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Fission Product Yield Data for the Transmutation of Minor Actinide ...

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(1) Read <strong>the</strong> value plotted in Fig. 2.2.7, i.e. 25<br />

± 2 mb from <strong>the</strong> 10–50 MeV bin;<br />

(2) Apply <strong>the</strong> branching ratio correction to give<br />

25 ± 2 × 1/(1 × 0.84) = 29.8 ± 2.4 mb.<br />

The data are compared to <strong>the</strong> systematics by<br />

Wahl [2.2.7] in green. At energies above 14 MeV,<br />

Wahl uses data from 238 U(p,f) and 232 Th(p,f). The<br />

evolution <strong>of</strong> <strong>the</strong> fragment production cross-section<br />

as a function <strong>of</strong> neutron energy (excitation<br />

function) exhibits correlations with <strong>the</strong> thresholds<br />

<strong>of</strong> fission chances. However, <strong>for</strong> a given element,<br />

<strong>the</strong> behaviour differs strongly from one isotope to<br />

ano<strong>the</strong>r.<br />

2.2.4. Conclusions<br />

New data on prompt photon emission during<br />

<strong>the</strong> intermediate energy neutron induced fission <strong>of</strong><br />

238 U have been obtained. Gamma ray measurements<br />

have enabled <strong>the</strong> extraction <strong>of</strong> individual<br />

post-neutron emission fragment production<br />

excitation functions. From X ray measurements, <strong>the</strong><br />

primary fragment Z distribution has been extracted<br />

<strong>for</strong> different incident neutron energies. Although<br />

<strong>the</strong>se last results have to be finalized, <strong>the</strong>y agree<br />

quite well with calculations and o<strong>the</strong>r<br />

measurements.<br />

REFERENCES TO SECTION 2.2<br />

[2.2.1] NELSON, R., et al., Nuclear <strong>Data</strong> <strong>for</strong> Science<br />

and Technology, Italian Physics Society (1997)<br />

445.<br />

[2.2.2] ETHVIGNOT, Th., et al., A fission-fragmentsensitive<br />

target <strong>for</strong> X-ray spectroscopy in<br />

neutron-induced fission, Nucl. Instrum. Methods<br />

Phys. Res. A 490 (2002) 559–565.<br />

[2.2.3] GRANIER, Th., et al., CEA Bruyères-le-<br />

Chatel, personal communication, 2003.<br />

[2.2.4] BEARDEN, J.A., X-ray wavelengths, Rev. Mod.<br />

Phys. 39 (1967) 78–124.<br />

[2.2.5] REISDORF, W., et al., <strong>Fission</strong> fragment K X-ray<br />

emission and nuclear charge distribution <strong>for</strong><br />

<strong>the</strong>rmal neutron fission <strong>of</strong> 233 U, 235 U, 239 Pu and<br />

spontaneous fission <strong>of</strong> 252 Cf, Nucl. Phys. A 177<br />

(1971) 337–378.<br />

[2.2.6] BREISMEISTER, J., Ed., MCNP — A Monte-<br />

Carlo N-particle Transport Code, Rep. LA-<br />

12625-M, Los Alamos National Laboratory, NM<br />

(1997).<br />

[2.2.7] WAHL, A.C., Contribution to Compilation and<br />

Evaluation <strong>of</strong> <strong>Fission</strong> <strong>Yield</strong>s Nuclear <strong>Data</strong>, Rep.<br />

LA-13928, Los Alamos National Laboratory,<br />

NM (2002).<br />

[2.2.8] ZÖLLER, C.M., <strong>Fission</strong> Fragment Properties in<br />

<strong>the</strong> 238 U(n,f) Reaction at Incident Neutron<br />

Energies from 1 MeV to 500 MeV, Rep. IKDA-<br />

95/25, Technische Hochschule Darmstadt (1995).<br />

[2.2.9] CHEIFETZ, E., et al., Determination <strong>of</strong> <strong>the</strong><br />

charge and mass distribution in <strong>the</strong> fission <strong>of</strong><br />

252 Cf, Phys. Rev. C 4 (1971) 1913–1926.<br />

[2.2.10] CASOLI, P., Étude de la <strong>Product</strong>ion de<br />

Fragments dans la <strong>Fission</strong> Induite par Neutrons<br />

sur l’Uranium-238, PhD <strong>the</strong>sis, Université de<br />

Bordeaux (2003).<br />

23

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