Fission Product Yield Data for the Transmutation of Minor Actinide ...

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[4.2.28] BELHAFAF, D., et al., Kinetic energy distributions around symmetric thermal fission of U 234 and U 236 , Z. Phys. A 309 (1983) 253–259. [4.2.29] WAHL, A.C., Nuclear-charge distribution and delayed-neutron yields for thermal-neutroninduced fission of 235 U, 233 U and 239 Pu and for spontaneous fission of 252 Cf, At. Data Nucl. Data Tables 39 (1988) 1–156. [4.2.30] HOWERTON, R.J., n – revisited, Nucl. Sci. Eng. 62 (1977) 438–454. [4.2.31] DJEBARA, M., et al., Mass and nuclear-charge yields for 249 Cf(n th ,f) at different fission-product kinetic energies, Nucl. Phys. A 496 (1989) 346– 366. [4.2.32] TRACY, B.L., et al., Rb and Cs isotopic cross sections from 40–60 MeV proton fission of 238 U, 232 Th and 235 U, Phys. Rev. C 5 (1972) 222–234. [4.2.33] NIKKINEN, L., Independent yields of Rb, In and Cs isotopes in the proton-induced fission of 232 Th, Phys. Rev. C 22 (1980) 617–626. [4.2.34] MANERO, F., KONSHIN, V.A., Status of the energy-dependent n – -values for the heavy isotopes (Z > 90) from thermal to 15 MeV and of n – -values for spontaneous fission, At. Energy Rev. 10 (1972) 637–756. [4.2.35] AXTON, E.J., “Evaluation of the thermal neutron constants of 233 U, 235 U, 239 Pu and 241 Pu and the fission neutron yield of 252 Cf”, Nuclear Standard Reference Data (Proc. Advisory Group Mtg Geel, 1984), IAEA-TECDOC-335, IAEA, Vienna (1985) 214–234. [4.2.36] JAMES, M.F., et al., A New Evaluation of Fission Product Yields and the Production of a New Library (UKFY2) of Independent and Cumulative Yields, Part 1, Methods and Outline of the Evaluation, Rep. AEA-TRS-1015, United Kingdom Atomic Energy Authority (1991). [4.2.37] DERUYTTER, A.J., et al., “Recent differential low energy cross sections and thermal evaluations”, Nuclear Data for the Calculation of Thermal Reactor Reactivity Coefficients (Proc. Advisory Group Mtg Vienna, 1987), IAEA- TECDOC-491, IAEA, Vienna (1989) 115–123 . [4.2.38] TERRELL, J., Neutron yields from individual fission fragments, Phys. Rev. 127 (1962) 880–904. [4.2.39] APALIN, V.F., et al., Neutron emission from U 233 , U 235 and Pu 239 fission fragments, Nucl. Phys. 71 (1965) 553–560. [4.2.40] MASLIN, E.E., et al., Prompt neutron emission from U-235 fission fragments, Phys. Rev. 164 (1967) 1520–1527. [4.2.41] BOLDEMAN, J.W., et al., Prompt neutrons from 236 U fission fragments, Aust. J. Phys. 24 (1971) 821–833. [4.2.42] MILLER, R., Fragment velocities, energies and masses from fast neutron induced fission of 235 U, Phys. Rev. C 29 (1984) 885–905. [4.2.43] BOWMAN, H.R., et al., Further studies of the prompt neutrons from the spontaneous fission of Cf-252, Phys. Rev. 129 (1963) 2133–2147. [4.2.44] SIGNARBIEUX, C., et