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Fission Product Yield Data for the Transmutation of Minor Actinide ...

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FIG. 4.6.1. <strong>Fission</strong> product mass yields from 190 MeV proton induced fission <strong>of</strong> nat W, 197 Au, nat Pb and 208 Pb. The lines indicate<br />

<strong>the</strong> fitted Gaussian mass distributions; <strong>the</strong> filled circles denote <strong>the</strong> independent and cumulative yields used in <strong>the</strong> fit; triangles<br />

correspond to <strong>the</strong> experimental mass yields deduced from <strong>the</strong>se measured independent and cumulative yields.<br />

slope <strong>of</strong> <strong>the</strong> ECD lines will probably attain a value<br />

closer to <strong>the</strong> fitted slope. It is impossible to draw a<br />

conclusion as to which model gives <strong>the</strong> best<br />

predictions on <strong>the</strong> most probable charges <strong>of</strong> <strong>the</strong><br />

fission fragments.<br />

4.6.3.3. <strong>Fission</strong> in thorium<br />

4.6.3.3.1. Symmetric and asymmetric fission<br />

contributions<br />

Fitting Eq. (4.6.1) to <strong>the</strong> measured yields <strong>of</strong><br />

232 Th produces <strong>the</strong> mass yields and <strong>the</strong> mass<br />

214<br />

distribution, as shown in Fig. 4.6.4. The result is<br />

certainly not a Gaussian, as is <strong>the</strong> case <strong>for</strong> <strong>the</strong> subactinide<br />

targets. Fur<strong>the</strong>rmore, <strong>the</strong> fission crosssection<br />

obtained in this manner is 630 ± 60 mb,<br />

which is much lower than <strong>the</strong> value by Eismont et<br />

al. <strong>of</strong> 1236 mb from systematics [4.6.25]. The values<br />

<strong>of</strong> <strong>the</strong> fit parameters can be found in Table 4.6.3.<br />

Looking carefully at <strong>the</strong> 232 Th mass yields, one<br />

notices a dip around fragment mass 125. There<strong>for</strong>e,<br />

<strong>the</strong> suggestion is that <strong>the</strong> fragment mass distribution<br />

<strong>for</strong> 232 Th cannot be properly described by a single<br />

Gaussian, but ra<strong>the</strong>r is a superposition <strong>of</strong> a wide<br />

flattened distribution and a narrower Gaussian.

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