |s〈V |i + |V 〉s|V 〉i〈H|s〈H|i (4.11) c = dqsdqiΦ 1 q(qs, qi)Φ 2 q(qs, qi). (4.12)

4.3. Effect of the Poynting vector walk-off on the OAM transfer Length 0.5mm 2mm beam waist Concurrence 1 50 500m Figure 4.9: The concurrence of the polarization entangled state given by equation 4.8 decreases when the effect of the azimuthal variation is stronger, that is for small pump beam waist or for large crystals. The degree of correlation between space and polarization is given by the purity of the polarization state T r[ρ 2 p] = 0.5 0.0 1 + |c|2 . (4.13) 2 If the walk-off effect is negligible T r[ρ 2 p] = 1, then space and polarization are not correlated. If the walk-off is not negligible, the azimuthal changes in the spatial shape are correlated with the polarization of the photons. Figure 4.9 indirectly shows the effect of the azimuthal spatial information over the polarization entanglement. The entanglement between the photons is quantified using the concurrence C = |c|, which is equal to 1 for maximally entangled states. The figure shows the variation of C as a function of the pump beam waist for two crystal lengths. For small pump beam waist, the azimuthal effect is stronger and the concurrence decreases. As the waist increases, the walk-off effect becomes weaker and the value of the concurrence increases. This effect is more important for longer crystals, where the walk-off modifies the pump beam shape more. 4.3.2 Experiment To experimentally corroborate the predicted azimuthal changes in the signal spatial shape we set up the experiment described by the parameters listed in table 4.3 and shown in figure 4.10. We used a continuous wave diode laser emitting at λp = 405 nm and with an approximate Gaussian spatial profile, obtained by using a spatial filter. A half wave plate (hwp) controlled the direction of polarization of the beam, while a lense focalized it on the input face of the crystal, with a beam waist of wp = 136 µm. The 5 mm liio3 crystal produced pairs of photons at 810 nm that propagated at ϕs,i = 4 ◦ . Due to the crystal birefringence, the pump beam exhibited a Pointing vector walk-off 47

4. OAM transfer in noncollinear configurations<br />

ing induced by the spatial walk-off. The symmetry breaking implies that the<br />

correlations between oam modes do not follow the relationship lp = ls + li.<br />

Figure 4.7 also shows that for larger pump beams the azimuthal changes are<br />

smoothened out.<br />

The insets in figure 4.7 show the oam decomposition at α = 90 ◦ and at<br />

α = 360 ◦ . At α = 90 ◦ , the walk-off effect compensates the noncollinear effect,<br />

and the weight of the ls = 0 mode is larger than the weight of any other<br />

mode. This angle is optimal for the generation of heralded single photons with<br />

a Gaussian shape.<br />

The degree of spatial entanglement between the photons also exhibits az-<br />

imuthal variations depending on their emission direction. Figure 4.8 shows the<br />

] as a function of the azimuthal angle α with and with-<br />

signal purity T r[ρ2 signal<br />

out walk-off, for a pump beam waist wp = 100 µm with collection modes of<br />

ws = wi = 50 µm. When considering the walk-off, the degree of entanglement<br />

increases and becomes a function of the azimuthal angle. The purity has a<br />

minimum for α = 0◦ and α = 180◦ and maximum for α = 90◦ and α = 270◦ .<br />

The spatial azimuthal dependence affects especially those experimental configurations<br />

where photons from different parts of the cone are used, as in the<br />

case in the experiment reported in reference [12] for the generation of photons<br />

entangled in polarization. Using two identical type-i spdc crystals with the<br />

optical axes rotated 90◦ with respect to each other, the authors generated a<br />

space-frequency quantum state given by<br />

|Ψ〉 = 1<br />

<br />

√ dqsdqi Φ<br />

2<br />

1 q(qs, qi)|H〉s|H〉i + Φ 2 <br />

q(qs, qi)|V 〉s|V 〉i<br />

(4.8)<br />

where Φ 1 q(qs, qi) is the spatial mode function of the photons generated in the<br />

first crystal<br />

Φ 1 q(qs, qi) = Φq(qs, qi, α = 0 ◦ ) exp [iL tan ρ0(q y s + q y<br />

i )], (4.9)<br />

and Φ 2 q(qs, qi) is the spatial mode function of the photons generated in the<br />

second crystal<br />

Φ 2 q(qs, qi) = Φq(qs, qi, α = 90 ◦ ). (4.10)<br />

Since the photons generated in the first crystal are affected by the walk-off as<br />

they pass by the second crystal, the mode functions are different.<br />

Following chapter 2, the polarization state of the generated photons is calculated<br />

by tracing out the spatial variables from equation 4.8. The resulting<br />

state is described by the density matrix<br />

where<br />

46<br />

ˆρp = 1<br />

<br />

|H〉s|H〉i〈H|s〈H|i + |V 〉s|V 〉i〈V |s〈V |i<br />

2<br />

<br />

+c|H〉s|H〉i〈V |s〈V |i + |V 〉s|V 〉i〈H|s〈H|i<br />

(4.11)<br />

<br />

c = dqsdqiΦ 1 q(qs, qi)Φ 2 q(qs, qi). (4.12)

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