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Fission Product Yield Data for the Transmutation of Minor Actinide ...

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4.3.3. Examination <strong>of</strong> parameters<br />

Several measured mass distributions are<br />

available. The measured mass distributions were<br />

decomposed into five Gaussian functions by least<br />

squares fits. A x and s x in Eq. (4.3.2) were obtained<br />

from <strong>the</strong> decomposed Gaussian functions. R and F<br />

were calculated using <strong>the</strong> following relationships:<br />

fragment yield given by two asymmetric components<br />

R =<br />

fragment yield given by <strong>the</strong> symmetric component<br />

150<br />

Y + Y + Y + Y<br />

h h l l<br />

=<br />

Y<br />

1 2 1 2<br />

s<br />

, (4.3.5)<br />

fragment yield given by component 2<br />

F =<br />

fragment yield given by component 1<br />

Y + Y h2 l2<br />

=<br />

Y + Y<br />

h1 l1<br />

(4.3.6)<br />

where Y h1 , Y h2 , Y l1 and Y l2 are <strong>the</strong> yields <strong>of</strong> <strong>the</strong><br />

asymmetric components, and Y s is <strong>the</strong> yield <strong>of</strong> <strong>the</strong><br />

symmetric component. The resulting parameters<br />

were examined by plotting <strong>the</strong>se data against<br />

various variables such as <strong>the</strong> mass <strong>of</strong> fissioning<br />

nuclides, energy <strong>of</strong> incident particles, etc. Thus <strong>the</strong><br />

dependence <strong>of</strong> <strong>the</strong> parameters on <strong>the</strong> various<br />

variables was determined.<br />

Examples <strong>of</strong> such dependences are given in<br />

Figs 4.3.1 and 4.3.2. Figure 4.3.1 shows <strong>the</strong><br />

dependence <strong>of</strong> <strong>the</strong> R parameter on <strong>the</strong> incident<br />

particle energy. The solid circles represent yields<br />

from measured mass distributions <strong>of</strong> 238 U <strong>for</strong><br />

various incident neutron energies [4.3.3]. The<br />

behaviour <strong>of</strong> <strong>the</strong> measured data in Fig. 4.3.1<br />

suggests an energy dependence proportional to<br />

1/(E C 1 + C 2 ). The values <strong>of</strong> C 1 and C 2 were<br />

determined by least squares fit. Figure 4.3.2 shows<br />

<strong>the</strong> shell factor dependence <strong>of</strong> <strong>the</strong> R parameter,<br />

which seems to exhibit a sinusoidal dependence on<br />

<strong>the</strong> shell factor. The shell factor mentioned here is<br />

that given by Meyers and Swiatecki [4.3.4].<br />

O<strong>the</strong>r examples <strong>of</strong> <strong>the</strong> examination are<br />

illustrated in Figs 4.3.3 and 4.3.4. Figure 4.3.3 shows<br />

<strong>the</strong> energy dependence <strong>of</strong> <strong>the</strong> F parameter. Since a<br />

clear energy dependence is not evident, we assume<br />

no energy dependence <strong>for</strong> <strong>the</strong> F parameter.<br />

However, <strong>the</strong> shell factor dependence is clearly seen<br />

in Fig. 4.3.4. The F parameter is assumed to be<br />

linearly dependent on <strong>the</strong> shell factor.<br />

FIG. 4.3.1. Energy dependence <strong>of</strong> <strong>the</strong> R parameter.<br />

Derived from measured data<br />

Fitted result<br />

FIG. 4.3.2. Shell factor dependence <strong>of</strong> <strong>the</strong> R parameter.<br />

FIG. 4.3.3. Energy dependence <strong>of</strong> <strong>the</strong> F parameter.<br />

Similar examinations were per<strong>for</strong>med <strong>for</strong><br />

o<strong>the</strong>r parameters. The resulting parameters <strong>for</strong> <strong>the</strong><br />

present systematics are described below.

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