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Fission Product Yield Data for the Transmutation of Minor Actinide ...

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FIG. 4.2.24. Number <strong>of</strong> protons emitted be<strong>for</strong>e fission.<br />

4.2.3.7. Evaluation <strong>of</strong> systematic model estimates<br />

<strong>of</strong> yields<br />

FI and FC yields were calculated using<br />

Gaussian parameters derived from <strong>the</strong> systematic<br />

model functions in Tables 4.2.2 and 4.2.3 and<br />

compared to experimental values as ratios <strong>of</strong> <strong>the</strong><br />

two <strong>for</strong> several fission reactions. Some ratios are<br />

plotted in Figs 4.2.25–4.2.28. These figures show that<br />

<strong>the</strong> ratios cluster about 1.0, as <strong>the</strong>y should, but that<br />

a number deviate considerably from 1.0, especially<br />

<strong>for</strong> <strong>the</strong> lower experimental FI, FC values (50 MeV protons):<br />

(1) Many FI values fall above <strong>the</strong> curves as shown<br />

in Fig 4.2.30(a), contrary to <strong>the</strong> requirement<br />

that <strong>the</strong> sum <strong>of</strong> FI at unit intervals <strong>of</strong> A¢ be 1.0.<br />

FIG. 4.2.25. Ratios <strong>of</strong> Sys. F1 to Expt. F1 <strong>for</strong> U235T.<br />

FIG. 4.2.26. Ratios <strong>of</strong> Sys. F1 to Expt. F1 <strong>for</strong> CF249T.<br />

FIG. 4.2.27. Ratios <strong>of</strong> Sys. F1 to Expt. F1 <strong>for</strong> U238H.<br />

Compensation <strong>for</strong> this behaviour can be<br />

achieved by normalizing <strong>the</strong> experimental<br />

independent yield data (IN, %) so that <strong>the</strong><br />

sum <strong>for</strong> each element (Rb or Cs) equals <strong>the</strong><br />

sum from <strong>the</strong> model.<br />

137

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