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Non-dispersive wave packets in periodically driven quantum systems

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A. Buchleitner et al. / Physics Reports 368 (2002) 409–547 425<br />

carries over to <strong>quantum</strong> mechanics, and allows the creation of non-<strong>dispersive</strong> <strong>wave</strong> <strong>packets</strong>, as will<br />

be expla<strong>in</strong>ed <strong>in</strong> detail <strong>in</strong> Section 3.1.2.<br />

1.5. The <strong>in</strong>terest of non-<strong>dispersive</strong> <strong>wave</strong> <strong>packets</strong><br />

Schrod<strong>in</strong>ger dreamt of the possibility of build<strong>in</strong>g <strong>quantum</strong> <strong>wave</strong> <strong>packets</strong> follow<strong>in</strong>g classical trajectories<br />

[2]. He succeeded for the harmonic oscillator, but failed for other <strong>systems</strong> [31]. It was<br />

then believed that <strong>wave</strong> <strong>packets</strong> must spread if the system is non-l<strong>in</strong>ear, and this is correct for<br />

time-<strong>in</strong>dependent <strong>systems</strong>. However, this is not true <strong>in</strong> general, and we have seen <strong>in</strong> the previous<br />

section that clever use of the non-l<strong>in</strong>earity may, on the contrary, stabilize a <strong>wave</strong> packet and preserve<br />

it from spread<strong>in</strong>g. Such non-<strong>dispersive</strong> <strong>wave</strong> <strong>packets</strong> are thus a realization of Schrod<strong>in</strong>ger’s<br />

dream.<br />

One has to emphasize strongly that they are not some variant of the coherent states of the harmonic<br />

oscillator. They are of <strong>in</strong>tr<strong>in</strong>sically completely di erent orig<strong>in</strong>. Paradoxically, they exist only if there<br />

is some non-l<strong>in</strong>earity, i.e., some unharmonicity, <strong>in</strong> the classical system. They have some resemblance<br />

with classical solitons which are localized solutions of a non-l<strong>in</strong>ear equation that propagate without<br />

spread<strong>in</strong>g. However, they are not solitons, as they are solutions of the l<strong>in</strong>ear Schrod<strong>in</strong>ger equation.<br />

They are simply new objects.<br />

<strong>Non</strong>-<strong>dispersive</strong> <strong>wave</strong> <strong>packets</strong> <strong>in</strong> atomic <strong>systems</strong> were identi ed for the hydrogen atom exposed to<br />

a l<strong>in</strong>early polarized [32,33] and circularly polarized [34] micro<strong>wave</strong> elds quite <strong>in</strong>dependently and<br />

us<strong>in</strong>g di erent physical pictures. The former approach associated the <strong>wave</strong> <strong>packets</strong> with s<strong>in</strong>gle Floquet<br />

states localized <strong>in</strong> the vic<strong>in</strong>ity of the periodic orbit correspond<strong>in</strong>g to atom-micro<strong>wave</strong> non-l<strong>in</strong>ear<br />

resonance. The latter treatment relied on the fact that a transformation to a frame corotat<strong>in</strong>g with the<br />

micro<strong>wave</strong> eld removes the explicit time-dependence of the Hamiltonian for the circular polarization<br />

(see Section 3.4). The states localized near the equilibria of the rotat<strong>in</strong>g system were baptized<br />

“Trojan <strong>wave</strong> <strong>packets</strong>” to stress the analogy of the stability mechanism with Trojan asteroids. Such<br />

an approach is, however, restricted to a narrow class of <strong>systems</strong> where the time-dependence can be<br />

removed and lacks the identi cation of the non-l<strong>in</strong>ear resonance as the relevant mechanism. We thus<br />

prefer to use <strong>in</strong> this review the more general term “non-<strong>dispersive</strong> <strong>wave</strong> <strong>packets</strong>” not<strong>in</strong>g also that<br />

<strong>in</strong> several other papers “non-spread<strong>in</strong>g <strong>wave</strong> <strong>packets</strong>” appear equally often.<br />

Apart from their possible practical applications (for example, for the purpose of <strong>quantum</strong> control<br />

of atomic or molecular fragmentation processes [28], or for <strong>in</strong>formation storage [35–38] <strong>in</strong><br />

a con ned volume of (phase) space for long times), they show the fruitful character of classical<br />

non-l<strong>in</strong>ear dynamics. Indeed, here the non-l<strong>in</strong>earity is not a nuisance to be m<strong>in</strong>imized, but<br />

rather the essential <strong>in</strong>gredient. From complex non-l<strong>in</strong>ear dynamics, a simple object is born. The<br />

existence of such non-<strong>dispersive</strong> <strong>wave</strong> <strong>packets</strong> is extremely di cult to understand (let alone to<br />

predict) from <strong>quantum</strong> mechanics and the Schrod<strong>in</strong>ger equation alone. The classical non-l<strong>in</strong>ear<br />

dynamics po<strong>in</strong>t of view is by far more illum<strong>in</strong>at<strong>in</strong>g and predictive. It is the classical mechanics<br />

<strong>in</strong>side which led Berman and Zaslavsky [39] to the pioneer<strong>in</strong>g discussion of states associated<br />

with the classical resonance island, the subsequent studies [40–42] further identi ed such states<br />

for <strong>driven</strong> one-dimensional <strong>systems</strong> us<strong>in</strong>g the Mathieu approach without, however, discuss<strong>in</strong>g the<br />

<strong>wave</strong>-packet aspects of the states. The best proof of the importance of the classical mechanics<br />

<strong>in</strong>side is that the non-<strong>dispersive</strong> <strong>wave</strong> <strong>packets</strong> could have been discovered for a very long<br />

time (immediately after the formulation of the Schrod<strong>in</strong>ger equation), but were actually identi ed

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