al., “Étude expérimentale de la corrélation entre les nombres de neutrons prompts émis par les deux fragments complémentaires dans la fission spontanée de 252 Cf”, Physics and Chemistry of Fission 1973 (Proc. 3rd IAEA Symp. Rochester, NY, 1973), Vol. 2, International Atomic Energy Agency, Vienna (1974) 179–188. [4.2.45] WALSH, R.L., BOLDEMAN, J.W., Fine [4.2.46] structure in the neutron emission n(A) from 252 Cf spontaneous fission fragments, Nucl. Phys. A 276 (1977) 189–200. GINDLER, J., Dependence of neutron yield on fragment mass for several low-energy fissioning systems, Phys. Rev. C 19 (1979) 1806–1819. [4.2.47] SCHMIDT, R., HENSCHEL, H., Comparison of the spontaneous fission of 244 Cm and 252 Cf, Nucl. Phys. A 395 (1983) 29–43. [4.2.48] HENKEL, R.L., “Fission by fast neutrons”, Fast Neutron Physics, Part II (MARION, J.B., FOWLER, J.L., Eds), Interscience (1963) 2006, 2016. [4.2.49] VANDENBOSCH, R., HUIZENGA, J.R., [4.2.50] Nuclear Fission, Academic Press, New York 1973. GOLDBERG, M.D., et al., Neutron Cross Sections, Z = 61 to 87, Rep. BNL-325, Vol. IIC, 2nd edn, Supplement 2, Brookhaven National Laboratory, NY (1966). [4.2.51] BRITT, H.C., WHETSTONE, S.L., Jr., Alphaparticle-induced fission of Th230 , Th 232 and U 233 , Phys. Rev. 133 (1964) B603–B613. [4.2.52] CHEIFETZ, E., et al., Measurement of the prompt neutrons emitted in the fission of 209 Bi and 238 U induced by 155-MeV protons, Phys. Rev. C 2 (1970) 256–288. [4.2.53] DIKSIC, M., et al., Nuclear charge dispersion in mass chains 130–135 from the fission of 238U by medium energy protons, J. Inorg. Nucl. Chem. 36 (1974) 7–16. [4.2.54] SARKAR, S., YAFFE, L., Nuclear charge distribution in the region of symmetric fission of 238U by protons of energy 20–85 MeV, Can. J. Chem. 54 (1976) 2349–2358. [4.2.55] CHEIFETZ, E., FRAENKEL, Z., Prompt neutrons from fission of U-238 induced by 12 MeV protons, Phys. Rev. Lett. 21 (1968) 36–39. [4.2.56] BURNETT, S.C., et al., Neutron emission and fission energetics in the proton-induced fission of 233U and 238U, Phys. Rev. C 3 (1970) 2034–2048. [4.2.57] BISHOP, C.J., et al., Excitation energy dependence of neutron yields and fragment kinetic energy release in the proton-induced fission of 233 238 U and U, Nucl. Phys. A 150 (1970) 129–142. 147
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Fission Product Yield Data for the
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AFGHANISTAN ALBANIA ALGERIA ANGOLA
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COPYRIGHT NOTICE All IAEA scientifi
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CONTRIBUTING AUTHORS Denschlag, J.-
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3.2.1. Introduction . . . . . . . .
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6. BENCHMARK EXERCISE . . . . . . .
