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Documentation of the Evaluation of CALPUFF and Other Long ...

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puffs exp<strong>and</strong> until <strong>the</strong>y exceed <strong>the</strong> size <strong>of</strong> <strong>the</strong> meteorological grid cell (ei<strong>the</strong>r horizontally<br />

or vertically) <strong>and</strong> <strong>the</strong>n split into several new puffs, each with its share <strong>of</strong> <strong>the</strong> pollutant<br />

mass. In <strong>the</strong> particle model, a fixed number <strong>of</strong> particles are advected about <strong>the</strong> model<br />

domain by <strong>the</strong> mean wind field <strong>and</strong> spread by a turbulent component. The model's default<br />

configuration assumes a 3‐dimensional particle distribution (horizontal <strong>and</strong> vertical).<br />

FLEXPART 12 : The FLEXPART (Version 6.2; Siebert, 2006; Stohl et al., 2005 13 ) model is a<br />

Lagrangian particle dispersion model developed at <strong>the</strong> Norwegian Institute for Air<br />

Research in <strong>the</strong> Department <strong>of</strong> Atmospheric <strong>and</strong> Climate Research. FLEXPART was<br />

originally designed for calculating <strong>the</strong> long‐range <strong>and</strong> mesoscale dispersion <strong>of</strong> air<br />

pollutants from point sources, such as after an accident in a nuclear power plant. In <strong>the</strong><br />

meantime FLEXPART has evolved into a comprehensive tool for atmospheric transport<br />

modeling <strong>and</strong> analysis<br />

CAMx 14 : The Comprehensive Air‐quality Model with extensions (CAMx; ENVIRON, 2010) is<br />

a photochemical grid model (PGM) that simulates inert or chemical reactive pollutants<br />

from <strong>the</strong> local to continental scale. As a grid model, it simulates transport <strong>and</strong> dispersion<br />

using finite difference techniques on a three‐dimensional array <strong>of</strong> grid cells. To treat <strong>the</strong><br />

near‐source dispersion <strong>of</strong> plumes, CAMx includes a subgrid‐scale Lagrangian puff Plume‐<br />

in‐Grid (PiG) module whose mass is transferred to <strong>the</strong> grid model when <strong>the</strong> plume size is<br />

comparable to <strong>the</strong> grid size.<br />

CALGRID: The California Mesoscale Photochemical Grid Model (Yamartino, et al., 1989,<br />

Scire et al., 1989; Earth Tech, 2005) is a PGM that simulates chemically reactive pollutants<br />

from <strong>the</strong> local to regional scale. As with CAMx, it is a grid model that simulates transport<br />

<strong>and</strong> dispersion using finite differencing techniques on a three‐dimensional array <strong>of</strong> grid<br />

cells. CALGRID was originally designed to utilize meteorological fields produced by <strong>the</strong><br />

CALMET meteorological processor (Scire et al., 2000a), but was updated in 2006 to utilize<br />

meteorology <strong>and</strong> emissions in UAM format (Earth Tech, 2006).<br />

Although up to six LRT dispersion models were run for two <strong>of</strong> <strong>the</strong> tracer field experiments, a key<br />

component <strong>of</strong> this study was <strong>the</strong> evaluation <strong>of</strong> <strong>the</strong> <strong>CALPUFF</strong> model <strong>and</strong> running <strong>CALPUFF</strong> with<br />

various configurations <strong>of</strong> its meteorological drivers, CALMET <strong>and</strong> MMIF to help inform<br />

regulatory guidance on <strong>the</strong> operation <strong>of</strong> <strong>the</strong> <strong>CALPUFF</strong> system. Key to developing insight into<br />

<strong>the</strong> performance <strong>of</strong> any single model is to evaluate o<strong>the</strong>r models when configured similarly <strong>and</strong><br />

using similar meteorological databases. Table 2‐1 summarizes which LRT models were run with<br />

<strong>the</strong> four field study tracer experiments presented in this report.<br />

For <strong>the</strong> GP80 <strong>CALPUFF</strong>/CALMET application, numerous <strong>CALPUFF</strong> sensitivity tests were<br />

performed using different configurations <strong>of</strong> CALMET including with <strong>and</strong> without MM5 data <strong>and</strong><br />

use <strong>of</strong> no observations. A limited set <strong>of</strong> <strong>CALPUFF</strong> sensitivity tests were also conducted using<br />

different dispersion options. The o<strong>the</strong>r LRT models (save CALGRID) results were also evaluated<br />

for <strong>the</strong> 600 km distant arc <strong>of</strong> receptors, but are not presented in <strong>the</strong> <strong>CALPUFF</strong> comparison<br />

because this evaluation is based upon <strong>the</strong> NOAA DATEM statistical framework <strong>and</strong> is not<br />

consistent with how <strong>CALPUFF</strong> was evaluated by EPA for this experiment in 1998.<br />

12 http://transport.nilu.no/flexpart<br />

13 http://www.atmos‐chem‐phys.net/5/2461/2005/acp‐5‐2461‐2005.html<br />

14 http://www.camx.com/<br />

6

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