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However, this CRP entered an entire
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‘Provisional masses’ are determ
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Three scientists were invited to pa
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8 (d) Prompt or delayed neutron emi
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[2.1.40] ITKIS, M.G., OGANESSIAN, Y
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[2.1.96] PATE, B.D., et al., Distri
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[2.1.152] JACOBS, E., et al., Produ
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16 2.2. MEASUREMENTS OF THE ENERGY
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FIG. 2.2.3. 94 Sr: best experimenta
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FIG. 2.2.15. 132 Te: best experimen
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FIG. 2.2.27. 146 Ba: best experimen
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3. EVALUATIONS 3.1. ACTINIDE NUCLEO
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3.1.2. Statistical model At least t
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J Â K=-J 2 2 2 ^ sym Krot ( U, J)
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nuclei with N > 144. However, for h
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neutron number. The observed fissio
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FIG. 3.1.6. 235 U(n,f) fission cros
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FIG. 3.1.10. 237 Np(n,f) fission cr
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from higher fission chances [3.1.43
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[3.1.48] DUSHIN, V.N., et al., Stat
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where Y S is our new standard, and
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TABLE 3.2.2. EVALUATED REFERENCE FI
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TABLE 3.2.2. EVALUATED REFERENCE FI
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TABLE 3.2.3. EVALUATED REFERENCE YI
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TABLE 3.2.3. EVALUATED REFERENCE YI
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The comparisons of our evaluated da
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TABLE 3.2.4. COMPARISON OF RECOMMEN
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TABLE 3.2.8. COMPARISON OF THE UNCE
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REFERENCES TO SECTION 3.2 [3.2.1] I
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where N C , N U are the modified an
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activities were recorded with a pro
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3.3.4. Results and discussion The r
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FIG. 3.3.10. Li Ze et al. data: com
Page 107 and 108: 96 Annex 3.3.1 EVALUATED EXPERIMENT
Page 109 and 110: Li Ze et al. [3.3.8] Thierens et al
Page 111 and 112: 100 Annex 3.3.3 EVALUATED DATA SET
Page 113 and 114: The range of target nuclides availa
Page 115 and 116: condensation of cross-sections by t
Page 117 and 118: (h) REFERENCE (C,80KIEV,171,1980) i
Page 119 and 120: uncertainties of the calculation. T
Page 122 and 123: 4. SYSTEMATICS AND MODELS FOR THE P
Page 124 and 125: FIG. 4.1.2. 235 U total cross-secti
Page 126 and 127: FIG. 4.1.9. Total and mode separate
Page 128 and 129: 4.2. SYSTEMATICS OF FISSION PRODUCT
Page 130 and 131: A - = (PA - NT)/2 (4.2.1b) 4.2.2.3.
Page 132 and 133: FIG. 4.2.4(a). 238 U + 5.5 MeV n, L
Page 134 and 135: FIG. 4.2.8(a). U238 + 300 MeV p, LS
Page 136 and 137: TABLE 4.2.1. EQUATIONS FOR SYSTEMAT
Page 138 and 139: values (points) and the derived fun
Page 140 and 141: distributions. Values of N(A) seldo
Page 142 and 143: FIG. 4.2.19. Systematic Z P paramet
Page 144 and 145: FIG. 4.2.21. Systematic Z P paramet
Page 146 and 147: FIG. 4.2.23. Nuclear charge displac
Page 148 and 149: FIG. 4.2.24. Number of protons emit
Page 150 and 151: epresenting model values and thus s
Page 152 and 153: FIG. 4.2.36. n T(A) for CF249T. FIG
Page 154 and 155: FIG. 4.2.41. U235T, line: model; po
Page 156 and 157: The FAST subroutine in the CYFP pro
Page 160 and 161: 4.3. FIVE GAUSSIAN SYSTEMATICS FOR
Page 162 and 163: Derived from measured data Fitted r
Page 164 and 165: FIG. 4.3.7. Mass distribution of 23
Page 166 and 167: FFIG. 4.3.12. Mass distribution of
Page 168 and 169: 4.4. PHENOMENOLOGICAL MODEL FOR FRA
Page 170 and 171: where = 2mE is the wavelength, E
Page 172 and 173: FIG. 4.4.4. Fragment mass distribut
Page 176 and 177: fragment mass distributions are des
Page 180 and 181: FIG. 4.4.10. Fragment mass distribu
Page 182 and 183: P LD È Ê * E - 44. 7ˆ ˘ = Í1 +
Page 184 and 185: FIG. 4.4.13. Pre-neutron emission m
Page 186 and 187: FIG. 4.4.15. Post-neutron emission
Page 188 and 189: FIG. 4.4.17. Post-neutron emission
Page 190 and 191: fragment mass and charge distributi
Page 192 and 193: of the energy dependence of the fus
Page 194 and 195: 4.5. MODAL APPROACH TO THE DESCRIPT
Page 196 and 197: This information was used for the p
Page 198 and 199: two neighbouring isotopes at differ
Page 200 and 201: FIG.4.5.2. Experimental relative ma
Page 202 and 203: Frequently, the yields Y i (M) are
Page 204 and 205: the nine optimum description parame
Page 206 and 207: TABLE 4.5.6. RELATIVE CONTRIBUTIONS
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TABLE 4.5.8. RELATIVE CONTRIBUTIONS
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Extracted values of s 2 M,S demonst
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FIG. 4.5.10. Fission fragment charg
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FIG. 4.5.12. Unchanged charge densi
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FIG. 4.5.16. Mass yield variance fo
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FIG. 4.5.20. Experimental mass yiel
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[4.5.24] GOVERDOVSKII, A.A., MITROF
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TABLE 4.6.1. FISSION PRODUCT YIELD
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TABLE 4.6.2. FIT PARAMETER VALUES O
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FIG. 4.6.2. Charge distributions fo
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model which is elucidated elsewhere
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the agreement is better. The observ
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inner barrier is much lower than th
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e determined in a self-consistent m
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FIG. 4.6.11. Overview of the coupli
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cross-section also has to be incorp
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FIG. 4.6.16. Same as Fig. 4.6.15, b
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FIG. 4.6.20. Pre-neutron emission m
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present have a reasonable contribut
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TABLE 4.6.5. ACCURACIES OBTAINED FR
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[4.6.7] BEIJERS, J.P.M., et al., Se
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5. NEW MODELS AND SYSTEMATICS: DEFI
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therefore his benchmark calculation
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mass distributions and practically
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5.2. BENCHMARK EXERCISE 5.2.1. Benc
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thorough and detailed analysis of t
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the fissioning nucleus and the numb
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should be undertaken — such a stu
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experimental method in order to der
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256 Valley heights and peak-to-vall
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FIG. 6.2.3. Benchmark exercise, par
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260 Wahl uncert. margins Wahl uncer
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264 Wahl uncert. margins (adj. Wahl
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Wahl (1.6-160 MeV): Distributions a
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TABLE 6.2.2. 238 U PRE-NEUTRON EMIS
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as most features are very similar t
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FIG. 6.2.14. Benchmark exercise, pa
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Page 287 and 288:
Page 289 and 290:
278 REFERENCES TO SECTION 6 [6.1] B
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As mentioned above, the mass distri
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I.3.2.6. Liu Conggui et al. [I.8] M
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after prompt-neutron emission, and
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286 Zöller (1995) 89-110 MeV, post
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(1) Data were linearly interpolated
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1. 290 Annex to Appendix I RECOMMEN
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1.2. E n = 5.5 MeV 292 Nagy et al.
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1.3. E n ª 8 MeV 294 Chapman (1978
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1.5. E n = 14-15 MeV 296 Daroczy et
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1.7. E n = 27.5 (22-33) MeV, Zölle
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1.9. E n = 99.5 (89-110) MeV, Zöll
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3. 302 239 Pu NEUTRON INDUCED FISSI
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Appendix II DATA ADJUSTMENT FOR MAS
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Vivès [II.8], Zöller [II.7] and
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Annex 1 to Appendix II ADJUSTED DAT
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Zöller (1995) [II.7] E n = 13 (11.
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E n = 50 (45-55) MeV Post-neutron e
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Äystö et al. (1998) [II.9] E p =
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E n = 1.60 MeV Pre-neutron emission
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E n = 27.5 (22-33) MeV Post-neutron
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E n = 99.5 (89-110) MeV Post-neutro
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Appendix III FISSION YIELD SYSTEMAT
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FIG. III.6. Dependence of chain yie
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TABLE III.2. Ln(y)-LINEAR(E) FIT CO
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FIG. III.14. Dependence of paramete
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FIG. III.26. Comparison of the mass
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FIG. III.38. Comparison of the mass
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TABLE III.3. QUADRATIC FUNCTION FIT
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Uncertainty ratio or uncertainty Ad
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CONTENTS OF THE CD-ROM The attached
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